Complex formation of trinitromethane and 1,1-dinitroethane with etheetype solvents

  • Yu. M. Golub
  • M. V. Ershov
  • V. I. Slovetskii
  • S. A. Shevelev
  • A. A. Fainzil'berg
Physical Chemistry
  • 21 Downloads

Conclusions

  1. 1.

    C-H acids of a number of polynitroalkanes with ether-type solvents form intermolecular hydrogen bonds, forming stable complexes with a 1∶1 composition.

     
  2. 2.

    The replacement of the methyl group in the α-position of C-H acids by a nitro group increases their proton donor capacity and the energy of the hydrogen bond,

     
  3. 3.

    The change in the structure of the investigated ethers-hydrogen acceptors — leads to a change in the value of the dissociation constant of the complexes and does not affect the shift of the C-D band and, consequently, the energy of the hydrogen bond.

     

Keywords

Hydrogen Methyl Hydrogen Bond Complex Formation Dissociation Constant 
These keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.

Preview

Unable to display preview. Download preview PDF.

Unable to display preview. Download preview PDF.

Literature cited

  1. 1.
    H. Ungnade, E. Roberts, and L. Kissinger, J. Phys. Chem.,68, 3225 (1964).Google Scholar
  2. 2.
    A. V. Iogansen and G. D. Litovchenko, Opt. Spek.,16, 700 (1964).Google Scholar
  3. 3.
    Sung Su, Hwei-Kwan Hong, Spectrochim. Acta,24A, 1461 (1968).Google Scholar
  4. 4.
    N. O. Cherskaya, V. I. Shilenko, V. A. Shlyapochnikov, and S. S. Novikov, Izv. Akad. Nauk SSSR, Ser. Khim., 620 (1972).Google Scholar
  5. 5.
    L. V. Okhlobystina, V. M. Khutoretskii, A. D. Naumov, and A. V. Kessenikh, Izv. Akad. Nauk SSSR, Ser. Khim., 545 (1972).Google Scholar
  6. 6.
    A. V. Iogansen, Dissertation [in Russian], Moscow (1970).Google Scholar
  7. 7.
    M. I. Bulatov and I. P. Kalinkin, Practical Handbook of Photomerric and Spectrophotometric Methcds of Analysis [in Russian], “Khimiya,” Leningrad (1972).Google Scholar
  8. 8.
    H. Shechter and H. Cates, J. Org. Chem.,26, 51 (1961).Google Scholar

Copyright information

© Plenum Publishing Corporation 1976

Authors and Affiliations

  • Yu. M. Golub
    • 1
  • M. V. Ershov
    • 1
  • V. I. Slovetskii
    • 1
  • S. A. Shevelev
    • 1
  • A. A. Fainzil'berg
    • 1
  1. 1.N. D. Zelinskii Institute of Organic ChemistryAcademy of Sciences of the USSRMoscow

Personalised recommendations