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Thermal Lensing Effect in Laser Nanofluids Based on Poly (aniline-co-ortho phenylenediamine)@\(\text{TiO}_{2}\) Interaction

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Abstract

A poly (aniline-co-ortho phenylenediamine)@\(\text{TiO}_{2}\) (PACOPDA@\(\text{TiO}_{2}\)) nanocomposite was constructed by in situ copolymerization and its nanofluid was prepared via a two-step process. The prepared materials were characterized employing Fourier-transform infrared (FTIR) spectroscopy, energy dispersive X-ray (EDX), X-ray diffraction (XRD), field emission scanning electron microsopy (FESEM), and thermogravimetric analysis (TGA). The thermo-optical response of the PACOPDA@\(\text{TiO}_{2}\) nanofluid with different input pump power of a laser was investigated. The optical properties of the prepared materials were examined by ultraviolet-visible (UV-Vis) spectroscopy. Spatial self-phase modulation and Z-scan were utilized to study the PACOPDA@\(\text{TiO}_{2}\) nanofluid nonlinearity. An enhancement in the thermo-optical property with an increase in the input pump power and concentration of the PACOPDA@\(\text{TiO}_{2}\) was observed. The results showed that the PACOPDA@\(\text{TiO}_{2}\) nanocomposite offers new potential in nonlinear optical applications. Furthermore, a one-order increase in the nonlinear refractive index of the PACOPDA@\(\text{TiO}_{2}\) nanofluid vis-á-vis the PACOPDA was observed. The thermo-optical behavior of the PACOPDA@\(\text{TiO}_{2}\) shifts from self-defocussing to self-focusing with increasing intensity and concentration.

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  1. School of Physics, Damghan University, Damghan, Semnann, 36716-41167, Iran

    Samaneh Dadkhah & Yasser Rajabi

  2. School of Chemistry, Damghan University, Damghan, Semnann, 36716-41167, Iran

    Ehsan Nazarzadeh Zare

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  1. Samaneh Dadkhah
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Dadkhah, S., Rajabi, Y. & Zare, E.N. Thermal Lensing Effect in Laser Nanofluids Based on Poly (aniline-co-ortho phenylenediamine)@\(\text{TiO}_{2}\) Interaction. Journal of Elec Materi 50, 4896–4907 (2021). https://doi.org/10.1007/s11664-021-09028-x

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