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Fabrication and Characterization of Al2O3 Particles Reinforced Ni-P-Polytetrafluoroethylene Nanocomposite Coating by Jet Electrodeposition

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Abstract

In order to achieve the purpose of material surface strengthening and protection, Ni-P-Al2O3-PTFE nanocomposite coatings were prepared by jet electrodeposition, and the effect of Al2O3 nanoparticle concentration in the plating solution on the microstructure and mechanical properties of the composite coatings was investigated. The surface morphology, microstructure, wear resistance and elastoplasticity of the composite coatings were characterized by x-ray diffractometer, scanning electron microscope, energy-dispersive spectrometer, friction and wear tester and nanoindenter. The experimental results show that the deposition of Al2O3 nanoparticles can significantly improve the comprehensive properties of the composite coating. When the addition amount of Al2O3 sol in the plating solution is 40 ml/L, the surface morphology of the composite coating is uniform and dense, the content of Al and F elements reaches the maximum value of 1.49 and 0.77 wt.%, the average friction coefficient and wear scar width reach the minimum value of 0.1456 and 131.40 μm, and the elastic recovery ratio (he/hmax) reaches the maximum value of 0.32. At this time, the nanocomposite coating exhibits excellent wear resistance and toughness. The development of this research will have a positive effect in the field of preparation and optimization of nanocomposite coatings.

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References

  1. S. Roy, B.M. Mishra, and G.K. Bose, Characterization of Ni-P Based Poly-Alloy and Composite Coatings Involving Nanoindentation and Nanoscratch Tests, Mater. Today Commun., 2021, 29, p 102991. https://doi.org/10.1016/j.mtcomm.2021.102991

    Article  CAS  Google Scholar 

  2. A.P. Meshram, M.K. Punith Kumar, and C. Srivastava, Enhancement in Anti-Corrosive Behavior of Ni-P Coatings by Incorporation of Carbon Nanotubes, J. Mater. Eng. Perform., 2021, 31, p 1573–1584. https://doi.org/10.1007/s11665-021-06260-8

    Article  CAS  Google Scholar 

  3. T. Rabizadeh, S.R. Allahkaram, and A. Zarebidaki, An Investigation on Effects of Heat Treatment on Corrosion Properties of Ni-P Electroless Nano-Coatings, Mater. Design, 2010, 31, p 3174–3179. https://doi.org/10.1016/j.matdes.2010.02.027

    Article  CAS  Google Scholar 

  4. S. Sharma, S. Sharma, A. Sharma, and V. Agarwala, Co-Deposition of Synthesized ZnO Nanoparticles into Ni-P Matrix Using Electroless Technique and Their Corrosion Study, J. Mater. Eng. Perform., 2016, 25, p 4383–4393. https://doi.org/10.1007/s11665-016-2292-0

    Article  CAS  Google Scholar 

  5. M. Rostami, A. Fahami, B. Nasiri-Tabrizi, R. Ebrahimi-Kahrizsangi, and A. Saatchi, Characterization of Electrodeposited Ni-SiC-Cg Nanocomposite Coating, Appl. Surf. Sci., 2013, 265, p 369–374. https://doi.org/10.1016/j.apsusc.2012.11.014

    Article  CAS  Google Scholar 

  6. C.M. Pacheco, B.A. Cecilia, G. Reyes, C. Oviedo, A. Fernández-Pérez, M. Elso, and O.J. Rojas, Nanocomposite Additive of SiO2/TiO2/Nanocellulose on Waterborne Coating Formulations for Mechanical and Aesthetic Properties Stability on Wood, Mater. Today Commun., 2021, 29, p 102990. https://doi.org/10.1016/j.mtcomm.2021.102990

    Article  CAS  Google Scholar 

  7. A. Kumar and A.K. Das, Correction to: Development of Al-Ni-TiC Composite Coating on Commercially Pure Al Using Tungsten Inert Gas Welding Route and its Wear Behavior, J. Mater. Eng. Perform., 2022, 31, p 5332. https://doi.org/10.1007/s11665-022-06801-9

    Article  CAS  Google Scholar 

  8. D.J. Liu, B.L. Jiang, Z. Liu, Y.F. Ge, and Y.M. Wang, Preparation and Catalytic Properties of Cu2O-CoO/Al2O3 Composite Coating Prepared on Aluminum Plate by Microarc Oxidation, Ceram. Int., 2014, 40, p 9981–9987. https://doi.org/10.1016/j.ceramint.2014.02.096

    Article  CAS  Google Scholar 

  9. S.F. Shi, S. Cho, T. Goto, and T. Sekino, The Effects of Sintering Temperature on Mechanical and Electrical Properties of Al2O3/Ti Composites, Mater. Today Commun., 2020, 25, p 101522. https://doi.org/10.1016/j.mtcomm.2020.101522

    Article  CAS  Google Scholar 

  10. S.A. Lajevardi, T. Shahrabi, and J.A. Szpunar, Tribological Properties of Functionally Graded Ni-Al2O3 Nanocomposite Coating, J. Electrochem. Soc., 2017, 164, p D275–D281. https://doi.org/10.1149/2.0731706jes

    Article  CAS  Google Scholar 

  11. S. Aslan and E. Duru, Microstructure and Wear Properties of Electrodeposited Ni-B-Al2O3 Composite Coating on Low Carbon Steel at Elevated Temperature, J. Mater. Eng. Perform., 2022, 31, p 1693–1704. https://doi.org/10.1007/s11665-021-06290-2

    Article  CAS  Google Scholar 

  12. S. Karthikeyan and B. Ramamoorthy, Effect of Reducing Agent and nano Al2O3 Particles on the Properties of Electroless Ni-P Coating, Appl. Surf. Sci., 2014, 307, p 654–660. https://doi.org/10.1016/j.apsusc.2014.04.092

    Article  CAS  Google Scholar 

  13. X.Y. Wang, F. Liu, Y. Song, Z.K. Liu, and D. Qin, Structure and Properties of Al2O3 Coatings Formed on NiTi alloy by Cathodic Plasma Electrolytic Deposition-Science Direct, Surf. Coat. Tech., 2016, 285, p 128–133. https://doi.org/10.1016/j.surfcoat.2015.11.034

    Article  CAS  Google Scholar 

  14. B.H. Park, M.H. Lee, B.K. Sang, and Y.M. Jo, Evaluation of the Surface Properties of PTFE Foam Coating Filter Media Using XPS and Contact Angle Measurements, Appl. Surf. Sci., 2011, 257, p 3709–3716. https://doi.org/10.1016/j.apsusc.2010.11.116

    Article  CAS  Google Scholar 

  15. H.Y. Wang, L. Yan, D. Gao, D.J. Liu, C. Wang, L.Y. Sun, and Y.J. Zhu, Tribological Properties of Superamphiphobic PPS/PTFE Composite Coating in the Oilfield Produced Water, Wear, 2014, 319, p 62–68. https://doi.org/10.1016/j.wear.2014.07.012

    Article  CAS  Google Scholar 

  16. E. Mortezanejad, M. Atapour, H. Salimijazi, A. Alhaji, and A. Hakimizad, Wear and Corrosion Behavior Of Aluminate-and Phosphate-Based Plasma Electrolytic Oxidation Coatings with Polytetrafluoroethylene Nanoparticles on AZ80 Mg Alloy, J. Mater. Eng. Perform., 2021, 30, p 4030–4044. https://doi.org/10.1007/s11665-021-05803-3

    Article  CAS  Google Scholar 

  17. H.H. Sheu, S.Y. Jian, M.H. Lin, C. Hsu, K.H. Hou, and M.D. Ger, Electroless Ni-P/PTFE Self-Lubricating Composite thin Films Applied for Medium-Carbon Steel Substrate, Int. J. Electrochem. Sc., 2017, 12, p 5464–5482. https://doi.org/10.20964/2017.06.30

    Article  CAS  Google Scholar 

  18. N. Jiang and C.Q. Fu, Research on the Microstructure and Tribological Properties of the Electroless Ni-P-PTFE Composite Repairing Coating on Gears, Appl. Mech. Mater., 2013, 327, p 136–139. https://doi.org/10.4028/www.scientific.net/AMM.327.136

    Article  Google Scholar 

  19. T.C. Chen, S.R. Ge, H.T. Liu, Q.H. Sun, W. Zhu, W. Yan, and J.W. Qi, Fabrication of Low Adhesive Superhydrophobic Surfaces Using Nano Cu/Al2O3 Ni-Cr Composited Electro-Brush Plating, Appl. Surf. Sci., 2015, 356, p 81–90. https://doi.org/10.1016/j.apsusc.2015.08.045

    Article  CAS  Google Scholar 

  20. Y.K. Liu, Q.L. Lu, Z. Huang, S.Q. Sun, B. Yu, U. Evariste, and G.H. Jiang ang J.M. Yao, Electrodeposition of Ni-Co-S Nanosheet Arrays on N-Doped Porous Carbon Nanofibers for Flexible Asymmetric Supercapacitors, J. Alloy. Compd., 2018, 762, p 301–311. https://doi.org/10.1016/j.jallcom.2018.05.239

    Article  CAS  Google Scholar 

  21. J.E. Park, Y.S. Jang, S.Y. Kim, J.B. Choi, T.S. Bae, I.S. Park, and M.H. Lee, Corrosion Properties and Biocompatibility of Strontium Doped Calcium Phosphate Coated Magnesium Prepared by Electrodeposition, Mater. Today Commun., 2022, 31, p 103759. https://doi.org/10.1016/j.mtcomm.2022.103759

    Article  CAS  Google Scholar 

  22. M. Cao, X. Zhang, J. Ren, Y. Sun, and N. Dai, Chemical Bath Deposition of SnS:Cu/ZnS for Solar Hydrogen Production and Solar Cells, J. Alloy. Compd., 2012, 863, p 158727. https://doi.org/10.1016/j.jallcom.2021.158727

    Article  CAS  Google Scholar 

  23. G.P. Sklar, K. Paramguru, M. Misra, and J.C. Lacombe, Pulsed Electrodeposition into AAO Templates for CVD Growth of Carbon Nanotube Arrays, Nanotechnology, 2015, 16, p 1265–1271. https://doi.org/10.1088/0957-4484/16/8/047

    Article  CAS  Google Scholar 

  24. R. Levinas, N. Tsyntsaru, and H. Cesiulis, Insights into Electrodeposition and Catalytic Activity of MoS2 for Hydrogen Evolution Reaction Electrocatalysis, Electrochim. Acta, 2019, 317, p 427–436. https://doi.org/10.1016/j.electacta.2019.06.002

    Article  CAS  Google Scholar 

  25. R.V. Prataap and S. Mohan, Electrodeposition of Ni-La2O3 Composite on AA6061 Alloy and its Enhanced Hardness, Corrosion Resistance and Thermal Stability, Surf. Coat. Tech., 2017, 324, p 471–477. https://doi.org/10.1016/j.surfcoat.2017.06.011

    Article  CAS  Google Scholar 

  26. A. Zoikis-Karathanasis, E.A. Pavlatou, and N. Spyrellis, Pulse Electrodeposition of Ni-P Matrix Composite Coatings Reinforced by SiC Particles, J. Alloy. Compd., 2010, 494, p 396–403. https://doi.org/10.1016/j.jallcom.2010.01.057

    Article  CAS  Google Scholar 

  27. Y.B. Zhong, P.W. Zhou, J.F. Zhou, H. Wang, L.J. Fan, L.C. Dong, T.X. Zheng, and W.W. Shen, Study on the Pulse Reverse Electrodeposition of Fe-Nano-Si Composite Coatings in Magnetic Field, Appl. Surf. Sci., 2014, 309, p 278–284. https://doi.org/10.1016/j.apsusc.2014.05.030

    Article  CAS  Google Scholar 

  28. M.K. Camargo, I. Tudela, U. Schmidt, A.J. Cobley, and A. Bund, Ultrasound Assisted Electrodeposition of Zn and Zn-TiO2 Coatings, Electrochim. Acta, 2016, 198, p 287–295. https://doi.org/10.1016/j.electacta.2016.03.078

    Article  CAS  Google Scholar 

  29. X.L. Chen, J.S. Chen, K.K. Saxena, J.J. Zhu, X.L. Gu, and Z.N. Guo, Localization of Jet Electrochemical Additive Manufacturing With a Liquid Confinement Technique, J. Manuf. Process., 2022, 81, p 48–64. https://doi.org/10.1016/j.jmapro.2022.06.053

    Article  Google Scholar 

  30. W. Cui, K. Wang, F. Xia, and P. Wang, Simulation and Characterization of Ni-doped SiC Nanocoatings Prepared by Jet Electrodeposition, Ceram. Int., 2017, 44, p 5500–5505. https://doi.org/10.1016/j.ceramint.2017.12.189

    Article  CAS  Google Scholar 

  31. C.Y. Li, F.F. Xia, C.Y. Ma, and Q. Li, Research on the Corrosion Behavior of Ni-SiC Nanocoating Prepared Using a Jet Electrodeposition Technique, J. Mater. Eng. Perform., 2021, 30, p 6336–6344. https://doi.org/10.1007/s11665-021-05891-1

    Article  CAS  Google Scholar 

  32. H. Jin, R.J. Ji, T.C. Dong, S. Liu, Y.H. Liu, F. Zhang, C. Ma, and S.G. Liu, Fabrication and Characterization of WC Particles Reinforced Ni Fe Composite Coating By Jet Electrodeposition, Surf. Coat. Tech., 2021, 421, p 127368. https://doi.org/10.1016/j.surfcoat.2021.127368

    Article  CAS  Google Scholar 

  33. W. Jiang, X. Li, Y.L. Chen, H.G. Li, L.D. Li, Y. Chen, Z.J. Tian, and Y.X. Lao, Research on the Wear and Corrosion Resistance of Ni-GO-TiC Composite Coating by Scanning Jet Electrodeposition, Surf. Topogr-Metrol., 2022, 10, p 015048. https://doi.org/10.1088/2051-672X/ac5c67

    Article  Google Scholar 

  34. H. Fan, J. Jiang, Y.P. Zhao, S.K. Wang, and Z.J. Li, Improvement of Microstructure and Properties of Ni-Al2O3 Composite Coating Via Jet Electrodeposition, Int. J. Mod. Phys. B, 2020, 34, p 2050243. https://doi.org/10.1142/S0217979220502434

    Article  CAS  Google Scholar 

  35. C.A. Huang, C.H. Shen, and P.Y. Li, Effect of Fabrication Parameters on Grinding Performances of Electroplated Ni-B-Diamond Tools with D150-Diamond Particles, J. Manuf. Process., 2022, 80, p 374–381. https://doi.org/10.1016/j.jmapro.2022.05.055

    Article  Google Scholar 

  36. A.G. Tang, M.L. Wang, W. Huang, and X.L. Wang, Composition Design of Ni-Nano-Al2O3-PTFE Coatings and their Tribological Characteristics, Surf. Coat. Tech., 2015, 282, p 121–128. https://doi.org/10.1016/j.surfcoat.2015.10.034

    Article  CAS  Google Scholar 

  37. N. Guglielmi, Kinetics of the Deposition of Inert Particles from Electrolytic Baths, J. Electrocheml. Soc., 1972, 119, p 1009–1012. https://doi.org/10.1149/1.2404383

    Article  CAS  Google Scholar 

  38. M.M. Peng, L.Q. Wang, L. Guo, J.Y. Guo, L.P. Zheng, F.W. Yang, Z. Ma, and X. Zhao, A Durable Nano-SiO2-TiO2/Dodecyltrimethoxysilane Superhydrophobic Coating for Stone Protection, Coatings, 2022, 12, p 1397. https://doi.org/10.3390/coatings12101397

    Article  CAS  Google Scholar 

  39. Y.K. Xu, M.Y. Fan, Y.Q. Luo, Y.N. Chen, J.M. Hao, and X.H. Hou, Tribology and Corrosion Properties Investigation of a Pulse Electrodeposition Duplex Hard-Particle-Reinforced Ni-Mo Nanocomposite Coating, Surf. Coat. Tech., 2020, 393, p 125797. https://doi.org/10.1016/j.surfcoat.2020.125797

    Article  CAS  Google Scholar 

  40. J.I. Langford and A.J.C. Wilson, Scherrer After Sixty Years: a Survey and Some New Results in the Determination of Crystallite Size, J. Appl. Crystallogr., 2015, 11, p 102–113. https://doi.org/10.1063/1.4928401

    Article  CAS  Google Scholar 

  41. A. Brenner and S. Senderoff, Electrodeposition of Alloys, J. Electrochem. Soc., 2011, 111, p 34C. https://doi.org/10.1149/1.2426105

    Article  Google Scholar 

  42. W. Jiang, L.D. Shen, M.B. Qiu, X. Wang, M.Z. Fan, and Z.J. Tian, Preparation of Ni-SiC Composite Coatings by Magnetic Field-Enhanced Jet Electrodeposition, J. Alloy. Compd., 2018, 762, p 115–124. https://doi.org/10.1016/j.jallcom.2018.05.097

    Article  CAS  Google Scholar 

  43. L. Chen, L.P. Wang, Z.X. Zeng, and T. Xu, Influence of Pulse Frequency on the Microstructure and Wear Resistance of Electrodeposited Ni-Al2O3 Composite Coatings, Surf. Coat. Tech., 2006, 201, p 599–605. https://doi.org/10.1016/j.surfcoat.2005.12.008

    Article  CAS  Google Scholar 

  44. S. Das, S. Banthia, A. Patra, S. Sengupta, and S.B. Singh, Novel bilayer Zn-Ni/Ni-Co-SiC Nanocomposite Coating with Exceptional Corrosion and Wear Properties by Pulse Electrodeposition, J. Alloy. Compd., 2018, 738, p 394–404. https://doi.org/10.1016/j.jallcom.2017.12.093

    Article  CAS  Google Scholar 

  45. Y.F. Li, Z.J. Yang, H.J. Han, M.Y. Liu, M.M. Zhang, Z.K. Wang, and T.T. Wu, Effects of Duty Ratio on Properties of Ni-P-(sol) Al2O3 Coating Prepared by Pulse-Assisted Chemical Deposition, J. Mater. Res. Technol., 2021, 15, p 924–935. https://doi.org/10.1016/j.jmrt.2021.08.077

    Article  CAS  Google Scholar 

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Acknowledgments

The authors gratefully acknowledge the supports from the Program for Innovative Research Team (in Science and Technology) in University of Henan Province (Grant no. 20IRTSTHN016), Scientific and Technological Research Projects of Henan Province (Grant no. 222102220030).

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Zheng, L., Li, Y., Liu, M. et al. Fabrication and Characterization of Al2O3 Particles Reinforced Ni-P-Polytetrafluoroethylene Nanocomposite Coating by Jet Electrodeposition. J. of Materi Eng and Perform 32, 8503–8515 (2023). https://doi.org/10.1007/s11665-022-07739-8

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