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Study of large rotating magnetocaloric effect in strongly anisotropic double perovskite Tb2CoMnO6

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Abstract

The rotating magnetocaloric effect has been researched in double perovskite Tb\(_{2}\)CoMnO\(_{6}\) by Monte Carlo simulation. The magnetization, specific heat and isothermal entropy change are presented for magnetic fields in different directions (\(h\parallel c\) and \(h\perp c\)). The rotating magnetic entropy, transition temperature and relative cooling power are given as well. Due to the different magnetic anisotropy, the spin of Co\(^{2+}\)/Mn\(^{4+}\) is parallel to c axis and the spin of Tb\(^{3+}\) is perpendicular to c axis. The corresponding A-type antiferromagnetic order appears at \(T_{C} = 94\) K, and at \(T_{N} = 15\) K, ferromagnetic state appears. Different orientations of spins result in a big negative and positive rotating magnetic entropy appeared in different temperature. Those findings may provide a wider temperature range for magnetic refrigeration applications.

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Acknowledgements

The work is supported by the National Natural Science Foundation of China (62001134), Guangxi Natural Science Foundation (2019GXNSFBA245077, 2020GXNSFAA159007, 2020GXNSFAA159047), and the Foundation of Guilin University of Aerospace Technology (XJ20KT03, XJ20KT05).

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Correspondence to W. C. Li.

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Liu, Z.Q., Li, W.C., Xie, D. et al. Study of large rotating magnetocaloric effect in strongly anisotropic double perovskite Tb2CoMnO6. Indian J Phys 96, 2017–2021 (2022). https://doi.org/10.1007/s12648-021-02162-6

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