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Impact of Ferromagnetic Ni Substitution on Structural and Magnetic Parameters of Ba0.8In0.2Fe12−xNixO19 (x = 0.00–2.00) Hexaferrites

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Abstract

In this work, Ba0.8In0.2Fe12−xNixO19 (x = 0.00–2.00) hexaferrites were prepared by the ceramic route, and the effect of ferromagnetic dopant Ni was retrieved on the structure and magnetic properties. Microstructural properties were explored using XRD and SEM. The range of the grain size was between 500 to 2000 nm. In addition to these, micro strain, dislocation density, and porosity were determined. According to the VSM findings, ferromagnetic nickel doping increased the magnetic saturation up to 58.36 emu/g. The coercivity values were observed within a defined range from 5.129 kOe to 5.512 kOe, showing only a slight change. Moreover, the magnetocrystalline anisotropy constant, anisotropy field, and anisotropy parameter were calculated. The results showed that the magnetocrystalline anisotropy constant and anisotropy field both increased up to 0.06308 emu/g.kOe and 1.722 kOe for an increase in doping concentrations and then dropped for x = 2.0. The magnetic moment per formula unit in terms of Bohr magneton was also computed and has an upper limit of 11.603. These results suggest that the synthesized material is a good contender for magnetic applications.

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Acknowledgements

The authors are thankful to the Deanship of Scientific Research at King Khalid University for funding this work through a large group Research Project under grant number RGP2/236/44.

Funding

This work was supported by Deanship of Scientific Research, King Khalid University (Grant No. RGP2/236/44)

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Author notes

  1. Sana Ullah Asif, Ubaid-ur-Rehman Ghori, Qasim Ali Ranjha, Fahim Ahmed, Gideon F. B. Solre, Ishfaq Ahmad, Fatma A. Ibrahim, Mohamed S. Hamdy, Ebraheem Abdu Musad Saleh, and Sayed M. Eldin have contributed equally to this work.

Authors and Affiliations

  1. Key Laboratory of LCR Materials and Devices of Yunnan Province, National Center for International Research On Photoelectric and Energy Materials, School of Materials and Energy, Yunnan University, Kunming, 650091, People’s Republic of China

    Sana Ullah Asif

  2. Department of Industrial & Manufacturing Engineering (RCET), University of Engineering & Technology, Lahore, Pakistan

    Ubaid-ur-Rehman Ghori

  3. Department of Mechanical Engineering, RCET Campus, University of Engineering and Technology, Lahore, Pakistan

    Qasim Ali Ranjha

  4. Department of Physics, Division of Science and Technology, University of Education, Lahore, Pakistan

    Fahim Ahmed & Ishfaq Ahmad

  5. School of Pharmaceutical Science and Technology, Tianjin University, Tianjin, 300072, People’s Republic of China

    Gideon F. B. Solre

  6. Catalysis Research Group (CRG), Department of Chemistry, College of Science, King Khalid University, P.O. Box 9004, Abha, 61413, Saudi Arabia

    Fatma A. Ibrahim & Mohamed S. Hamdy

  7. Department of Chemistry, College of Arts and Sciences, Prince Sattam Bin Abdulaziz University, Wadi Al-Dawasir, 11991, Saudi Arabia

    Ebraheem Abdu Musad Saleh

  8. Center of Research, Faculty of Engineering, Future University in Egypt, New Cairo, 11835, Egypt

    Sayed M. Eldin

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Contributions

All the authors contributed equally to this work. SUA, and FA, conceived the idea. IA and synthesized material, SUA, FA, FI, GFBS, EAMS, and MSH analyzed the data. QA, SME, and UG, formatted the initial draft. The work is a part of IA thesis. The manuscript was written through the contributions of all authors. All authors have approved the final version of the manuscript.

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Correspondence to Sana Ullah Asif or Fahim Ahmed.

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Asif, S.U., Ghori, UuR., Ranjha, Q.A. et al. Impact of Ferromagnetic Ni Substitution on Structural and Magnetic Parameters of Ba0.8In0.2Fe12−xNixO19 (x = 0.00–2.00) Hexaferrites. J Inorg Organomet Polym 33, 2721–2731 (2023). https://doi.org/10.1007/s10904-023-02713-w

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  • DOI: https://doi.org/10.1007/s10904-023-02713-w

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