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A wearable and sensitive carbon black-porous polydimethylsiloxane based pressure sensor for human physiological signals monitoring

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Abstract

Development of flexible, low cost, highly sensitive, and large-area compliance pressure sensors that can detect human physiological signals have become one of the vital component units for wearable electronics. Herein, a highly flexible and stretchable carbon black-porous polydimethylsiloxane-based pressure sensor has been successfully fabricated using a simple and effective fabrication technique with a sacrificial power template method. The pore size on the performance of pressure sensor is systematically investigated using KCl, NaCl, and sugar as powder templates to produce the porous PDMS. Notably, the KCl-templated PDMS pressure sensor exhibits a maximum pressure sensitivity (1.07 kPa−1 in 0–2 kPa), which is significantly higher than that of the NaCl-templated PDMS pressure sensor (0.86 kPa−1 in 0–2.5 kPa) and the sugar-templated PDMS pressure sensor (0.40 kPa−1 in 0–2.8 kPa). The KCl-templated PDMS pressure sensor has other advantages as well, including a fast response time of − 16 ms, a wide sensing range of 0–11,700 Pa, a low detection limit of − 2 mN, and a good reproducibility for over 3000 cycles. With these advantages, it is demonstrated that the pressure sensor can monitor minute mechanical events and human physiological signals, such as weak airflow blown, swallowing motion, finger touch, and pronunciation. Therefore, this new pressure sensor, which exhibit excellent comprehensive performance, will have wide application prospects in health monitoring and wearable devices.

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References

  1. C.M. Boutry, L. Beker, Y. Kaizawa, C. Vassos, H. Tran, A.C. Hinckley, R. Pfattner, S. Niu, J. Li, J. Claverie, Z. Wang, J. Chang, P.M. Fox, Z. Bao, Nat. Biomed. Eng. 3, 47 (2019)

    Article  CAS  Google Scholar 

  2. S. Lee, D. Sasaki, D. Kim, M. Mori, T. Yokota, H. Lee, S. Park, K. Fukuda, M. Sekino, K. Matsuura, T. Shimizu, T. Someya, Nat. Nanotechnol. 14, 156 (2019)

    Article  CAS  Google Scholar 

  3. K. Takei, T. Takahashi, J.C. Ho, H. Ko, A.G. Gillies, P.W. Leu, R.S. Fearing, A. Javey, Nat. Mater. 9, 821 (2010)

    Article  CAS  Google Scholar 

  4. Y.J. Hong, H. Jeong, K.W. Cho, N. Lu, D.H. Kim, Adv. Funct. Mater. 29, 1808247 (2019)

    Article  CAS  Google Scholar 

  5. C. Yang, L. Li, J. Zhao, J. Wang, J. Xie, Y. Cao, M. Xue, C. Lu, A.C.S. Appl, Mater. Interfaces 10, 25811 (2018)

    Article  CAS  Google Scholar 

  6. S.M. Doshi, E.T. Thostenson, ACS Sens. 3, 1276 (2018)

    Article  CAS  Google Scholar 

  7. Y. Li, Y.A. Samad, T. Taha, G. Cai, S.-Y. Fu, K. Liao, ACS Sustain. Chem. Eng. 4, 4288 (2016)

    Article  CAS  Google Scholar 

  8. C. Yan, J. Wang, W. Kang, M. Cui, X. Wang, C.Y. Foo, K.J. Chee, P.S. Lee, Adv. Mater. 26, 2022 (2014)

    Article  CAS  Google Scholar 

  9. L.Q. Tao, K.N. Zhang, H. Tian, Y. Liu, D.Y. Wang, Y.Q. Chen, Y. Yang, T.L. Ren, ACS Nano 11, 8790 (2017)

    Article  CAS  Google Scholar 

  10. M. Han, H. Wang, Y. Yang, C. Liang, W. Bai, Z. Yan, H. Li, Y. Xue, X. Wang, B. Akar, H. Zhao, H. Luan, J. Lim, I. Kandela, G.A. Ameer, Y. Zhang, Y. Huang, J.A. Rogers, Nat. Electron. 2, 26 (2019)

    Article  Google Scholar 

  11. R. Nur, N. Matsuhisa, Z. Jiang, M.O.G. Nayeem, T. Yokota, T. Someya, Nano Lett. 18, 5610 (2018)

    Article  CAS  Google Scholar 

  12. Y. Wan, Z. Qiu, J. Huang, J. Yang, Q. Wang, P. Lu, J. Yang, J. Zhang, S. Huang, Z. Wu, C.F. Guo, Small 14, 1801657 (2018)

    Article  CAS  Google Scholar 

  13. Z. Han, Z. Cheng, Y. Chen, B. Li, Z. Liang, H. Li, Y. Ma, X. Feng, Nanoscale 11, 5942 (2019)

    Article  CAS  Google Scholar 

  14. A. Tewari, S. Gandla, S. Bohm, C.R. McNeill, D. Gupta, A.C.S. Appl, Mater. Interfaces 10, 5185 (2018)

    Article  CAS  Google Scholar 

  15. S. Wagner, C. Yim, N. McEvoy, S. Kataria, V. Yokaribas, A. Kuc, S. Pindl, C.-P. Fritzen, T. Heine, G.S. Duesberg, M.C. Lemme, Nano Lett. 18, 3738 (2018)

    Article  CAS  Google Scholar 

  16. E.J. Curry, K. Ke, M.T. Chorsi, K.S. Wrobel, A.N. Miller, A. Patel, I. Kim, J. Feng, L. Yue, Q. Wu, C.-L. Kuo, K.W.-H. Lo, C.T. Laurencin, H. Ilies, P.K. Purohit, T.D. Nguyen, Proc. Natl. Acad. Sci. USA 115, 909 (2018)

    Article  CAS  Google Scholar 

  17. J. Zou, M. Zhang, J. Huang, J. Bian, Y. Jie, M. Willander, X. Cao, N. Wang, Z.L. Wang, Adv. Energy Mater. 8, 1702671 (2018)

    Article  CAS  Google Scholar 

  18. Y.-C. Lai, J. Deng, R. Liu, Y.-C. Hsiao, S.L. Zhang, W. Peng, H.-M. Wu, X. Wang, Z.L. Wang, Adv. Mater. 30, 1801114 (2018)

    Article  CAS  Google Scholar 

  19. M. Jian, K. Xia, Q. Wang, Z. Yin, H. Wang, C. Wang, H. Xie, M. Zhang, Y. Zhang, Adv. Funct. Mater. 27, 1606066 (2017)

    Article  CAS  Google Scholar 

  20. B. Zhu, Z. Niu, H. Wang, W.R. Leow, H. Wang, Y. Li, L. Zheng, J. Wei, F. Huo, X. Chen, Small 10, 3625 (2014)

    Article  CAS  Google Scholar 

  21. Y. Ma, L. Zhi, Small Methods 3, 1800199 (2019)

    Article  CAS  Google Scholar 

  22. C. Stampfer, T. Helbling, D. Obergfell, B. Schoberle, M.K. Tripp, A. Jungen, S. Roth, V.M. Bright, C. Hierold, Nano Lett. 6, 233 (2006)

    Article  CAS  Google Scholar 

  23. H.-J. Kim, A. Thukral, C. Yu, A.C.S. Appl, Mater. Interfaces 10, 5000 (2018)

    Article  CAS  Google Scholar 

  24. S. Gong, W. Schwalb, Y. Wang, Y. Chen, Y. Tang, J. Si, B. Shirinzadeh, W. Cheng, Nat. Commun. 5, 3132 (2014)

    Article  CAS  Google Scholar 

  25. J.H. Kong, N.S. Jang, S.H. Kim, J.M. Kim, Carbon 77, 199 (2014)

    Article  CAS  Google Scholar 

  26. T. Yamada, Y. Hayamizu, Y. Yamamoto, Y. Yomogida, A. Izadi-Najafabadi, D.N. Futaba, K. Hata, Nat. Nanotechnol. 6, 296 (2011)

    Article  CAS  Google Scholar 

  27. J. Zhou, H. Yu, X. Xu, F. Han, G. Lubineau, A.C.S. Appl, Mater. Interfaces 9, 4835 (2017)

    Article  CAS  Google Scholar 

  28. J.R. Jeong, H. Park, S.W. Jin, S.Y. Hong, S.S. Lee, J.S. Ha, Adv. Funct. Mater. 25, 4228 (2015)

    Article  CAS  Google Scholar 

  29. S. Chen, Z. Lou, D. Chen, K. Jiang, G. Shen, Adv. Mater. Technol. 1, 1600136 (2016)

    Article  CAS  Google Scholar 

  30. J. Lee, S. Kim, J. Lee, D. Yang, B.C. Park, S. Ryu, I. Park, Nanoscale 20, 1 (2014)

    CAS  Google Scholar 

  31. S. Ryu, P. Lee, J.B. Chou, R. Xu, R. Zhao, A.J. Hart, S.G. Kim, ACS Nano 9, 5929 (2015)

    Article  CAS  Google Scholar 

  32. J.T. Muth, D.M. Vogt, R.L. Truby, Y. Mengüç, D.B. Kolesky, R.J. Wood, J.A. Lewis, Adv. Mater. 26, 6307 (2014)

    Article  CAS  Google Scholar 

  33. N. Luo, W. Dai, C. Li, Z. Zhou, L. Lu, C.C.Y. Poon, S.-C. Chen, Y. Zhang, N. Zhao, Adv. Funct. Mater. 26, 1178 (2016)

    Article  CAS  Google Scholar 

  34. Y. Ma, Y. Yue, H. Zhang, F. Cheng, W. Zhao, J. Rao, S. Luo, J. Wang, X. Jiang, Z. Liu, N. Liu, Y. Gao, ACS Nano 12, 3209 (2018)

    Article  CAS  Google Scholar 

  35. H. Zhang, N. Liu, Y. Shi, Y. Yue, S. Wang, Y. Ma, L. Wen, L. Li, F. Long, Z. Zou, Y. Gao, A.C.S. Appl, Mater. Interfaces 8, 22374 (2016)

    Article  CAS  Google Scholar 

  36. H. Chen, Z. Su, Y. Song, X. Cheng, X. Chen, B. Meng, Z. Song, D. Chen, H. Zhang, Adv. Funct. Mater. 27, 1604434 (2016)

    Article  CAS  Google Scholar 

  37. J. Li, S. Zhao, X. Zeng, W. Huang, Z. Gong, G. Zhang, R. Sun, C.P. Wong, A.C.S. Appl, Mater. Interfaces 8, 18954 (2016)

    Article  CAS  Google Scholar 

  38. L. Lv, P. Zhang, T. Xu, L. Qu, A.C.S. Appl, Mater. Interfaces 9, 22885 (2017)

    Article  CAS  Google Scholar 

  39. J. Park, S. Wang, M. Li, C. Ahn, J.K. Hyun, D.S. Kim, D.K. Kim, J.A. Rogers, Y. Huang, S. Jeon, Nat. Commun. 916, 1 (2012)

    Google Scholar 

  40. M. Chen, L. Zhang, S. Duan, S. Jing, H. Jiang, C. Li, Adv. Funct. Mater. 24, 7548 (2014)

    Article  CAS  Google Scholar 

  41. Y. Song, H. Chen, Z. Su, X. Chen, L. Miao, J. Zhang, X. Cheng, H. Zhang, Small 13, 1702091 (2017)

    Article  CAS  Google Scholar 

  42. H.B. Yao, J. Ge, C.F. Wang, X. Wang, W. Hu, Z.J. Zheng, Y. Ni, S.H. Yu, Adv. Mater. 25, 6692 (2013)

    Article  CAS  Google Scholar 

  43. H. Park, J.W. Kim, S.Y. Hong, G. Lee, D.S. Kim, J.H. Oh, S.W. Jin, Y.R. Jeong, S.Y. Oh, J.Y. Yun, J.S. Ha, Adv. Funct. Mater. 28, 1707013 (2018)

    Article  CAS  Google Scholar 

  44. R. Iglio, S. Mariani, V. Robbiano, L. Strambini, G. Barillaro, A.C.S. Appl, Mater. Interfaces 10, 13877 (2018)

    Article  CAS  Google Scholar 

  45. T. Wang, J. Li, Y. Zhang, F. Liu, B. Zhang, Y. Wang, R. Jiang, G. Zhang, R. Sun, C.-P. Wong, Chem. Eur. J. 25, 6378 (2019)

    Article  CAS  Google Scholar 

  46. L. Ding, S. Xuan, L. Pei, S. Wang, T. Hu, S. Zhang, X. Gong, A.C.S. Appl, Mater. Interfaces 10, 30774 (2018)

    Article  CAS  Google Scholar 

  47. Y. Gao, G. Yu, J. Tan, F. Xuan, Sens. Actuat. A 280, 205 (2018)

    Article  CAS  Google Scholar 

  48. G. Yu, J. Hu, J. Tan, Y. Gao, Y. Lu, F. Xuan, Nanotechnology 29, 115502 (2018)

    Article  CAS  Google Scholar 

  49. L. Dan, S. Shi, H.-J. Chung, A. Elias, A.C.S. Appl, Nano Mater. 2, 4869 (2019)

    Article  CAS  Google Scholar 

  50. C. Mu, Y. Song, W. Huang, A. Ran, R. Sun, W. Xie, H. Zhang, Adv. Funct. Mater. 28, 1707503 (2018)

    Article  CAS  Google Scholar 

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Acknowledgements

This work was supported by the Program for Talent Scientific Research Fund of LNPU (No. 2015XJJ-003) and Scientific Research Fund of Liaoning Provincial Education Department (No. L2020039).

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Correspondence to Jiuyu Ji.

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Yuan, N., Wang, C., Ji, J. et al. A wearable and sensitive carbon black-porous polydimethylsiloxane based pressure sensor for human physiological signals monitoring. J Mater Sci: Mater Electron 32, 27656–27665 (2021). https://doi.org/10.1007/s10854-021-07143-3

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