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Dielectric and ferroelectric properties evolution of (1−x)(Bi0.5Na0.5TiO3)–xK0.5Na0.5NbO3 piezoceramics

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Abstract

In this work, piezoceramics of (1−x)(Bi0.5Na0.5)TiO3–x(K0.5Na0.5)NbO3, (1−x)BNT–xKNN, in the compositional range 0.00 ≤ x ≤ 0.07, were prepared by a mechanochemically activated solid-state method. The structural phase formation and microstructural, dielectric, and ferroelectric properties were studied. Although changes, in symmetry of the perovskite structure, were not detected with the composition (i.e., from a perspective of its intrinsic properties), the microstructural evolution was strongly dependent on the content of the KNN phase (i.e., based on its extrinsic properties). Specifically, KNN favoured the formation of a microstructure with cubic grains, typical morphology of the alkaline niobate ceramics. After KNN addition, both the maximum permittivity temperature and the long-range to short-range ordered transition temperature were reduced. Additionally, ferroelectric loops and strain deformation curves also reflect the long-range to short-range order evolution with KNN addition and temperature.

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Acknowledgements

This work has been possible with the help of the National Council of Scientific and Technical Research (CONICET), the National Agency for Scientific and Technological Promotion (ANPCyT, PICT2014-1314) and the National University of Mar del Plata (UNMdP, 15/G527) and thanks to them for their economic and institutional support. Dr F Rubio-Marcos is also indebted to the MINECO (Spain) project MAT2017-86450-C4-1-R for their financial support. FR-M is indebted to MINECO for a ‘Ramon y Cajal’ contract (ref: RyC-2015-18626), which is co-financed by the European Social Fund. FR-M also acknowledges support from a 2018 Leonardo Grant for Researchers and Cultural Creators, BBVA Foundation.

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Authors and Affiliations

  1. Institute of Research in Materials Science and Technology (INTEMA), Av. Colón 10850, B7606BWV, Mar del Plata, Argentina

    A PRADO, L RAMAJO & M S CASTRO

  2. Electroceramic Department, Instituto de Cerámica y Vidrio, CSIC, Kelsen 5, 28049, Madrid, Spain

    F RUBIO-MARCOS

  3. Escuela Politécnica Superior, Universidad Antonio de Nebrija, Pirineos 55, 28040, Madrid, Spain

    F RUBIO-MARCOS

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  1. A PRADO
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  4. M S CASTRO
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Correspondence to M S CASTRO.

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PRADO, A., RUBIO-MARCOS, F., RAMAJO, L. et al. Dielectric and ferroelectric properties evolution of (1−x)(Bi0.5Na0.5TiO3)–xK0.5Na0.5NbO3 piezoceramics. Bull Mater Sci 43, 282 (2020). https://doi.org/10.1007/s12034-020-02246-9

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  • DOI: https://doi.org/10.1007/s12034-020-02246-9

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