Skip to main content
Log in

Magnetostriction and Magnetic Anisotropy of (Pr0.5Nd0.5)1−xCexFe1.93 Alloys

  • Original Paper
  • Published:
Journal of Superconductivity and Novel Magnetism Aims and scope Submit manuscript

Abstract

Polycrystalline alloys of (Pr0.5Nd0.5)1−xCexFe1.93 (0 ≤ x ≤ 1.0) are arc melted and investigated for structural, magnetic, and magnetoelastic properties. The light rare earth Ce presents a mixed-valence behavior and helps form a single C15 Laves phase for the composition of x ≥ 0.40. Both the lattice parameter a and the saturation magnetization MS of the Laves phase decrease with increasing Ce content, and the dependence of a on the Ce concentration deviates the linear Vegard law. The easy direction of magnetization (EMD) at room temperature is detected toward <111> axis by performing X-ray diffraction on magnetic-field–aligned powders. The Ce introduction into (Pr,Nd)Fe2 system can reduce the magnetocrystalline anisotropy, resulting in an enhancement of the magnetostriction at low magnetic fields. The good magnetoelastic properties, that is, a low anisotropy and a high low-field anisotropic magnetostriction λa ~ 165 ppm at 1 kOe, can be obtained for the free-heavy rare earth (Pr0.5Nd0.5)0.6Ce0.4Fe1.93 alloy, and may make it a promising candidate for applications.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5

Similar content being viewed by others

References

  1. Clark, A.E.: In: Wohlfarth, E.P. (ed.) Ferromagnetic Materials, vol. 1, p. 531. North-Holland, Amsterdam (1980)

    Google Scholar 

  2. Engdahl, G.: Handbook of Giant Magnetostrictive Materials. Academic Press, San Diego (2000)

    Google Scholar 

  3. Zhang, Z., Lu, W.J., Dong, S.Z., Bai, H.R., Yang, T.N., We, D.H., et al.: Design of high resistivity light-rare-earth-based PrFe1.93 magnetostrictive alloys: Si doping and high-pressure annealing. J. Magn. Magn. Mater. 471, 64–69 (2019)

    Article  ADS  Google Scholar 

  4. Tang, Y.M., He, Y., Huang, Y., Zhang, L., Tang, S.L., Du, Y.W.: Spin reorientation and giant low-temperature magnetostriction of polycrystalline NdFe1.9 compound. J. Magn. Magn. Mater. 451, 515–519 (2018)

    Article  ADS  Google Scholar 

  5. Murtaza, A., Yang, S., Chang, T.Y., Ghani, A., Tahir Khan, M., Zhang, R., Zhou, C., Song, X.P., Suchomel, M., Ren, Y.: Spin reorientation and magnetoelastic properties of ferromagnetic Tb1-xNdxCo2 systems with amorphotropic phase boundary. Phys. Rev. B. 97, 104410 (2018)

    Article  ADS  Google Scholar 

  6. Rajasekhar, P., Markandeyulu, G.: Magnetostriction and spin reorientation studies on Sm0.9-xNdxPr0.1Fe1.93 (x = 0, 0.12, 0.2, 0.24, 0.32, 0.36) compounds. J. Magn. Magn. Mater. 448, 82–87 (2018)

    Article  ADS  Google Scholar 

  7. Li, F., Liu, J.J., Zhu, X.Y., Shen, W.C., Lin, L.L., Du, J., Si, P.Z., et al.: Solid State Commun. 275, 63–67 (2018)

    Article  ADS  Google Scholar 

  8. Shi, Y.G., Zhai, L., Tang, S.L., Chen, R.J.: Magnetostriction in high-pressure synthesized PrxNd1-xFe1.9 (0 ≤ x ≤ 1) alloys. J. Appl. Phys. 109, 07A915 (2011)

    Article  Google Scholar 

  9. Tang, C.C., Li, Y.X., Du, J., Wu, G.H., Zhan, W.S.: Growth of iron-based Laves phase containing Pr and Nd magnetostrictive materials. J. Cryst. Growth. 186, 471–474 (1998)

    Article  ADS  Google Scholar 

  10. Franse, J.J.M., Radwanski, R.J.: In: Buschow, K.H.J. (ed.) Handbook of Magnetic Materials, vol. 7, p. 307. North-Holland, Amsterdam (1993)

    Google Scholar 

  11. Jammalamadaka, S.N., Markandeyulu, G., Balasubramaniam, K.: Magnetostriction and anisotropy compensation in TbxDy0.9-xNd0.1Fe1.93 (0 ≤ x ≤ 1). Appl. Phys. Lett. 97, 242502 (2010)

    Article  ADS  Google Scholar 

  12. Buschow, K.H.J.: Intermetallic compounds of rare-earth and 3d transition metals. Rep. Prog. Phys. 40, 1179 (1977)

    Article  ADS  Google Scholar 

  13. Tang, C.C., Zhan, W.S., Li, Y.X., Chen, D.F., Du, J., Wu, G.H., Li, J.Y., Jia, K.C.: Synthesis and magnetic properties of PrxCe1-xFe2 compounds. J. Phys.: Condens. Matter. 9, 9651–9659 (1997)

    ADS  Google Scholar 

  14. Ren, W.J., Yang, J.L., Li, B., Li, D., Zhao, X.G., Zhang, Z.D.: Magnetostriction and magnetic anisotropy of (Sm,Ce)Fe2 compounds. Physica B. 404, 3410–3412 (2009)

    Article  ADS  Google Scholar 

  15. Chikazumi, S.: Physics of Ferromagnetism, 2nd edn, p. 503. Oxford University Press, New York (1997)

    Google Scholar 

  16. Pan, Z.B., Liu, J.J., Liu, X.Y., Li, X., Song, X.H., Zhang, Z.R., Ren, W.J.: Structural, magnetic and magnetoelastic properties of Laves-phase Tb0.3Dy0.6Nd0.1 -(Fe1-xCox)1.93 compounds. Intermetallics. 64, 1–5 (2015)

    Article  Google Scholar 

  17. Westwood, P., Abell, J.S., Pitman, K.C.: Phase relationships in the Tb-Dy-Fe ternary system. J. Appl. Phys. 67, 4998–5000 (1990)

    Article  ADS  Google Scholar 

  18. Koon, N.C., Schindler, A.I., Williams, C.M., Carter, F.L.: Magnetostrictive properties of HoxTb1-xFe2 intermetallic compounds. J. Appl. Phys. 45, 5389 (1974)

    Article  ADS  Google Scholar 

  19. Shi, Y.G., Tang, S.L., Huang, Y.J., Lv, L.Y., Du, Y.W.: Anisotropy compensation and magnetostriction in TbxNd1-xFe1.9 cubic Laves alloys. Appl. Phys. Lett. 90, 142515 (2007)

    Article  ADS  Google Scholar 

Download references

Acknowledgments

This work was supported by the National Natural Science Foundation of China (No. 50801039), Zhejiang Province (LY18E010001), Ningbo City (2019A610167), and K.C. Wong Magna Fund in Ningbo University.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Z.B. Pan.

Additional information

Publisher’s note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Ding, Q., Liu, J., Wang, M. et al. Magnetostriction and Magnetic Anisotropy of (Pr0.5Nd0.5)1−xCexFe1.93 Alloys. J Supercond Nov Magn 33, 2031–2036 (2020). https://doi.org/10.1007/s10948-020-05443-z

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10948-020-05443-z

Keywords

Navigation