Abstract
Internal conversion electron and gamma-ray spectroscopy measurements were carried out on the 10.551 y 133Ba electron-capture decay with our electron and gamma spectrometers—a mini-orange electron transporter paired to a Si(Li) detector and a large-volume HPGe detector, respectively. The relative and absolute gamma-ray intensities of all the nine transitions in 133Cs were determined. We also report the relative conversion intensities of eighteen conversion lines and their corresponding internal conversion coefficients (ICCs), four of which are being reported for the first time. Transition intensity balance at each energy level, showed that the measured values are self-consistent. This exhaustive dataset of gamma-ray intensities, internal conversion electron intensities and the ICCs that have low uncertainty, will be highly valuable for the purposes of energy and efficiency calibration of semiconductor gamma ray detectors and electron spectrometers.
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References
Thun JE, Tornkvist S, Nielsen KB, Snellman H, Falk F, Mocoroa A (1966) Levels and transitions in 133Cs. Nucl Phys 88:289–306. https://doi.org/10.1016/0029-5582(66)90589-X
Notea A, Gurfinkel Y (1968) Transitions in 133Cs from the decay of 133Ba. Nucl Phys A 107:193–208. https://doi.org/10.1016/0375-9474(68)90736-7
Bosch HE, Haverfield AJ, Szichman E, Abecasis SM (1968) High-resolution studies in the decay of 133Ba with semiconductor counters. Nucl Phys A 108:209–220. https://doi.org/10.1016/0375-9474(68)90154-1
Donnelly DP, Reidy JJ, Wiedenbeck ML (1968) High-resolution gamma-ray spectroscopic study of the decay 133Ba à 133Cs. Phys Rev 173:1192–1201. https://doi.org/10.1103/PhysRev.173.1192
Schötzig U, Debertin K, Walz KF (1977) Standardization and decay data of 133Ba. Intern J Appl Radiat Isot 28:503–507. https://doi.org/10.1016/0020-708x(77)90185-5
Yoshizawa Y, Iwata Y, Katoh T, Ruan JZ, Kawada Y (1983) Precision measurements of gamma-ray intensities IV. Low energy region: 75Se and 133Ba. Nucl Instrum Methods 212:249–257. https://doi.org/10.1016/0167-5087(83)90700-7
Danilenko VN, Konstantinov AA, Kurenkov NV, Kurchatova LN, Malinin AB, Mamelin AV, Matveev SV, Sazonova TE, Stepano EK, Sepman SV, Toporov YuG (1989) Methods of producing radionuclides for spectrometric gamma-ray sources and their standardization-1. Barium-133. Appl Radiat Isot 40:707–710. https://doi.org/10.1016/0883-2889(89)90082-8
Kumahora H (1985) Precision energy measurement of gamma rays from the decay of 75Se and 133Ba. Nucl Instrum Methods Phys Res A 238:431–442. https://doi.org/10.1016/0168-9002(85)90482-6
Mucciolo ER, Helene O (1987) Energy measurement of gamma rays from 133Ba decay: consistency with cascade cross-over relations. Nucl Instrum Methods Phys Res A 256:153–160. https://doi.org/10.1016/0168-9002(87)91050-3
Helmer RG, van der Leun C (2000) Recommended standards for γ-ray energy calibration (1999). Nucl Instrum Methods Phys Res A 450:35–70. https://doi.org/10.1016/S0168-9002(00)00252-7
Chauvenet B, Morel J, Legrand J (1983) An international intercomparison of photon emission-rate measurements of x- and gamma-rays emitted in the decay of 133Ba. Intern J Appl Radiat Isot 34:479–485. https://doi.org/10.1016/0020-708X(83)90265-X
Be MM, Chiste V, Dulieu C, Kellet MA, Mougeot X, Arinc A, Chechev VP, Kuzmenko NK, Kibedi T, Luca A, Nichols AL (2016) Table of radionuclides, vol 8—A = 41 to 198). https://www.bipm.org/utils/common/pdf/monographieRI/Monographie_BIPM-5_Tables_Vol8.pdf
Khazov Y, Rodionov A, Kondev FG (2011) Nuclear data sheets for A = 133. Nucl Data Sheets 112:855–1113. https://doi.org/10.1016/j.nds.2011.03.001
Hwang HY, Lee CB, Park TS (1998) Subtractions of accidental coincidences and Compton scattered events by multi-channel time scaling technique in γ-ray spectrometry. Appl Radiat Isot 49:1201–1205. https://doi.org/10.1016/S0969-8043(97)10046-X
Miyahara H, Usami K, Mori C (1996) Precise measurement of the emission probabilities for the weak 161 and 223 keV gamma-rays of 133Ba. Nucl Instrum Methods Phys Res A 374:193–196. https://doi.org/10.1016/0168-9002(95)01420-9
Avignone FT, Frey GD, Hendrick LD (1970) Internal-conversion penetration effects in M1 transitions of 133Cs. Phys Rev C 1:635–643. https://doi.org/10.1103/PhysRevC.1.635
Hennecke HJ, Manthuruthil JC, Bergman O, Cothern CR (1967) Internal-conversion-electron study of the decay of Ba133 to Cs133. Phys Rev 159:955–968. https://doi.org/10.1103/PhysRev.159.955
Sergeenkov YV (1984) In: Proceedings of 5th seminar on precise measurements in nuclear spectroscopy, Vilnius, pp 67–70
Venkataramaniah K, Sainath M, Sai K, Rao D, Seetharaman D (2020) Design and development of a mini-orange magnetic spectrometer with multichannel facility for conversion electron spectroscopy. J Nucl Phys Mater Sci Radiat Appl 8:25–31. https://doi.org/10.15415/jnp.2020.81004
Deepa S, Vijay Sai K, Gowrishankar R, Venkataramaniah K (2012) Conversion electron measurements and determination of rotational parameters in 177Lu and 177Hf. Eur Phys J A 48:126–136. https://doi.org/10.1140/epja/i2012-12126-2
GammaVision-32 (1998) Version 5.10 spectrum acquisition and analysis software. https://www.ortec-online.com/products/application-software/gammavision
Bikit I, Nemes T, Mrda D, Jovančević N (2009) On the absolute source activity measurement with a single detector: the 133Ba case. Nucl Instrum Methods Phys Res A 612:103–111. https://doi.org/10.1016/j.nima.2009.09.060
Petkov V, Bakaltchev N (1990) FIT a computer program for decomposition of powder diffraction patterns and profile analysis of pair correlation functions. J Appl Cryst 23:138–140. https://doi.org/10.1107/S002188988901410X
X- and Gamma-Ray Decay Data Standards for Detector Calibration Pub1287_Vol2_web. https://www.google.com/url?sa=t&rct=j&q=&esrc=s&source=web&cd=&ved=2ahUKEwiq2siq6pnvAhXDzDgGHYJhDsAQFjAAegQIAhAD&url=https%3A%2F%2Fwww-pub.iaea.org%2FMTCD%2FPublications%2FPDF%2FPub1287_Vol2_web.pdf&usg=AOvVaw2-N0M8FAApGyOU_D5mo7JB
Rao DR, Vijay Sai K, Sainath M, Venkataramaniah K (2005) Precision electron-gamma spectroscopic measurements in 75As. Eur Phys J A 26:41–50. https://doi.org/10.1140/epja/i2005-10152-9
Patil A, Santhosh D, Vijay Sai K, Sainath M, Venkataramaniah K (2006) Precision measurements in 124Te following the decay of 124Sb. Appl Radiat Isot 64:693–699. https://doi.org/10.1016/j.apradiso.2005.12.010
Chechev VP, Kuzmenko NK (2015) 133Ba - Comments on evaluation of decay data. - Comments on evaluation of decay data. https://www.google.com/url?sa=t&rct=j&q=&esrc=s&source=web&cd=&cad=rja&uact=8&ved=2ahUKEwirgcOJg5XwAhU-zTgGHV8fCoMQFjAAegQIAxAD&url=http%3A%2F%2Fwww.nucleide.org%2FDDEP_WG%2FNuclides%2FBa-133_com.pdf&usg=AOvVaw1KlMTMNWxj3cKOkZ1vrp0W. Accessed 4 Mar 2021
BRICC Online Conversion Coefficient Calculator—Version 2.3S (2018) http://bricc.anu.edu.au/
GTOL Program Package—Version 7.2f (2010) https://www-nds.iaea.org/public/ensdf_pgm/
ENSDAT—Evaluated Nuclear Structure Drawings and Tables. Version 12.13. https://www-nds.iaea.org/workshops/smr1939/Codes/ENSDF_Codes/mswindows/ensdat/ensdat_win.html
Logft Program Package. https://www.nndc.bnl.gov/logft/
GABS Program Package Version 12 (2020) https://www-nds.iaea.org/public/ensdf_pgm/
Törnkvist S, Hasselgren L, Ström S, Thun JE, Antman S (1970) Internal conversion studies of transitions populating and depopulating the 161 keV level in 133Cs. Nucl Phys A 142:238–250. https://doi.org/10.1016/0375-9474(70)90526-9
Ramaniah KV, Reddy KV (1975) Nuclear-structure effect in the K-conversion process of the 223 keV transition in 133Cs. Il Nuovo Cimento A 26:237–242. https://doi.org/10.1007/bf02769010
Church EL, Weneser J (1960) Nuclear structure effects in internal conversion. Annu Rev Nucl Part Sci 10:193–234. https://doi.org/10.1146/annurev.ns.10.120160.001205
Hager RS, Seltzer EC (1969) Internal conversion tables part III: coefficients for the analysis of penetration effects in internal conversion and E0 internal conversion. Nucl Data Sheets Sect A 6:1–127. https://doi.org/10.1016/S0550-306X(69)80002-9
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The authors express their gratitude to the Sri Sathya Sai Institute of Higher Learning, for providing all the laboratory and instrument facilities for undertaking this research work.
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Deepa, S., Vijay Sai, K., Rao, D. et al. EC-decay of 133Ba revisited by electron-gamma spectroscopy. J Radioanal Nucl Chem 328, 1001–1010 (2021). https://doi.org/10.1007/s10967-021-07731-x
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DOI: https://doi.org/10.1007/s10967-021-07731-x