Abstract
The cross sections for the 63Cu(n,α)60(m+g)Co,65Cu(n,2n)64Cu, and 65Cu(n,p)65Ni reactions have been studied in the neutron energy range of 13.5–14.8 MeV using the activation technique. The neutron beams were produced via the 3H(d,n)4He reaction. The neutron energies of different directions in the measurements were determined beforehand by the method of cross section ratios for the 90Zr(n,2n)89m+gZr and 93Nb(n,2n)92mNb reactions. The results in the present work were discussed and compared with measurement results found in the literatures.
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References
Experimental Nuclear Reaction Data (EXFOR), Database Version of 2017-09-04, Nuclear Data Services. https://www-nds.iaea.org/
M.M. Rahman, S.M. Qaim, Excitation functions of some neutron threshold reactions on isotopes of molybdenum. Nucl. Phys. A 435, 43–53 (1985). https://doi.org/10.1016/0375-9474(85)90301-x
M. Bostan, S.M. Qaim, Excitation functions of threshold reactions on Sc45 and Mn55 induced by 6 to 13 MeV neutrons. Phys. Rev. C 49, 266–271 (1994). https://doi.org/10.1103/physrevc.49.266
F. Cserpák, S. Sudár, J. Csika et al., Excitation functions and isomeric cross section ratios of the Cu63(n,α)60Com, g, Cu65(n,α)62Com, g, and Ni60(n, p)60Com, g processes from 6 to 15 MeV. Phys. Rev. C 49, 1525–1533 (1994). https://doi.org/10.1103/physrevc.49.1525
C.D. Nesaraja, S. Sudár, S.M. Qaim, Cross sections for the formation of 69Znm, g and 71Znm, g in neutron induced reactions near their thresholds: effect of reaction channel on the isomeric cross-section ratio. Phys. Rev. C 68, 024603 (2003). https://doi.org/10.1103/physrevc.68.024603
V.E. Levis, K.J. Zieba, A transfer standard for d + T neutron fluence and energy. Nucl. Instrum. Methods 174, 141–144 (1980). https://doi.org/10.1016/0029-554X(80)90422-X
NuDat 2.6 (selected evaluated nuclear structure data), Decay Radiation database version of 2017-5-18, IAEA Nuclear Data Services. https://www-nds.iaea.org/
R.B. Firestone, V.S. Shirley, Table of Isotopes (Wiley, New York, 1996)
X.Z. Kong, R. Wang, Y.C. Wang et al., Cross sections for 13.5–14.7 MeV neutron induced reactions on palladium isotopes. Appl. Radiat. Isot. 50, 361–364 (1999). https://doi.org/10.1016/s0969-8043(97)10144-0
M. Wagner, H. Vonach, A. Pavlik et al., Evaluation of cross sections for 14 important neutron-dosimetry reactions. Phys. Daten Phys. Data 13–5, 183 (1990)
A.A. Filatenkov, Neutron activation cross sections measured at KRI in neutron energy region 13.4–14.9 MeV. USSR report to the INDC. No. 0460, Austria (2016). https://www-nds.iaea.org/publications/indc/indc-ccp-0460-rev.pdf
V. Semkova, A.J.M. Plompen, D.L. Smith, Measurement of the 58Ni(n,t)56Co, 59Co(n,p)59Fe, and 63Cu(n,α)60Co Reaction Cross Sections from 14 to 20 MeV. In Conference on Nuclear Data for Science and Technology, AIP Conference Proceedings 769, 1019 (2005). https://doi.org/10.1063/1.1945179
J.W. Meadows, D.L. Smith, L.R. Greenwood et al., Measurement of fast-neutron activation cross sections for copper, europium, hafnium, iron, nickel, silver, terbium and titanium at 10.0 and 14.7 MeV and for the Be(d, n) thick-target spectrum. Ann. Nucl. Energy 23, 877–899 (1996). https://doi.org/10.1016/0306-4549(95)00068-2
Y. Ikeda, C. Konno, A. Kumar, et al., Summary of activation cross sections measurements at FNS. In Conference IAEA Nuclear Data Section report to the INDC. 19–23 June, 1995. INDC(NDS)-342, 19–28.(1996). http://www-nds.iaea.org/publications/indc/indc-nds-0342/
C. Konno, Y. Ikeda, K. Oishi, et al., Activation Cross section measurements at neutron energy from 13.3 to 14.9 MeV. Japan Atomic Energy Agency (JAERI) Reports 1329 (1993). http://www-nds.iaea.org/EXFOR/22637.005
J. Csikai, C.M. Buczko, R. Pepelnik et al., Activation cross-sections related to nuclear heating of high Tc superconductors. Ann. Nucl. Energy 18, 1–4 (1991). https://doi.org/10.1016/0306-4549(91)90030-2
H.L. Lu, W.R. Zhao, W.X. Yu, et al., Activation cross section of 63Cu (n,alpha) 60Co reaction. Chin. J. Nucl. Phys. 12, 373 (1990). http://www-nds.iaea.org/EXFOR/31407.002
Y.C. Wang, J.Q. Yuan, Z.L. Ren, et al., The cross section measurement for the 63Cu (n,a) 60Co reaction. HEP & NP. 14,919 (1990). http://www-nds.iaea.org/EXFOR/32576.002
L.R. Greenwood, Recent research in neutron dosimetry and damage analysis for materials irradiations. In Conference American Society of Testing and Materials Reports 956, 743 (1987). http://www-nds.iaea.org/EXFOR/12977.016
W. Mannhart, D. Schmidt, Measurement of neutron activation cross sections in the energy range from 8 MeV to 15 MeV. Rept: Phys. Techn. Bundesanst., Neutronenphysik Reports 53 (2007). http://www-nds.iaea.org/EXFOR/22976.027
M.A. Hafiz, Measurement of excitation functions of the reactions 58Ni(n,2n) 57Ni and 65Cu(n,2n)64Cu in the neutron energy range 13.90-14.71 MeV. Indian J. Pure Appl. Phys. 45, 425 (2007). http://www-nds.iaea.org/EXFOR/31598.003
A.K.M. Harun, M.U. Khandaker, M.N. Islam et al., Measurement of cross sections for the reactions 65Cu(n,alpha)62gCo, 65Cu(n,p)65Ni, 65Cu(n,2n)64Cu, 58Ni(n,2n)57Ni and 58N(n, p)58m+gCo at 14.8 MeV neutron energy. Indian J. Phys. 80, 737 (2006). http://www-nds.iaea.org/EXFOR/31600.006
Y. Ikeda, D.L. Smith, Y. Uno et al., New Measurement of activation cross section for the 63Cu (n,2n) 62 Cu and 64Cu (n,2n) 63Cu reactions at energy range of 13.3 to 14.9 MeV. In Conference on Nuclear Data for Science and Technology, 2,944 (1994). http://www-nds.iaea.org/EXFOR/22547.004
N.I. Molla, R.U. Miah, S. Basunia et al., Cross sections of (n,p), (n,a) and (n,2n) processes on scandium, vanadium, cobalt, copper and zinc isotope in the energy range 13.57–14.71 MeV. In Conference on Nuclear Data for Science and Technology. 2,938 (1994). http://www-nds.iaea.org/EXFOR/31449.009
A. Ercan, M.N. Erduran, M. Subasi et al., 14.6 MeV neutron induced reaction cross section measurements. Nucl. Data Sci. Technol. (1992). https://doi.org/10.1007/978-3-642-58113-7_110
Y. Ikeda, C. Konno, K. Oishi, et al., Activation cross section measurements for fusion reactor structural materials at neutron energy from 13.3 to 15.0 MeV using FNS facility. JAERI Reports 1312 (1988). http://www-nds.iaea.org/EXFOR/22089.050
J.W. Meadows, D.L. Smith, M.M. Bretscher et al., Measurement of 14.7 MeV neutron-activation cross sections for fusion. Ann. Nucl. Energy 14, 489–497 (1987). https://doi.org/10.1016/0306-4549(87)90066-1
F. Ghanbari, J.C. Robertson, The 63Cu(n,2n)62Cu and 65Cu(n,2n)64Cu cross sections at 14.8 MeV. Ann. Nucl. Energy 13, 301–306 (1986). https://doi.org/10.1016/0306-4549(86)90085-x
G. Winkler, T.B. Ryves, Precise measurement of cross sections for the reaction 65Cu(n,2n)64Cu in the 14 MeV region and simultaneous reevaluation of some important cross sections at 14.70 MeV. Ann. Nucl. Energy 10, 601–606 (1983). https://doi.org/10.1016/0306-4549(83)90063-4
J. Csikai, Study of excitation functions around 14 MeV neutron energy. In Nuclear Data for Science and Technology, pp. 414–417 (1983). https://doi.org/10.1007/978-94-009-7099-1_89
Y. Uwamino, H. Sugita, Y. Kondo et al., Measurement of neutron activation cross sections of energy up to 40 MeV using semimonoenergetic p-Be neutrons. Nucl. Sci. Eng. 111, 391–403 (1992). https://doi.org/10.13182/nse111-391
R. Pepelnik, B. Anders, B.M. Bahal, et al., 14 MeV neutron activation cross sections. Rept: Ges.Kernen.-Verwertung, Schiffbau and Schiffahrt E86, 29 (1986). http://www-nds.iaea.org/EXFOR/21999.015
J.P. Gupta, H.D. Bhardwaj, R. Prasad, Pre-equilibrium emission effect in (n,p) reaction cross section at 14.8 MeV. Pramana 24, 637–642 (1985). https://doi.org/10.1007/BF02846733
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We thank the crew of the K-400 Neutron Generator at Institute of Nuclear Physics and Chemistry China Academy of Engineering Physics for performing irradiation work.
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This work was supported by the National Natural Science Foundation of China (Nos. 11575090 and 11605099) and the Young Key Teachers Training Porgram of He’nan Higher Education in China (No. 2015GGJS-258).
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Ma, JJ., Zhou, FQ., Sun, XJ. et al. Activation cross sections for reactions induced by 14 MeV neutrons on natural copper. NUCL SCI TECH 29, 150 (2018). https://doi.org/10.1007/s41365-018-0485-y
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DOI: https://doi.org/10.1007/s41365-018-0485-y