Abstract
Photopolymerization-based additive printing of functional inorganics has drawn great attention in recent years and one important challenge is the photoresin loading with diverse inorganics. Here, we introduce a Maillard reaction-derived laser lithography strategy for an unprecedented direct printing of diverse inorganic compounds. The sugar-assisted laser lithography (SLL) is powerful to carry choice metal ions and versatile for the generation of patterned inorganic materials comprising metal oxides, metal sulfides, and metal nitrides, characterized by ferroelectric, magnetic, semiconductivity, superconductivity, or other properties. The material architecture is flexibly manipulated by the laser intensity, power, printing speed, precursor solution, and computer-aided design to satisfy the practical requirements. This work demonstrates a new possibility for the further development of laser lithography in the directly printing of feature-rich inorganic materials and devices.
Similar content being viewed by others
Change history
20 September 2022
An Erratum to this paper has been published: https://doi.org/10.1007/s11426-022-1393-1
References
Li J, Pumera M. Chem Soc Rev, 2021, 50: 2794–2838
Pan JA, Rong Z, Wang Y, Cho H, Coropceanu I, Wu H, Talapin DV. J Am Chem Soc, 2021, 143: 2372–2383
Cui H, Hensleigh R, Yao D, Maurya D, Kumar P, Kang MG, Priya S, Zheng XR. Nat Mater, 2019, 18: 234–241
Capel AJ, Rimington RP, Lewis MP, Christie SDR. Nat Rev Chem, 2018, 2: 422–436
Blasco E, Müller J, Müller P, Trouillet V, Schön M, Scherer T, Barner-Kowollik C, Wegener M. Adv Mater, 2016, 28: 3592–3595
Shukla S, Vidal X, Furlani EP, Swihart MT, Kim KT, Yoon YK, Urbas A, Prasad PN. ACS Nano, 2011, 5: 1947–1957
Vyatskikh A, Delalande S, Kudo A, Zhang X, Portela CM, Greer JR. Nat Commun, 2018, 9: 593
Vyatskikh A, Ng RC, Edwards B, Briggs RM, Greer JR. Nano Lett, 2020, 20: 3513–3520
Eckel ZC, Zhou C, Martin JH, Jacobsen AJ, Carter WB, Schaedler TA. Science, 2016, 351: 58–62
Wang X, Schmidt F, Hanaor D, Kamm PH, Li S, Gurlo A. Addit Manuf, 2019, 27: 80–90
Kotz F, Arnold K, Bauer W, Schild D, Keller N, Sachsenheimer K, Nargang TM, Richter C, Helmer D, Rapp BE. Nature, 2017, 544: 337–339
Zeng Y, Yan Y, Yan H, Liu C, Li P, Dong P, Zhao Y, Chen J. J Mater Sci, 2018, 53: 6291–6301
He R, Liu W, Wu Z, An D, Huang M, Wu H, Jiang Q, Ji X, Wu S, Xie Z. Ceram Int, 2018, 44: 3412–3416
Hildebrand G, Sänger JC, Schirmer U, Mantei W, Dupuis Y, Houbertz R, Liefeith K. Ceramics, 2021, 4: 224–239
Sun YL, Li Q, Sun SM, Huang JC, Zheng BY, Chen QD, Shao ZZ, Sun HB. Nat Commun, 2015, 6: 8612
Wang Y, Fedin I, Zhang H, Talapin DV. Science, 2017, 357: 385–388
Yee DW, Lifson ML, Edwards BW, Greer JR. Adv Mater, 2019, 31: 1901345
Chung J, Bieri NR, Ko S, Grigoropoulos CP, Poulikakos D. Appl Phys A, 2004, 79: 1259–1261
Ko SH, Pan H, Grigoropoulos CP, Luscombe CK, Fréchet JMJ, Poulikakos D. Nanotechnology, 2007, 18: 345202
Pan H, Hwang DJ, Ko SH, Clem TA, Fréchet JMJ, Bäuerle D, Grigoropoulos CP. Small, 2010, 6: 1812–1821
Hong S, Yeo J, Kim G, Kim D, Lee H, Kwon J, Lee H, Lee P, Ko SH. ACS Nano, 2013, 7: 5024–5031
Kim KK, Ha IH, Kim M, Choi J, Won P, Jo S, Ko SH. Nat Commun, 2020, 11: 2149
Jung J, Cho H, Choi SH, Kim D, Kwon J, Shin J, Hong S, Kim H, Yoon Y, Lee J, Lee D, Suh YD, Ko SH. ACS Appl Mater Interfaces, 2019, 11: 15773–15780
Kwon J, Cho H, Suh YD, Lee J, Lee H, Jung J, Kim D, Lee D, Hong S, Ko SH. Adv Mater Technol, 2016, 2: 1600222
Nam VB, Shin J, Choi A, Choi H, Ko SH, Lee D. J Mater Chem C, 2021, 9: 5652–5661
Shin J, Jeong B, Kim J, Nam VB, Yoon Y, Jung J, Hong S, Lee H, Eom H, Yeo J, Choi J, Lee D, Ko SH. Adv Mater, 2020, 32: 1905527
Nam VB, Shin J, Yoon Y, Giang TT, Kwon J, Suh YD, Yeo J, Hong S, Ko SH, Lee D. Adv Funct Mater, 2019, 29: 1806895
Stadler RH, Blank I, Varga N, Robert F, Hau J, Guy PA, Robert MC, Riediker S. Nature, 2002, 419: 449–450
Thorpe SR, Baynes JW. Amino Acids, 2003, 25: 275–281
Ajandouz EH, Tchiakpe LS, Ore FD, Benajiba A, Puigserver A. J Food Sci, 2001, 66: 926–931
Friedman M. Lysinoalanine formation in soybean proteins: kinetics and mechanisms. In: Cherry JP, Ed. Food Protein Deterioration. Vol. 206. Chapter 10. Washington: American Chemical Society, 1982. 231–273
Finot PA, Bujard E, Mottu F, Mauron J. Availability of the true Schiff’s bases of lysine. Chemical evaluation of the Schiff’s base between lysine and lactose in milk. In: Friedman M, Ed. Protein Crosslinking. Advances in Experimental Medicine and Biology. Vol 86. Boston: Springer. 1977. 343–v365
Kobayashi S, Hiroishi K, Tokunoh M, Saegusa T. Macromolecules, 1987, 20: 1496–1500
Zou GF, Zhao J, Luo HM, McCleskey TM, Burrell AK, Jia QX. Chem Soc Rev, 2013, 42: 439–449
Skliutas E, Lebedevaite M, Kabouraki E, Baldacchini T, Ostrauskaite J, Vamvakaki M, Farsari M, Juodkazis S, Malinauskas M. Nanophotonics, 2021, 10: 1211–1242
Jansen RJJ, van Bekkum H. Carbon, 1995, 33: 1021–1027
Martins SIFS, Jongen WMF, van Boekel MAJS. Trends Food Sci Tech, 2000, 11: 364–373
O’Neill W, Kun Li W. IEEE J Sel Top Quantum Electron, 2009, 15: 462–470
Hsiao WT, Tseng SF, Huang KC, Wang YH, Chen MF. Int J Adv Manuf Technol, 2011, 56: 223–231
Aydinli A, Lo HW, Lee MC, Compaan A. Phys Rev Lett, 1981, 46: 1640–1643
Arca E, Fleischer K, Shvets IV. J Phys Chem C, 2009, 113: 21074–21081
Bandara J, Divarathne CM, Nanayakkara SD. Sol Energy Mater Sol Cells, 2004, 81: 429–437
Luo H, Lin Y, Wang H, Chou CY, Suvorova NA, Hawley ME, Mueller AH, Ronning F, Bauer E, Burrell AK, McCleskey TM, Jia QX. J Phys Chem C, 2008, 112: 20535–20538
Baker MA, Greaves SJ, Wendler E, Fox V. Thin Solid Films, 2000, 377–378: 473–477
Li H, Zhang Q, Yap CCR, Tay BK, Edwin THT, Olivier A, Baillargeat D. Adv Funct Mater, 2012, 22: 1385–1390
Tan JMR, Lee YH, Pedireddy S, Baikie T, Ling XY, Wong LH. J Am Chem Soc, 2014, 136: 6684–6692
Yi Q, Wu J, Zhao J, Wang H, Hu J, Dai X, Zou G. ACS Appl Mater Interfaces, 2017, 9: 1602–1608
Kang L, Jin BB, Liu XY, Jia XQ, Chen J, Ji ZM, Xu WW, Wu PH, Mi SB, Pimenov A, Wu YJ, Wang BG. J Appl Phys, 2011, 109: 033908
Costa ACFM, Tortella E, Morelli MR, Kiminami RHGA. J Magn Magn Mater, 2003, 256: 174–182
Mao HJ, Song C, Xiao LR, Gao S, Cui B, Peng JJ, Li F, Pan F. Phys Chem Chem Phys, 2015, 17: 10146–10150
Merkininkaitė G, Aleksandravičius E, Malinauskas M, Gailevičius D, šakirzanovas S. Opto-Electron Adv, 2022, 5: 210077
Gonzalez-Hernandez D, Varapnickas S, Merkininkaitė G, Čiburys A, Gailevičius D, Šakirzanovas S, Juodkazis S, Malinauskas M. Photonics, 2021, 8: 577
Son Y, Yeo J, Moon H, Lim TW, Hong S, Nam KH, Yoo S, Grigoropoulos CP, Yang DY, Ko SH. Adv Mater, 2011, 23: 3176–3181
Hong S, Lee H, Yeo J, Ko SH. Nano Today, 2016, 11: 547–564
Huo F, Zheng Z, Zheng G, Giam LR, Zhang H, Mirkin CA. Science, 2008, 321: 1658–1660
Chen Y. Microelectron Eng, 2015, 135: 57–72
Acknowledgements
This work was supported by the National Natural Science Foundation of China (21971172, 21671141, and 21601130) and the Priority Academic Program Development (PAPD) of Jiangsu Higher Education Institutions for Optical Engineering in Soochow University.
Author information
Authors and Affiliations
Corresponding author
Additional information
Supporting information The supporting information is available online at http://chem.scichina.com and http://link.springer.com/journal/11426. The supporting materials are published as submitted, without typesetting or editing. The responsibility for scientific accuracy and content remains entirely with the authors.
Conflict of interest
The authors declare no conflict of interest.
The online version of the original article can be found at https://doi.org/10.1007/s11426-022-1393-1
Rights and permissions
About this article
Cite this article
Dai, X., Jiang, Y., Wang, X. et al. Maillard reaction-derived laser lithography for printing functional inorganics. Sci. China Chem. 65, 1306–1314 (2022). https://doi.org/10.1007/s11426-022-1230-x
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s11426-022-1230-x