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Removal of Dimethyl Arsenic Acid from Aqueous Solution by Ferric Manganese Binary Oxide

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Abstract

This study addresses the environmental concern of organic-arsenic pollution resulting from the discharge of dimethyl arsenic acid (DMA) through non-point sources into surface and groundwater, posing severe health risks. While efforts have primarily focused on eliminating inorganic arsenic, the toxicity of organic arsenic, particularly DMA, has been over-disregarded and necessitates a thorough examination. In response, this research focuses on developing effective adsorbents for the removal of organic arsenic, with a specific emphasis on DMA. Using the co-precipitation method, ferric manganese binary oxide (FMBO) was synthesized and compared with manganese dioxide (MnO2) and ferric oxide (FeOOH). The produced adsorbents were evaluated using a range of characterization methods, such as X-ray powder diffraction (XRD), specific surface area (SBET), zeta (ζ)-potential, scanning electron microscopy (SEM) with energy dispersive X-ray (EDX), and Fourier transform infrared spectroscopy (FTIR). The impact of pH, adsorption kinetics, and adsorption isotherms were investigated in batch studies to ascertain efficacy. The Elovich model, which suggests heterosphere diffusion reactions, best explained the adsorption data, according to the results followed by the pseudo-second-order model. pH had a major impact on DMA adsorption; at pH 4.0, FMBO showed a maximum adsorption capacity of 665.28 μg/g, which was higher than that of FeOOH (581.32 μg/g) and MnO2 (510.56 μg/g). Fitting descriptions of DMA adsorption onto FMBO, FeOOH, and MnO2 were provided by the Langmuir and Sips models. Systematic characterization by FTIR and SEM–EDX highlighted FMBO’s predominant role in DMA adsorption at lower pH. Regeneration experiments demonstrated a slight decrease in DMA adsorption from 99.04 to 94.90% after five consecutive cycles, affirming FMBO’s substantial capability to remove DMA from aqueous solutions. This study underscores the potential of FMBO as an efficient adsorbent for combating organic-arsenic pollution.

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Data Availability

The datasets used and/or analyzed during the current study are available from the corresponding author on reasonable request.

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Acknowledgements

This research work was carried out with the aid of a grant from UNESCO and the International Development Research Centre (IDRC), Ottawa, Canada. The views expressed herein do not necessarily represent those of UNESCO, IDRC, or its Board of Governors. We are grateful to the Key Laboratory of Drinking Water Science and Technology at the Research Center for Eco-Environmental Sciences of the Chinese Academy of Sciences, Beijing 100085, China, for helping the characterization of the adsorbents with partial financial support by the National Natural Science Foundation of China (Grant-Number: 51908541) and the Alliance of International Science Organizations (ANSO-CR-KP-2020-05). We are grateful to the Nepal Academy of Science and Technology (NAST) for providing all the laboratory facilities.

Funding

UNESCO and the International Development Research Center (IDRC), Ottawa, Canada, Grant Number: 4500406708, Author Tista Prasai Joshi has received funds.

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Authors and Affiliations

  1. Environment Research Laboratory, Faculty of Science, Nepal Academy of Science and Technology, Khumaltar, Lalitpur, Nepal

    Naina Byanjankar, Tista Prasai Joshi & Agni Dhakal

  2. Central Department of Microbiology, Tribhuvan University, Kathmandu, Nepal

    Dev Raj Joshi

  3. State Key Laboratory of Environmental Aquatic Chemistry, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, 100085, China

    Rashmi Koju, Zenglu Qi & Chengzhi Hu

  4. Center for Water and Ecology, State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing, 100084, China

    Ruiping Liu

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  1. Naina Byanjankar
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Contributions

Naina Byanjankar: methodology, conceptualization, and writing—original draft preparation; Tista Prasai Joshi: conceptualization, methodology, writing—reviewing and editing, and supervision; Agni Dhakal: methodology; Dev Raj Joshi: writing—reviewing and editing; Rashmi Koju: methodology, reviewing, and editing; Zenglu Qi: methodology and software; Chengzhi Hu: validation; Ruiping Liu: supervision. All authors read and approved the final manuscript.

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Correspondence to Tista Prasai Joshi.

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Byanjankar, N., Joshi, T.P., Dhakal, A. et al. Removal of Dimethyl Arsenic Acid from Aqueous Solution by Ferric Manganese Binary Oxide. Water Air Soil Pollut 235, 196 (2024). https://doi.org/10.1007/s11270-024-07008-5

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