Abstract
The current study discourses the impact of variation in PM2.5 concentration on the ambient air quality of Delhi. The 24-hourly PM2.5 concentration dataset was obtained from air quality measurement site (Anand Vihar) of Delhi Pollution Control Committee (DPCC) for the duration of April 2015 to December 2018. The annual and seasonal variability in the trend of ambient PM2.5 along with cumulative impact of meteorological parameters have been analyzed. The overall percentage increase in annual PM2.5 concentration, compared to National Ambient Air Quality Standards (NAAQS) guidelines, is observed to be 286.09%. The maximum concentration of fine particulate matter was recorded to be 788.6 µg/m3 during post-monsoon season and it was found to be associated with lower ambient temperature of 21.34°C and wind speed of 0.33 m/sec. Further, PM2.5 concentration was found to be correlated with CO (R = 0.6515) and NH3 (R = 0.6396) indicating similar sources of emission. Further, backward trajectory analysis revealed contribution in PM2.5 concentration from the states of Punjab and Haryana. The results indicated that particulate pollution is likely to occur in urban atmospheric environments with low temperatures and low wind speeds.
Research highlights
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PM2.5/PM10 ratio was observed to be highest in November, December and January, attributing aggravated levels of particle pollution to anthropogenic sources.
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Seasonal analysis of PM2.5 concentration indicated that particulate pollution was severe during post monsoon and winter months.
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Carbon monoxide (R = 0.6515; R2 = 0.4244) and Ammonia (R = 0.6396; R2 = 0.4088) were found to be correlated with PM2.5.
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Backward air mass trajectory depicted that air mass direction was coming to the receptor site (Anand Vihar) from the states of Haryana and Punjab.
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References
Badarinath K V S, Kharol S K and Sharma A R 2009 Long-range transport of aerosols from agriculture crop residue burning in Indo-Gangetic Plains – a study using LIDAR, ground measurements and satellite data; J. Atmos. Sol.-Terr. Phys. 71(1) 112–120, https://doi.org/10.1016/j.jastp.2008.0.035.
Balakrishnan K, Dey S, Gupta T, Dhaliwal R S, Brauer M, Cohen A J, Stanaway J D, Beig G, Joshi T K, Aggarwal A N and Sabde Y 2019 The impact of air pollution on deaths, disease burden, and life expectancy across the states of India: The global burden of disease study 2017; Lancet Planet. Health 3(1) 26–39, https://doi.org/10.1016/S2542-5196(18)30261-4.
Cheng Z, Luo L, Wang S, Wang Y, Sharma S, Shimadera H, Wang X, Bressi M, de Miranda R M, Jiang J and Zhou W 2016 Status and characteristics of ambient PM2.5 pollution in global megacities; Environ. Int. 89 212–221, https://doi.org/10.1016/j.envint.2016.02.003.
Cusworth D H, Mickley L J, Sulprizio M P, Liu T, Marlier M E, DeFries R S, Guttikunda S K and Gupta P 2018 Quantifying the influence of agricultural fires in northwest India on urban air pollution in Delhi, India; Environ. Res. Lett. 13(4) 044018, https://doi.org/10.1088/1748-9326/aab303.
Dang H and Unger N 2015 Contrasting regional versus global radiative forcing by megacity pollution emissions; Atmos. Environ. 119 322–329, https://doi.org/10.1016/j.atmosenv.2015.08.055.
Evagelopoulos V, Zoras S, Triantafyllou A G and Albanis T A 2006 PM10–PM2.5 time series and fractal analysis; Global NEST. J. 8(3) 234–240.
Fenger J 1999 Urban air quality; Atmos. Environ. 33(29) 4877–4900, https://doi.org/10.1016/S1352-2310(99)00290-3.
Field C B, Barros V R, Dokken D J, Mach K J, Mastrandrea M D, Bilir T E, Chatterjee M, Ebi K L, Estrada Y O, Genova R C, Girma B, Kissel E S, Levy A N, MacCracken S, Mastrandrea P R, White L L, Adger W N, Pulhin J M, Barnett J, Dabelko G D, Hovelsrud G K, Levy M Ú, Oswald S and Vogel C H 2014 Climate Change 2014: Impacts, adaptation, and vulnerability. Part A: Global and sectoral aspects; In: Contribution of Working Group II to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change, University Press, Cambridge, United Kingdom and New York, NY, USA, 1132p.
Ganguly R, Sharma D and Kumar P 2019 Trend analysis of observational PM10 concentrations in Shimla city, India; Sustain. Cities Soc. 51 101719, https://doi.org/10.1016/j.scs.2019.101719.
Ganguly R and Thapa S 2016 An assessment of ambient air quality in Shimla city; Curr. Sci. 111(3) 509–516, https://www.jstor.org/stable/24908656.
Gordon T, Balakrishnan K, Dey S, Rajagopalan S, Thornburg J, Thurston G, Agrawal A, Collman G, Guleria R, Limaye S and Salvi S 2018 Air pollution health research priorities for India: Perspectives of the Indo-US communities of researchers; Environ. Int. 119 100–108, https://doi.org/10.1016/j.envint.2018.06.013.
Goyal P 2002 Effect of winds on SO2 and SPM concentrations in Delhi; Atmos. Environ. 36(17) 2925–2930, https://doi.org/10.1016/S1352-2310(02)00218-2.
Gurjar B R, Ravindra K and Nagpure A S 2016 Air pollution trends over Indian megacities and their local-to-global implications; Atmos. Environ. 142 475–495, https://doi.org/10.1016/j.atmosenv.2016.06.030.
Guttikunda S K and Gurjar B R 2012 Role of meteorology in seasonality of air pollution in megacity Delhi, India; Environ. Monit. Assess. 184(5) 3199–3211, https://doi.org/10.1007/s10661-011-2182-8.
Guttikunda S K, Goel R and Pant P 2014 Nature of air pollution, emission sources, and management in the Indian cities; Atmos. Environ. 95 501–510, https://doi.org/10.1016/j.atmosenv.2014.07.006.
Hama S M, Kumar P, Harrison R M, Bloss W J, Khare M, Mishra S, Namdeo A, Sokhi R, Goodman P and Sharma C 2020 Four-year assessment of ambient particulate matter and trace gases in the Delhi-NCR region of India; Sustain. Cities Soc. 54 102003.
Kanawade V P, Srivastava A K, Ram K, Asmi E, Vakkari V, Soni V K, Varaprasad V and Sarangi C 2020 What caused severe air pollution episode of November 2016 in New Delhi?; Atmos. Environ. 222 117125.
Kannan G K and Kapoor J C 2004 Relationship of Sulphur dioxide and its particulate converts in urban ambient air; Indian J. Air Pollut. Control. 4(2) 1–8.
Kumar A, Singh D, Singh B P, Singh M, Anandam K, Kumar K and Jain V K 2015 Spatial and temporal variability of surface ozone and nitrogen oxides in urban and rural ambient air of Delhi-NCR, India; Air Qual. Atmos. Heath. 8(4) 391–399, https://doi.org/10.1007/s11869-014-0309-0.
Kumar P, Jain S, Gurjar B R, Sharma P, Khare M, Morawska L and Britter R 2013 New directions: Can a ‘blue sky’ return to Indian mega cities?; Atmos. Environ. 71 198–201, https://doi.org/10.1016/j.atmosenv.2013.01.055.
Khanum F, Chaudhry M N and Kumar P 2017 Characterization of five-year observation data of fine particulate matter in the metropolitan area of Lahore; Air Qual. Atmos. Heath. 10(6) 725–736, https://doi.org/10.1007/s11869-017-0464-1.
Khan M A H, Lowe D, Derwent R G, Foulds A, Chhantyal-Pun R, McFiggans G and Shallcross D E 2020 Global and regional model simulations of atmospheric ammonia; Atmos. Res. 234 104702, https://doi.org/10.1016/j.atmosres.2019.104702.
Laakso L, Koponen I K, Mönkkönen P, Kulmala M, Kerminen V M, Wehner B, Wiedensohler A, Wu Z and Hu M 2006 Aerosol particles in the developing world: A comparison between New Delhi in India and Beijing in China; Water Air Soil Pollut. 173(1–4) 5–20, https://doi.org/10.1007/s11270-005-9018-5.
Lin Y, Zou J, Yang W and Li C Q 2018 A review of recent advances in research on PM2.5 in China; Int. J. Environ. Res. Public Health. 15(3) 438, https://doi.org/10.3390/ijerph15030438.
Littlejohn D, Wang Y and Chang S G 1993 Oxidation of aqueous sulfite ion by nitrogen dioxide; Environ. Sci. Technol. 27(10) 2162–2167, https://doi.org/10.1021/es00047a024.
Mallik C, Ghosh D, Ghosh D, Sarkar U, Lal S and Venkataramani S 2014 Variability of SO2, CO, and light hydrocarbons over a megacity in Eastern India: Effects of emissions and transport; Environ. Sci. Pollut. Res. 21(14) 8692–8706, https://doi.org/10.1007/s11356-014-2795-x.
Mayer H 1999 Air pollution in cities; Atmos. Environ. 33 4029–4037, https://doi.org/10.1016/S1352-2310(99)00144-2.
Mishra A K and Shibata T 2012 Synergistic analyses of optical and microphysical properties of agricultural crop residue burning aerosols over the Indo-Gangetic Basin (IGB); Atmos. Environ. 57 205-218, https://doi.org/10.1016/j.atmosenv.2012.04.025.
Mohan M and Bhati S 2009 Why is megacity Delhi prone to high atmospheric pollution potential?; In: TFMM-TF HTAP Joint Workshop, Paris, http://www.htap.org/meetings/2009/2009_06/presentations/tfhtap-20090618-am/mmohan-06-18.pdf.
Mohan M and Payra S 2009 Influence of aerosol spectrum and air pollutants on fog formation in urban environment of megacity Delhi, India; Environ. Monit. Assess. 151(1–4) 265–277, https://doi.org/10.1007/s10661-008-0268-8.
Monks P S, Granier C, Fuzzi S, Stohl A, Williams M L, Akimoto H, Amann M, Baklanov A, Baltensperger U, Bey I and Blake N 2009 Atmospheric composition change – global and regional air quality; Atmos. Environ. 43(33) 5268–5350, https://doi.org/10.1016/j.atmosenv.2009.08.021.
Mukherjee T, Asutosh A, Pandey S K, Yang L, Gogoi P P, Panwar A and Vinoj V 2018 Increasing potential for air pollution over megacity New Delhi: A study based on 2016 Diwali episode; Aerosol Air Qual. Res. 18(9) 2510–2518, https://doi.org/10.4209/aaqr.2017.11.0440.
Murari V, Kumar M, Mhawish A, Barman S C and Banerjee T 2017 Airborne particulate in Varanasi over middle Indo-Gangetic Plain: Variation in particulate types and meteorological influences; Environ. Monit. Assess 189(4) 157, https://doi.org/10.1007/s10661-017-5859-9.
New Delhi, India, Central Pollution Control Board (CPCB) 2008 National ambient air quality status NAAQMS//2009–10; http://www.indiaenvironmentportal.org.in/files/Air-Report-2008.pdf.
New Delhi (India), ENVIS Centre on Control of Pollution (Water, Air, & Noise) 2016 Air pollution in Delhi: An analysis; http://cpcbenvis.nic.in/envis_newsletter/Air pollution in Delhi.pdf.
New Delhi (India), Planning Department, Government of National Capital Territory of Delhi 2019 Economic Survey of Delhi 2018–2019; http://delhiplanning.nic.in/content/economic-survey-delhi-2018-19.
Patidar S and Afghan F R 2019 Influence of meteorological parameters on PM2.5 concentrations in the NCT Delhi; Indian conference on geotechnical and geo-environmental engineering (ICGGE-2019), MNNIT Allahabad, Prayagraj, India, 01–02 March 2019, https://www.researchgate.net/publication/336614550_INFLUENCE_OF_METEOROLOGICAL_PARAMETERS_ON_PM25_CONCENTRATION_IN_THE_NCT_OF_DELHI.
Payra S, Kumar P, Verma S, Prakash D and Soni M 2016 Potential source identification for aerosol concentrations over a site in northwestern India; Atmos. Res. 169(A) 65–72, https://doi.org/10.1016/j.atmosres.2015.09.022.
Pillai P S, Babu S S and Moorthy K K 2002 A study of PM, PM10 and PM2.5 concentration at a tropical coastal station; Atmos. Res. 61(2) 149–167, https://doi.org/10.1016/S0169-8095(01)00136-3.
Prasad A K, Singh R P and Kafatos M 2006 Influence of coal based thermal power plants on aerosol optical properties in the Indo‐Gangetic basin; Geophys. Res. Lett. 33(5), https://doi.org/10.1029/2005GL023801.
Pope III C A and Dockery D W 2006 Health effects of fine particulate air pollution: Lines that connect; J. Air Waste Manag. Assoc. 56(6) 709–742, http://dx.doi.org/10.1080/10473289.2006.10464485.
Prakash D, Payra S, Verma S and Soni M 2013 Aerosol particle behavior during dust storm and Diwali over an urban location in northwestern India; Nat. Hazards 69(3) 1767–1779.
Querol X, Alastuey A, Rodriguez S, Plana F, Ruiz C R, Cots N, Massagué G and Puig O 2001 PM10 and PM2.5 source apportionment in the Barcelona metropolitan area Catalonia Spain; Atmos. Environ. 35(36) 6407–6419.
Ramanathan V, Li F, Ramana M V, Praveen P S, Kim D, Corrigan C E, Nguyen H, Stone E A, Schauer J J, Carmichael G R and Adhikary B 2007 Atmospheric brown clouds: Hemispherical and regional variations in long‐range transport, absorption, and radiative forcing; J. Geophys. Res.: Atmos. 112(D22), https://doi.org/10.1029/2006JD008124.
Rolph G, Stein A and Stunder B 2017 Real-time environmental applications and display system; Environ. Modell. Softw. 95 210–228, https://doi.org/10.1016/j.envsoft.2017.06.025.
Saliba N A, El Jam F, El Tayar G, Obeid W and Roumie M 2010 Origin and variability of particulate matter (PM10 and PM2.5) mass concentrations over an Eastern Mediterranean city; Atmos. Res. 97(1–2) 106–114, https://doi.org/10.1016/j.atmosres.2010.03.011.
Sarkar S, Singh R P and Chauhan A 2018 Crop residue burning in northern India: Increasing threat to Greater India; J. Geophys. Res.: Atmos. 123(13) 6920–6934, https://doi.org/10.1029/2018JD028428.
Satheesh S K and Ramanathan V 2000 Large differences in tropical aerosol forcing at the top of the atmosphere and Earth’s surface; Nature 405(6782) 60–63, https://doi.org/10.1038/35011039.
Sati A P and Mohan M 2014 Analysis of air pollution during a severe smog episode of November 2012 and the Diwali Festival over Delhi India; Int. J. Remote Sens. 35(19) 6940–6954.
Seinfeld J H and Pandis S N 1998 Atmospheric chemistry and physics. From air pollution to climate change; New York, Wiley.
Seinfeld J H and Pandis S N 2016 Atmospheric Chemistry and Physics: From air pollution to climate change (3rd edn), John Wiley & Sons, Inc., Hoboken, New Jersey.
Sharma A K, Baliyan P and Kumar P 2018 Air pollution and public health: The challenges for Delhi, India; Rev. Environ. Health. 33(1) 77–86, https://doi.org/10.1515/reveh-2017-0032.
Sharma A R, Kharol S K, Badarinath K V S and Singh D 2010 Impact of agriculture crop residue burning on atmospheric aerosol loading – a study over Punjab State, India; Ann. Geophys. 28(2) 367–379, https://doi.org/10.5194/angeo-28-367-2010.
Sharma M, Kaskaoutis D G, Singh R P and Singh S 2014 Seasonal variability of atmospheric aerosol parameters over Greater Noida using ground sunphotometer observations; Aerosol Air Qual. Res. 14(3) 608–622, https://doi.org/10.4209/aaqr.2013.06.0219.
Soni M, Payra S and Verma S 2018 Particulate matter estimation over a semi-arid region Jaipur, India using satellite AOD and meteorological parameters; Atmos. Pollut. Res. 9(5) 949–958, https://doi.org/10.1016/j.apr.2018.03.001.
Stein A F, Draxler R R, Rolph G D, Stunder B J B, Cohen M D and Ngan F 2015 NOAA’s HYSPLIT atmospheric transport and dispersion modeling system; Bull. Am. Meteorol. Soc. 96 2059–2077, http://dx.doi.org/10.1175/BAMS-D-14-00110.1.
Stocker T F, Qin D, Plattner G-K, Tignor M, Allen S K, Boschung J, Nauels A, Xia Y, Bex V and Midgley P M 2013 IPCC: Climate change 2013: The physical science basis; In: Contribution of Working Group I to the Fifth Assessment Report of the Intergovernmental Panel on Climate Change, Cambridge University Press, Cambridge, UK and New York, NY, USA, 1535p.
Sugimoto N, Shimizu A, Matsui I and Nishikawa M 2016 A method for estimating the fraction of mineral dust in particulate matter using PM2.5-to-PM10 ratios; Particuology 28 114–120, https://doi.org/10.1016/j.partic.2015.09.005.
Tiwari S, Srivastava A K, Bisht D S, Parmita P, Srivastava M K and Attri S D 2013 Diurnal and seasonal variations of black carbon and PM2.5 over New Delhi, India: Influence of meteorology; Atmos. Res. 125 50–62.
Trinh T T, Trinh T T, Le T T and Tu B M 2019 Temperature inversion and air pollution relationship, and its effects on human health in Hanoi City, Vietnam; Environ. Geochem. Health 41(2) 929–937, https://doi.org/10.1007/s10653-018-0190-0.
Venkataraman C, Habib G, Eiguren-Fernandez A, Miguel A H and Friedlander S K 2005 Residential biofuels in South Asia: Carbonaceous aerosol emissions and climate impacts; Science 307(5714) 1454–1456.
Verma S, Payra S, Gautam R, Prakash D, Soni M, Holben B and Bell S 2013 Dust events and their influence on aerosol optical properties over Jaipur in northwestern India; Environ. Monit. Assess. 185(9) 7327–7342, https://doi.org/10.1007/s10661-013-3103-9.
Vijayakumar K, Safai P D, Devara P C S, Rao S V B and Jayasankar C K 2016 Effects of agriculture crop residue burning on aerosol properties and long-range transport over northern India: A study using satellite data and model simulations; Atmos. Res. 178 155–163, https://doi.org/10.1016/j.atmosenv.2012.04.025.
Wang Y, Wang M, Zhang R, Ghan S J, Lin Y, Hu J, Pan B, Levy M, Jiang J H and Molina M J 2014 Assessing the effects of anthropogenic aerosols on Pacific storm track using a multiscale global climate model; Proc. Natl. Acad. Sci. 111(19) 6894–6899, https://doi.org/10.1073/pnas.1403364111.
WHO 2006 Air quality guidelines: Global update 2005; Geneva: World Health Organization, http://www.euro.who.int.
Zheng S, Cao C X and Singh R P 2014 Comparison of ground based indices (API and AQI) with satellite based aerosol products; Sci. Total Environ. 488 398–412, https://doi.org/10.1016/j.scitotenv.2013.12.074.
Zheng S, Singh R P, Wu Y and Wu C 2017 A comparison of trace gases and particulate matter over Beijing (China) and Delhi (India); Water Air Soil Pollut. 228(5) 181, https://doi.org/10.1007/s11270-017-3360-2.
Zoran M A, Savastru R S, Savastru D M and Penache M C V 2019 Temporal trends of carbon monoxide (CO) and radon (222Rn) tracers of urban air pollution; J. Radioanal. Nucl. Chem. 320(1) 55–70, https://doi.org/10.1007/s10967-019-06443-7.
Acknowledgements
The authors wish to express their sincere thanks to Central Pollution Central Board (CPCB) for providing the pollutant concentration dataset and meteorological parameter dataset over Anand Vihar, Delhi. In addition, the authors gratefully acknowledge the NOAA Air Resources Laboratory (ARL) for the provision of the HYSPLIT transport and dispersion model and/or READY website (https://www.ready.noaa.gov) used in this publication. The authors wish to express sincere thanks for the financial support from Indian Space Research Organization under Respond program, Government of India (ISRO/RES/3/806/19-20).
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Janhavi Singh and Priyanshu Gupta did write-up and statistical analysis of paper. Data collection was done by Deepak Gupta. Dr. Swagata Payra and Dr. Divya Prakash carried review of the manuscript. Overall, paper supervised and conceptualised by Dr. Sunita Verma. Each author had participated sufficiently in the work to take public responsibility for appropriate portions of the content. All the authors read and approved the final manuscript.
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Singh, J., Gupta, P., Gupta, D. et al. Fine particulate pollution and ambient air quality: A case study over an urban site in Delhi, India. J Earth Syst Sci 129, 226 (2020). https://doi.org/10.1007/s12040-020-01495-w
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DOI: https://doi.org/10.1007/s12040-020-01495-w