Applied Physics A

, Volume 60, Issue 2, pp 191–196 | Cite as

Theory for the laser-induced femtosecond phase transition of silicon and GaAS

  • P. Stampfli
  • K. H. Bennemann
Article

Abstract

We analyze he femtosecond instability of the chamond lattice of silicon and GaAs, which is induced by a dense electron-hole plasma after excitation by a very imense laser pulse. We obtain that the electron-hole plasma causes an instability of both transverse acoustic and longitudinal optical phonons. So, within less than 200fs, the atoms are displaced more than 1 Å from their equilibrium position. The gap between the conduction and the valence band then vanishes and the symmetries of the diamond structure are destroyed, which has important effects on the optical reflectivity and second-harmonic generation. After that, the crystal melts very rapidly because of the high kinetic energy of the atoms. Note that mis is in good agreement with recent experiments done on Shand GaAs using a pump laser to excite a dense electron hole plasma and a probe laser to observe the resulting changes in the atomic and electronic structure.

PACS

61.80.Ba 63.20.-e 78.47.+p 

Preview

Unable to display preview. Download preview PDF.

Unable to display preview. Download preview PDF.

References

  1. 1.
    H.W.K. Tom, G.D. Aumiller, C.H. Brito-Cruz: Phys. Rev. Lett.60, 1438 (1988)Google Scholar
  2. 2.
    K. Sokolowski-Tinten, H. Schulz, J. Bialowski, D. von der Linde: Appl. Phys. A.53, 227 (1991)Google Scholar
  3. 3.
    C.V. Shank, R. Yen, C. Hirlimann: Phys. Rev. Lett51, 900 (1983)Google Scholar
  4. 4.
    P. Saeta, J.-K Wang, Y. Siegal, N. Bloembergen, E. Mazur: Phys. Rev. Lett.67, 1023 (1991)Google Scholar
  5. 5.
    S.V. Govorkov, T. Schroder, I.L. Shumay, P. Heist: Phys. Rev. B46, 6864 (1992)Google Scholar
  6. 6.
    S.V. Govorkov, V.I. Emelyanov, N.I. Koroteev, I.L. Shumay: J. Lumin53, 153 (1992)Google Scholar
  7. 7.
    S.V. Govorkov, I.L Shumay, W. Rudolph, T. Schroder: Opt. Lett.16, 1013 (1991)Google Scholar
  8. 8.
    P. Stampfli, K.H. Bennemann: Phys. Rev. B42, 7163 (1990)Google Scholar
  9. 9.
    P. Stampfli, K.H. Bennemann: Progr. Surf. Sci.35, 161 (1991)Google Scholar
  10. 10.
    P. Stampfli, K.H. Bennemann: Phys. Rev. B45, 10686 (1992)Google Scholar
  11. 11.
    P. Stampfli, K.H. Bennemann: Helv. Phys. Acta66, 897 (1994)Google Scholar
  12. 12.
    P. Stampfli, K.H. Bennemann: Phys. Rev. B49, 7299 (1994)Google Scholar
  13. 13.
    R.M. Martin: Phys. Rev.186, 871 (1969)Google Scholar
  14. 14.
    V. Heine, J.A. Van Vechten: Phys. Rev. B13, 1622 (1976)Google Scholar
  15. 15.
    M. Wautelet: Phys. Stat. Sol. (b)138, 447 (1986)Google Scholar
  16. 16.
    M. Wautelet, P.B. Legrand, P.M. Petropoulous: Surf. Sci.163, 230 (1985)Google Scholar
  17. 17.
    J. Bok: Phys. Lett. A.84, 448 (1981)Google Scholar
  18. 18.
    R. Biswas, V. Ambegaokar: Phys. Rev. B26, 1980 (1982)Google Scholar
  19. 19.
    C. KittelIntroduction to Solid State Physics (Wiley, New York 1953)Google Scholar
  20. 20.
    L. Kleinman: Phys. Rev.128, 2614 (1962)Google Scholar
  21. 21.
    W.A. Harrison:Electronic Structure and the Properties of Solids (Freeman, San Francisco 1980)Google Scholar
  22. 22.
    L. Rota, P. Lugli, T. Flsaesser, J. Shah: Phys. Rev. B47, 4226 (1993)Google Scholar
  23. 23.
    D.W. Snoke, W.W. Rühle, Y.-C. Lu, E. Bauser: Phys. Rev. Lett.68, 990 (1992)Google Scholar
  24. 24.
    D. Hulin, M. Combescot, J. Bok, A. Migus, J.Y Vinet, A. Antonetti: Phys. Rev. Lett.52, 1998 (1984)Google Scholar
  25. 25.
    W.H. Knox, D.S. Chemla, G. Livescu, J.E. Cunningham, J.E. Henry: Phys. Rev. Lett.61, 1290 (1988)Google Scholar
  26. 26.
    R.W. Schoenlein, W.Z. Lin, J.G. Fujimoto, G.L. Eesley: Phys. Rev. Lett.58, 1680 (1987)Google Scholar
  27. 27.
    S.D. Brorson, J.G. Fujimoto, E.P. Ippen: Phys. Rev. Lett59, 1962 (1987)Google Scholar
  28. 28.
    L.P. Kadanoff, G. Baym:Quantum Statistical Mechanics. (Benjamin, New York 1962) p. 54Google Scholar
  29. 29.
    J.A. Kash, J.C. Tsang, J.M. Hvam: Phys. Rev. Lett54, 2151 (1985)Google Scholar
  30. 30.
    A. Balderesci: Phys. Rev. B.7, 5212 (1973)Google Scholar
  31. 31.
    M. Van Schilfgaarde, A. Sher: Phys. Rev. B36, 4375 (1987)Google Scholar
  32. 32.
    D.J. Chadi: Phys. Rev. B20, 785 (1984)Google Scholar
  33. 33.
    H.B. Huntington: InSolid State Physics, ed. by F., Seitz, D. Turnbull, Vol. 7 (Academic, New York 1958)Google Scholar
  34. 34.
    G. Dolling: InInelastic Scattering of Neutrons in Solids and Liquids, Vol. II (Int'l Atomic Energy Agency, Vienna 1963) p. 37Google Scholar
  35. 35.
    O. Madelung (ed.):Semiconductors. Group IV Elements and III–V Compounds, Data Sci. Technol. (Springer, Berlin, Heidelberg 1991)Google Scholar

Copyright information

© Springer-Verlag 1995

Authors and Affiliations

  • P. Stampfli
    • 1
  • K. H. Bennemann
    • 1
  1. 1.Department of Theoretical PhysicsFreie Universität BerlinBerlinGermany

Personalised recommendations