Abstract
A hydrochemical study was undertaken in uranium impacted districts of southwest Punjab for evaluating the spatial and vertical trends as well as correlations with other hydrochemical parameters. Results infer that U is present in all samples (12.2–621 µg l−1) and 90% are contaminated. Contour diagram depicts contamination in entire region excepting some pockets in central part of the study area. Shallow zones (<50 m bgl) show higher U compared to deeper ones. Hydrochemistry infers a common source of U for both shallow and deep zones and alkalinity as the governing factor for U mobilization from the sediments.
Similar content being viewed by others
References
Gascoyne M (1992) Palaeoclimate determination from cave calcite deposits. Quat Sci Rev 11:609–632
Osmond JK, Ivanovich M (1992) Uranium-series mobilisation and surface hydrology. In: Ma H, Ivanovich RS (eds) Uranium series disequilibrium: applications to environmental problems. Clarendon Press, Oxford, pp 259–289
Nolan J, Weber KA (2015) Natural Uranium Contamination in major US aquifers linked to nitrate. Environ Sci Technol Lett 2(8):215–220
Selden AI, Lundholm C, Edlund B, Hogdahl C, Ek BM, Bergstrom BE et al (2009) Nephrotoxicity of uranium in drinking water from private drilled wells. Environ Res 109(4):486–494
Zamora ML, Zielinski JM, Moodie GB, Falcomer RAF, Hunt WC, Capello K (2009) Uranium in drinking water: renal effects of long-term ingestion by an aboriginal community. Arch Environ Occup Health 64(4):228–241
Kurttio P, Auvinen A, Salonen L, Saha H, Pekkanen J, Makelainen I, Vaisanen SB, Penttila IM, Komulainen H (2002) Renal effects of Uranium in drinking water. Environ Health Perspect 110(4):337–342
Lee MH, Choi GS, Cho YH, Lee CW, Shin HS (2001) Concentrations and activity ratios of uranium isotopes in the groundwater of the Okchun Belt in Korea. J Environ Radioact 57:105–116
Keesari T, Chawla D, Sinha UK, Kumar A, Rishi M (2015) In: Ramakumar KL, Kannan S, Kannan S, Mukerjee SK (eds) Occurrence of uranium in parts of southwest Punjab its interrelation with physicochemical parameters. Board of Research in Nuclear Sciences, Mumbai, India
Keesari T, Mohokar HV, Sahoo BK, Mallesh G (2014) Assessment of environmental radioactive elements in groundwater in parts of Nalgonda district, Andhra Pradesh, South India using scintillation detection methods. J Radioanal Nucl Chem 302:1391–1398
Thivya C, Chidambaram S, Keesari T, Prasanna MV, Thilagavathi R, Nepolian M (2014) Occurrence of the radionuclides in groundwater of crystalline hard rock regions of central Tamil Nadu, India. J Radioanal Nucl Chem 302:1349–1355
Babu MNS, Somashekar RK, Kumar SA, Shivanna K, Krishnamurthy V, Eappen KP (2008) Concentration of uranium levels in groundwater. Int J Environ Sci Technol 5(2):263–266
Brindha K (2013) Elango L (2012) Occurrence of uranium in groundwater of a shallow granitic aquifer and its suitability for domestic use in southern India. Radioanal Nucl Chem 295:357–367. doi:10.1007/s10967-012-2090-6;357-367
WHO (2012) Uranium in drinking-water. Background document for preparation of WHO Guidelines for drinking-water quality. Geneva, World Health Organization (WHO/SDE/WSH/03.04/118/Rev/1)
ATSDR (2011) Toxicological profile for uranium. U.S. Department of Health and Human Services. Public Health Service. Agency for Toxic Substances and Disease Registry. Atlanta, GA
Tanner AB (1980) Radon migration in the ground: a supplementary review. In: Gesell TF, Lowder WM (eds) The natural radiation environment III, vol 1. National Technical Information Services, Springfield, Alexandria, 5–56 CONF-780422
Jacques D, Mallants D, Simunek J, van Genuchten MT (2008) Modelling the fate of uranium from inorganic phosphorus fertilizer applications in agriculture. Loads and fate of fertilizer derived Uranium. Backhuys Publishers, Leiden, pp 57–65
Finkelstein MM, Kreiger N (1996) Radium in drinking water and risk of bone cancer in Ontario youths: a second study and combined analysis. Occup Environ Med 53(5):305–311
Sharma DA, Rishi MS, Keesari T (2016) Distribution of uranium in groundwater and its correlation with physicochemical parameters—a case study from Bathinda District of Punjab. In: Venkateswara Rao B (ed) Proceedings of the first indian national groundwater conference (ingwc-2016) on sustainable development and management of groundwater resources in arid and semi-arid regions, JNTU Hyderabad, 5th Oct–7th Oct, 2016. BS Publications, ISBN: 978-93-5230-149-2, pp 216–225
Kumar A, Usha N, Sawant PD, Tripathi RM, Raj SS, Mishra M, Rout S, Supreeta P, Singh J, Kumar S, Kushwaha HS (2011) Risk assessment for natural uranium in subsurface water of Punjab state, India. Hum Ecol Risk Assess 17:381–393
Kochhar N, Dadwal V, Rishi M, Sharma NK, Balaram V (2012) Evaluation of chemical quality of groundwater in parts of Sirsa (Harayana), Mansa, Bhatinda and Muktsar Districts, SW Punjab with emphasis on Uranium in relation to human health. In: Proceedings of 5th international groundwater conference (IGWC-2012) on the assessment and management of groundwater resources in hard rock systems with special reference to basaltic terrain, Maharashtra, India, pp 611—626
Singh L, Kumar R, Kumar S, Bajwa BS, Singh S (2012) Health risk assessments due to uranium contamination of drinking water in Bathinda region, Punjab state, India. Radioprotection doi: 10.1051/radiopro/2012042
Thivya C, Chidambaram S, Keesari T, Prasanna MV, Thilagavathi R, Adithya VS, Singaraja C (2016) Lithological and hydrochemical controls on distribution and speciation of uranium in groundwaters of hard-rock granitic aquifers of Madurai District, Tamil Nadu (India). Environ Geochem Health 38(2):497–509
Rani A, Singh S, Duggal V, Balaram v (2013) Uranium estimation in drinking water samples from some areas of Punjab and Himachal Pradesh, India using ICP-MS. Radiat Prot Dosimetry 157:146–151
Blaurock-Busch E, Busch YM, Friedle A, Buerner H, Prakash C, Kaur A (2014) Comparing the metal concentration in the hair of cancer patients and healthy people living in the malwa region of Punajb, India. Clin Med Insights Oncol 8:1–13. doi:10.4137/CMO.S13410
Singh J, Singh L, Singh G (1995) High U-contents observed in some drinking waters of Punjab, India. J Environ Radioact 26:217–222
Sharma N, Singh J (2016) Radiological and chemical risk assessment due to high uranium contents observed in the ground waters of Mansa District (Malwa region) of Punjab State, India: An Area of High Cancer Incidence. Expo Health. doi:10.1007/s12403-016-0215-9
Sahoo SK, Mohapatra S, Chakrabarty A, Sumesh CG, Jha VN, Tripathi RM, Puranik VD (2009) Distribution of uranium in drinking water and associated age-dependent radiation dose in India. Radiat Prot Dosim 136(2):108–113
CGWB (2014) Water Quality Issues and Challenges in Punjab. A report 160 http://cgwb.gov.in/NEW/WQ/Punjab%20Book%20Final%20for%20Printing.pdf
Singh H, Singh J, Singh S, Bajwa BS (2009) Uranium concentration in drinking water samples using the SSNTDs. Indian J Phys 83(7):1039–1044
LeMone DV, Goodell PC, Harris AH, Winston JW (2009) Phosphate Rocks: Sustainable Secondary Source for Uranium and their Agricultural Impact—9481. WM2009 Conference March 1–5, 2009 Phoenix AZ
Wang LK, Chen JP, Hung YT, Shammas NK (eds) (2009) Heavy metals in the environment. CRC Press, Boca Raton, p 23
AERB, DAE (2004) Drinking water specifications in India. Atomic Energy Regulatory Board, Mumbai
Jurgens BC, Fram MS, Belitz K, Burow KR, Landon MK (2010) Effects of groundwater development on Uranium: Central Valley, California, USA. Gwat 48(6):913–928
Drever JI (1988) The geochemistry of natural waters, 2nd edn. Prentice-Hall, New York
Sharma DA, Rishi MS, Keesari T (2016) Evaluation of groundwater quality and suitability for irrigation and drinking purposes in southwest Punjab, India using hydrochemical approach. Appl Water Sci. doi:10.1007/s13201-016-0456-6
Langmuir D (1997) Aqueous environmental geochemistry, 7th edn. Prentice Hall, New York
Hess CT, Michel J, Horton TR, Prichard HM, Conigilio WA (1985) The occurrence of radioactivity in public water supplies in the United States. Health Phys 48:553–586
Sonali PDB, Ajay K, Priyanka JR, Rupali K, Rajesh VK, Rajvir S, Pradeepkumari KS (2016) Comparison of radiometric and non-radiometric methods for uranium determination in groundwater of Punjab, India. J Radioanal Nucl Chem 307:395–405. doi:10.1007/s10967-015-4132-3
Langmuir D (1978) Uranium solution- mineral equilibria at low temperatures with applications to sedimentary ore deposits. Geochim Cosmochim Acta 42:547–569
Murphy W M, Shock EL (1999) Environmental aqueous geochemistry of actinides. In Burns PC, Finch R (ed) Uranium: Mineralogy, geochemistry and the environment. Reviews in Mineralogy, vol 38, pp. 221–254
Acknowledgements
The authors would like to acknowledge the Board of Research in Nuclear Sciences, Department of Atomic Energy, Government of India for providing the necessary financial support to carry out this work (Letter No. 35/14/11/2014-BRNS-193). Authors sincerely acknowledge the constant support and encouragement by Shri K.S.S. Sarma, Head, Isotope and Radiation Application Division, Bhabha Atomic Research Centre, Mumbai. Special thanks to scholars from Dept. of Environment Studies, Panjab University for the help and co-operation rendered during the sample collection and analysis. We thank anonymous reviewers for helping to improve the manuscript.
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Rishi, M.S., Keesari, T., Sharma, D.A. et al. Spatial trends in uranium distribution in groundwaters of Southwest Punjab, India - A hydrochemical perspective. J Radioanal Nucl Chem 311, 1937–1945 (2017). https://doi.org/10.1007/s10967-017-5178-1
Received:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s10967-017-5178-1