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Enhanced electrical properties in A-site K/Ce and B-site W/Cr co-substituted CaBi2Nb2O9 high temperature piezoelectric ceramic

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Abstract

A-site K/Ce and B-site W/Cr co-substituted CaBi2Nb2O9 ceramics were synthesized by a conventional solid-state reaction process. The structures, piezoelectricity and electrical conduction behaviors were investigated in detail. The Ca0.95(K1/2Ce1/2)0.05Bi2Nb1.99(W2/3Cr1/3)0.01O9 ceramic exhibited best properties with a high d33 (piezoelectric coefficient) of ~ 18.4 pC/N and a high TC (Curie temperature) of ~ 917 °C. In addition, the ceramic displayed an excellent thermal stability performance such that d33 remained 94% of its initial value even after annealing at 900 °C for 2 h. The planar electromechanical coupling factor was observed to increase from 9.00% at room temperature to 15.24% at 600 °C. Furthermore, a high electrical resistivity of 1.16 × 105 Ω cm at 600 °C and a good fatigue property were also achieved with this composition. The Ca0.95(K1/2Ce1/2)0.05Bi2Nb1.99(W2/3Cr1/3)0.01O9 ceramic was found to be a promising candidate for high-temperature piezoelectric applications.

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Acknowledgments

This work was supported by the National Natural Science Foundation of China (Nos. 51302056, 51502067), Key research and development projects of Zhejiang Province (2017C01056).

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Authors and Affiliations

  1. College of Electronics and Information, Hangzhou Dianzi University, Hangzhou, 310018, China

    Zhenning Chen, Xudong Li, Linsheng Sheng, Lili Li, Fei Wen, Peng Zheng, Wei Wu & Liang Zheng

  2. School of Materials Sciences and Engineering, Liaocheng University, Liaocheng, 252059, China

    Juan Du

  3. College of Materials and Environmental Engineering, Hangzhou Dianzi University, Hangzhou, 310018, China

    Wangfeng Bai

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  1. Zhenning Chen
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Correspondence to Peng Zheng.

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Chen, Z., Li, X., Sheng, L. et al. Enhanced electrical properties in A-site K/Ce and B-site W/Cr co-substituted CaBi2Nb2O9 high temperature piezoelectric ceramic. J Mater Sci: Mater Electron 30, 11727–11734 (2019). https://doi.org/10.1007/s10854-019-01534-3

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