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Low-temperature CO oxidation of Pt/Al0.1Ce0.9O x catalysts: Effects of supports prepared with different precipitants

  • Catalysis, Reaction Engineering
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Korean Journal of Chemical Engineering Aims and scope Submit manuscript

Abstract

We prepared 0.1Al-0.9Ce supports using various precipitants such as NH4OH, KOH, NaOH, K2CO3, and Na2CO3 to prepare Pt-based CO oxidation catalysts. Of the studied catalysts, the Pt/0.1Al-0.9Ce_NH4OH catalyst showed the optimum activity for CO oxidation. Catalysts prepared with carbonate-form precipitants revealed relatively lower activity than carbonate-free precipitants. A temperature at 50% CO conversion of all samples was observed in the low-temperature region in the presence of water vapor because of the promotional effect of the water-gas shift reaction. Several characterization results revealed that catalytic activity was related to oxygen capacity and Pt dispersion was attributable to precipitant nature.

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Authors and Affiliations

  1. Greenhouse Gas Resources Research Group, Korea Research Institute of Chemical Technology, Daejeon, 34114, Korea

    Jung-Hyun Park & Tae-Sun Chang

  2. Department of Chemical Engineering, Chungbuk National University, Cheongju, Chungbuk, 28644, Korea

    Hyeryeung Noh & Chae-Ho Shin

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  1. Jung-Hyun Park
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  2. Hyeryeung Noh
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Correspondence to Chae-Ho Shin.

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Park, JH., Noh, H., Chang, TS. et al. Low-temperature CO oxidation of Pt/Al0.1Ce0.9O x catalysts: Effects of supports prepared with different precipitants. Korean J. Chem. Eng. 35, 645–653 (2018). https://doi.org/10.1007/s11814-017-0343-3

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