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Synthesis and study of impendence spectroscopy properties of La0.6Ca0.2Na0.2MnO3 manganite perovskite prepared using sol–gel method

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Abstract

La0.6Ca0.2Na0.2MnO3 manganite was prepared using sol–gel method. Rietveld refinement of XRD pattern indicates that the prepared sample crystallizes in the rhombohedral \(R\overline{3}c\) structure. The impendence spectroscopy properties of the sample were studied by performing a series of measurements as a function of temperature and frequency of conductivity, dielectric constants, modulus, and impedance. From these measurements, the metal–semiconductor behavior was observed for the sample at a transition temperature of the order of 240 K. The studies of imaginary part of permittivity and tangent loss reveal that the prepared material may be a good candidate for low-frequency energy storage devices. An electrical relaxation phenomenon with non-Debye nature was observed in variations of imaginary parts of modulus and impedance. Electrical parameters deduced from the Nyquist plots analyses using an equivalent circuit reveal that the conduction process for the sample was caused due to the grain boundaries contribution.

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References

  1. S. Hcini, S. Zemni, A. Triki, H. Rahmouni, M. Boudard, J. Alloys Compd. 509, 1394 (2011)

    CAS  Google Scholar 

  2. G.H. Jonker, J.H. van Santen, Physica 16, 337 (1950)

    CAS  Google Scholar 

  3. J.H. Van Santen, G.H. Jonker, Physica 16, 599 (1950)

    Google Scholar 

  4. E.O. Wollan, W.C. Koehler, Phys. Rev. 100, 545 (1955)

    CAS  Google Scholar 

  5. M.B. Salomon, M. Jaime, Rev. Mod. Phys. 73, 583 (2001)

    Google Scholar 

  6. C. Zener, Phys. Rev. 81, 440 (1951)

    CAS  Google Scholar 

  7. R. von Helmolt, J. Wecker, B. Holzapfel, L. Schultz, K. Samwer, Phys. Rev. Lett. 71, 2331 (1993)

    Google Scholar 

  8. S. Jin, T.H. Tiefel, M. McCormack, R.A. Fastnacht, R. Ramesh, L.H. Chen, Science 264, 413 (1994)

    CAS  Google Scholar 

  9. H.D. Zhou, R.K. Zheng, G. Li, S.J. Feng, F. Liu, X.J. Fan, X.G. Lia, Eur. Phys. J. B 26, 467 (2002)

    CAS  Google Scholar 

  10. M. Pissas, G. Papavassiliou, J. Phys.: Condens. Matter 16, 6527 (2004)

    CAS  Google Scholar 

  11. B.M. Nagabhushana, R.P. Sreekanth Chakradhar, K.P. Ramesh, C. Shivakumara, G.T. Chandrappa, Mater. Chem. Phys. 102, 47 (2007)

    CAS  Google Scholar 

  12. R. Laiho, K.G. Lisunov, E. Lahderanta, V.N. Stamov, V.S. Zakhvalinskii, J. Phys.: Condens. Matter 13, 1233 (2001)

    CAS  Google Scholar 

  13. A.E. Pantoja, H.J. Trodahl, R.G. Buckley, Y. Tomioka, Y. Tokura, J. Phys.: Condens. Matter 13, 3741 (2001)

    CAS  Google Scholar 

  14. S.V. Trukhanov, N.V. Kasper, I.O. Troyanchuk, M. Tovar, H. Szymczak, K. Bärner, J. Solid State Chem. 169, 85 (2002)

    CAS  Google Scholar 

  15. Q. Yang, J. Yao, K. Zhang, W. Wang, X. Zuo, H. Tang, M. Wu, G. Li, J. Electroanal. Chem. 833, 1 (2019)

    CAS  Google Scholar 

  16. X.H. Huang, H.Y. Lin, Z.J. Cheng, Phys B: Condens Matter 529, 16 (2018)

    CAS  Google Scholar 

  17. T.-L. Phan, Y.D. Zhang, P. Zhang, T.D. Thanh, S.C. Yu, J. Appl. Phys. 112, 093906 (2012)

    Google Scholar 

  18. P. Singh, V. Kumar, G.L. Bhalla, P.K. Siwach, O.N. Srivastava, N. Khare, Solid State Commun. 140, 395 (2006)

    CAS  Google Scholar 

  19. R. Yadav, V. Shelke, J Mater Sci: Mater Electron 24, 1141 (2013)

    CAS  Google Scholar 

  20. T.A. Ho, N.T. Dang, T.-L. Phan, D.S. Yang, B.W. Lee, S.C. Yu, J. Alloys Compd. 676, 305 (2016)

    CAS  Google Scholar 

  21. F. Ayadi, S. Ammar, W. Cheikhrouhou-Koubaa, A. Cheikhrouhou, T. Gaudisson, S. Reguer, S. Nowak, J. Monnier, L. Sicard, J. Alloys Compd. 691, 474 (2017)

    CAS  Google Scholar 

  22. G. Dong, Y. Liu, S. Zhang, K. Chu, H. Li, X. Pu, T. Sun, F. Ji, X. Liu, Ceram. Int. 45, 21448 (2019)

    CAS  Google Scholar 

  23. U. Chaudhuri, A. Chanda, R. Mahendiran, J. Magn. Magn. Mater. 499, 166287 (2020)

    Google Scholar 

  24. H.M. Rietveld, J. Appl. Crystallogr. 2, 65 (1969)

    CAS  Google Scholar 

  25. R. Hamdi, A. Tozri, M. Smari, K. Nouri, E. Dhahri, L. Bessais, J. Mol. Struct. 1175, 844 (2019)

    CAS  Google Scholar 

  26. S.O. Manjunatha, A. Rao, V.P.S. Awana, G.S. Okram, J. Magn. Magn. Mater. 394, 130 (2015)

    CAS  Google Scholar 

  27. O.Z. Yanchevskii, A.I. Tovstolytkin, O.I. V’yunov, D.A. Durilin, A.G. Belous, Inorg Mater. 40, 744 (2004)

    CAS  Google Scholar 

  28. N. Dodiya, D. Varshney, J. Mol. Struct. 1031, 104 (2013)

    CAS  Google Scholar 

  29. E. Oumezzine, S. Hcini, E.K. Hlil, E. Dhahri, M. Oumezzine, J. Alloys Compd. 615, 553 (2014)

    CAS  Google Scholar 

  30. S. Khadhraoui, A. Triki, S. Hcini, S. Zemni, M. Oumezzine, J. Magn. Magn. Mater. 371, 69 (2014)

    CAS  Google Scholar 

  31. M. Hsini, N. Hamdaoui, S. Hcini, M.L. Bouazizi, S. Zemni, L. Beji, Phase Transit 91, 316 (2018)

    CAS  Google Scholar 

  32. S. Hcini, S. Khadhraoui, A. Triki, S. Zemni, M. Boudard, M. Oumezzine, J. Supercond. Nov. Magn. 27, 195 (2014)

    CAS  Google Scholar 

  33. S. Hcini, E. Oumezzine, M. Baazaoui, H. Rahmouni, K. Khirouni, E.K. Hlil, M. Oumezzine, Appl. Phys. A. 120, 1453 (2015)

    CAS  Google Scholar 

  34. A. Dhahri, J. Dhahri, S. Hcini, N. Talbi, E.K. Hlil, M. Oumezzine, K. Khirouni, Appl. Phys. A 120, 247 (2015)

    CAS  Google Scholar 

  35. H. Rahmouni, A. Dhahri, K. Khirouni, J. Alloys Compd. 591, 259 (2014)

    CAS  Google Scholar 

  36. R. Bellouz, S. Kallel, K. Khirouni, O. Pena, M. Oumezzine, Ceram. Int. 41, 1929 (2015)

    CAS  Google Scholar 

  37. M. Chebaane, N. Talbi, A. Dhahri, M. Oumezzine, K. Khirouni, J. Magn. Magn. Mater. 426, 646 (2017)

    CAS  Google Scholar 

  38. K. Funke, Prog. Solid State Chem. 22, 111 (1993)

    CAS  Google Scholar 

  39. S. Hcini, A. Omri, M. Boudard, M.L. Bouazizi, A. Dhahri, K. Touileb, J Mater Sci Mater. Electron. 29, 6879 (2018)

    CAS  Google Scholar 

  40. D. Tlili, N. Hamdaoui, S. Hcini, M.L. Bouazizi, S. Zemni, Phase Transit 90, 644 (2017)

    CAS  Google Scholar 

  41. M.H. Dhaou, S. Hcini, A. Mallah, M.L. Bouazizi, A. Jemni, Appl. Phys. A. 8, 123 (2017)

    Google Scholar 

  42. E. Oumezzine, S. Hcini, F.I.H. Rhouma, M. Oumezzine, J. Alloys Compd. 726, 187 (2017)

    CAS  Google Scholar 

  43. L. Alexander, H.P. Klug, J. Appl. Phys. 21, 137 (1950)

    CAS  Google Scholar 

  44. N.H. Vasoya, P.K. Jha, K.G. Saija, S.N. Dolia, K.B. Zankat, K.B. Modi, J. Electron. Mater. 45, 917 (2016)

    CAS  Google Scholar 

  45. S. Saha, T.P. Sinha, Phys. Rev. B 65, 1341 (2005)

    Google Scholar 

  46. K.P. Padmasree, D.D. Kanchan, A.R. Kulkami, Solid State Ionics 177, 475 (2006)

    CAS  Google Scholar 

  47. R. Bergman, J. Appl. Phys. 88, 1356 (2000)

    CAS  Google Scholar 

  48. K.S. Rao, P.M. Krishna, D.M. Prasad, D. Gangadharudu, J. Mater. Sci. 42, 4801 (2007)

    CAS  Google Scholar 

  49. F.B. Abdallah, A. Benali, S. Azizi, M. Triki, E. Dhahri, M.P.F. Graça, M.A. Valente, J. Mater. Sci. Mater. Electron. 30, 8457 (2019)

    CAS  Google Scholar 

  50. F.B. Abdallah, A. Benali, M. Triki, E. Dhahri, M.P.F. Graça, M.A. Valente, Superlattice Microstruct. 117, 260 (2018)

    CAS  Google Scholar 

  51. S. Khadhraoui, A. Triki, S. Hcini, S. Zemni, M. Oumezzine, J. Alloys Compd. 574, 290 (2013)

    CAS  Google Scholar 

  52. Johnson D. ZView: ass software program for IES analysis. Version 2.8. Southern Pines, NC: Scribner Associates, Inc.; 2008.

Download references

Acknowledgements

This work is supported by the Deanship of Scientific Research at Prince Sattam Bin Abdulaziz University under the research Project Number 2017/01/7373.

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Authors and Affiliations

  1. Department of Physics, College of Science, Qassim University, Buraidah, 51452, Saudi Arabia

    Faisal Alresheedi

  2. Research Unit of Valorization and Optimization of Exploitation of Resources, Faculty of Science and Technology of Sidi Bouzid, University Campus Agricultural City, University of Kairouan, 9100, Sidi Bouzid, Tunisia

    Sobhi Hcini

  3. Department of Mechanical Engineering, College of Engineering, Prince Sattam Bin Abdulaziz University, Alkharj, 11942, Saudi Arabia

    Mohamed Lamjed Bouazizi

  4. LMGP, CNRS, University of Grenoble Alpes, 38000, Grenoble, France

    Michel Boudard

  5. Laboratory of Physical Chemistry of Materials, Faculty of Science of Monastir, Department of Physics, University of Monastir, 5019, Monastir, Tunisia

    Abdessalem Dhahri

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  1. Faisal Alresheedi
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  3. Mohamed Lamjed Bouazizi
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Correspondence to Sobhi Hcini.

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Alresheedi, F., Hcini, S., Bouazizi, M.L. et al. Synthesis and study of impendence spectroscopy properties of La0.6Ca0.2Na0.2MnO3 manganite perovskite prepared using sol–gel method. J Mater Sci: Mater Electron 31, 8248–8257 (2020). https://doi.org/10.1007/s10854-020-03360-4

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