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A Review on the Recent Advances in the Reductions of Carbon–Carbon/Oxygen Multiple Bonds Including Aromatic Rings Using Raney Ni–Al Alloy or Al Powder in the Presence of Noble Metal Catalysts in Water

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Abstract

Over the past few years, heterogeneous catalysts have attracted much attention with a view to lowering reaction temperatures and improving the selectivity of many organic syntheses. When it comes to designing or optimizing a catalyst, a lot of attention is needed to be devoted to the nature of the active sites and how they interact with the reactants, intermediates and products of the catalytic process. To this end, Raney Ni–Al alloy and noble metal catalysts such as Ru/C, Rh/C, Pd/C and Pt/C turn out to be very effective in both selective and complete reductions of various functional groups as well as aromatic rings in water. Moreover, Al powder coupled with a noble metal catalyst has been found to be capable of reducing carbonyl group, an alkyne moiety and also the aromatic rings of biphenyl, fluorene, 9,10-dihydroanthracene, polyarenes and N-heterocycles in water under mild reaction conditions. So this review offers an overview on the most recent developments especially in this particular methodology.

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Acknowledgements

This work was conducted under the Cooperative Research Program of “Network Joint Research Center for Materials and Devices (Institute for Materials Chemistry and Engineering, Kyushu University)”. CR thanks the EPSRC for an Overseas Travel Grant.

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Authors and Affiliations

  1. Department of Applied Chemistry, Faculty of Science and Engineering, Saga University, Honjo-machi 1, Saga, 840-8502, Japan

    Ummey Rayhan, Zannatul Kowser & Takehiko Yamato

  2. Department of Chemistry, Dhaka University of Engineering and Technology, Gazipur, 1700, Bangladesh

    Ummey Rayhan & Md. Nurul Islam

  3. Department of Chemistry, Jessore University of Science and Technology, Jessore, 7408, Bangladesh

    Zannatul Kowser

  4. Chemistry, School of Mathematics and Physical Sciences, The University of Hull, Cottingham Road, Hull, Yorkshire, HU6 7RX, UK

    Carl Redshaw

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Dedicated to Prof. George A. Olah Memorial Issue.

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Rayhan, U., Kowser, Z., Islam, M.N. et al. A Review on the Recent Advances in the Reductions of Carbon–Carbon/Oxygen Multiple Bonds Including Aromatic Rings Using Raney Ni–Al Alloy or Al Powder in the Presence of Noble Metal Catalysts in Water. Top Catal 61, 560–574 (2018). https://doi.org/10.1007/s11244-018-0994-2

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