Reaction of butadiyne with amino alcohols and with amines

Communication 3. Stereochemistry of the addition of alkylamines and of dialkylamino alcohols to the triple bonds of butadiyne and 1-buten-3-ynes
  • M. F. Shostakovskii
  • I. A. Chekulaeva
  • L. V. Kondrat'eva
  • B. V. Lopatin
Organic and Biological Chemistry
  • 21 Downloads

Summary

  1. 1.

    The addition of alkylamines and of 2-dialkylaminoethanols at the triple bonds of butadiyne, N,N-diethyl-1-buten-3-ynylamine, and 2-(1-buten-3-ynyloxy)triethylamine proceeds stereospecifically with formation of the corresponding cis products in accordance with the “trans-addition” rule.

     
  2. 2.

    The reaction of N,N-diethyl-1-buten-3-ynylamine with ethanethiol is probably of free-radical character and proceeds nonstereospecifically with formation of a mixture of isomers.

     
  3. 3.

    Butadiyne does not react with arylamines at ordinary or elevated temperature.

     

Keywords

Alcohol Elevated Temperature Triethylamine Triple Bond Arylamines 
These keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.

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Literature cited

  1. 1.
    E. N. Prilezhaeva, L. V. Tsymbal, and M. F. Shostakovskii, Zh. obshch. khimii3l, No. 8, 2487 (1961).Google Scholar
  2. 2.
    M. F. Shostakovskii, I. A. Chekulaeva, L. V. Kondrat'eva, and B. V. Lopatin, Dok1. AN SSSR135, No. 1, 101 (1960).Google Scholar
  3. 3.
    M. F. Shostakovskii, I. A. Chekulaeva, and L. V. Kondrat'eva, Zh. obshch. khimii30, No. 1, 75 (1960).Google Scholar
  4. 4.
    M. F. Shostakovskii, I. A. Chekulaeva, and L. V. Kondrat'eva, Zh. obshch. khimii30, No. 10, 3179 (1960).Google Scholar

Copyright information

© Consultants Bureau Enterprises, Inc. 1963

Authors and Affiliations

  • M. F. Shostakovskii
    • 1
  • I. A. Chekulaeva
    • 1
  • L. V. Kondrat'eva
    • 1
  • B. V. Lopatin
    • 1
  1. 1.N. D. Zelinskii Institute of Organic ChemistryAcademy of SciencesUSSR

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