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Fabrication of 0.94NBT–0.06BT textured ceramics using plate-like NBT templates and their electrical properties

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Abstract

The effect of crystallographic texture on the properties of 0.94(Na0.5Bi0.5TiO3)–0.06BaTiO3 (0.94NBT–0.06BT) ceramics were investigated in this study. The optimized rectangular plate-like Na0.5Bi0.5TiO3 (NBT) templates synthesized by a three-step molten salt method were used for the texturing. Dimensions of the major surfaces of the templates which were parallel to the (001) planes were measured as 8.4 µm × 10 µm (length × width) and 1 µm thickness on the average. The green textured ceramics were fabricated by tape casting method and then sintered. All ceramics were crystallized in pure perovskite structure and the degree of grain orientation was calculated as f = 91%. Brick wall-like microstructure for the textured NBT–BT ceramics with average grain size of ~ 12 µm was obtained by scanning electron microscopy. Depolarization temperature (Td) and temperature of maximum (Tm) of the dielectric permittivity were determined as 119 °C and 341 °C at 10 kHz for the textured ceramic, respectively. The value of maximum dielectric permittivity of textured ceramics was measured as εrmax ~ 5409 at 10 kHz. The high field (@50 kV/cm) piezoelectric \(d_{33}^{\ast}\) value was increased from 239 to 412 pm/V by texturing of the 0.94NBT–0.06BT ceramics. NBT template addition and texture development led to a decrease in AC conductivity.

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Acknowledgements

The authors would like to thank Dr. Aligül Büyükaksoy for assisting in the impedance spectroscopy measurements.

Funding

This research did not receive any specific grant from funding agencies in the public, commercial, or not-for-profit sectors.

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Authors and Affiliations

  1. Department of Materials Science and Engineering, Gebze Technical University, 41400, Gebze, Kocaeli, Turkey

    Ayse Berksoy-Yavuz, Tubanur Avcı, Gizem Cakırbas & Ebru Menşur

  2. Department of Metallurgical and Materials Engineering, Istanbul Gedik University, 34953, Istanbul, Turkey

    Ayse Berksoy-Yavuz

  3. Department of Metallurgical and Materials Engineering, Bursa Technical University, 16330, Bursa, Turkey

    Mustafa Yunus Kaya

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  1. Ayse Berksoy-Yavuz
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  2. Mustafa Yunus Kaya
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  3. Tubanur Avcı
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  5. Ebru Menşur
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Contributions

AB-Y: Conceptualization, project administration, formal analysis, methodology, investigation, visualization, writing-original draft. MYK: formal analysis, visualization, writing-original draft, writing-review and editing. TA: investigation. GC: investigation. EM: resources, supervision, conceptualization, project administration, writing-review and editing.

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Correspondence to Ayse Berksoy-Yavuz.

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Berksoy-Yavuz, A., Kaya, M.Y., Avcı, T. et al. Fabrication of 0.94NBT–0.06BT textured ceramics using plate-like NBT templates and their electrical properties. J Mater Sci: Mater Electron 33, 2336–2349 (2022). https://doi.org/10.1007/s10854-021-07433-w

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