Abstract
The ceramics in (1 − x) CaLa4Ti5O17-xTiO2 (0 ≤ x ≤ 0.1) series were fabricated via conventional solid-state mix oxide sintering route. Their phase and microwave dielectric properties were investigated. Ca0.1La0.60TiO3 formed as the major phase while CaLa4Ti5O17 formed as secondary phase for the composition with x = 0. The addition of TiO2 content suppressed the formation of the parent CaLa4Ti5O17 phase that finally disappeared and Ca0.1La0.60TiO3 was formed as the only phase. The addition of TiO2 increased εr, Q u f o and τf values. In the present study, ε r ~ 155, Q u f o ~ 12678 GHz and τ f ~ 8.9 was achieved for the composition with x = 0.1 sintered at 1450 °C for 4 h.
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A. Manan, I. Qazi, Dielectric properties of ceramics for microwave and millimeter wave applications, 2013 International Conference on Aerospace Science & Engineering (ICASE), 2013 IEEE. (2013)
A. Manan, Y. Iqbal, Mater. Res. Bull. 47, 883 (2012)
Y.C. Chen, Y.W. Zeng, Opt. Technol. Lett. 51, 98 (2009)
Y.C. Chen, S.H. Yao, R.J. Tasi, K.C. Chen, J. Alloys. Compds. 486, 410 (2009)
Y.C. Chen, K.C. Chen, S.C. Wang, Ferroelectr. Lett. 37, 83 (2010)
I.N. Jawahar, N. Santha, M.T. Sebastian, P. Mohanan, J. Mater. Res. 17, 3084 (2002)
Y. Iqbal, A. Manan, I.M. Reaney, Mater. Res. Bull. 46, 1092 (2011)
B. Jancar, D. Suvorov, M. Valant, J. Mater, Sci. Lett. 20, 71 (2001)
L. Fang, H. Su, Q. Yu, H. Zhang, X. Cui, Mater. Lett. 62, 4121 (2008)
C. Hu, L. Fang, H. Su, L. Liu, J. Alloys. Compds. 487, 504 (2009)
H. Kagata, J. Kato, Jpn. J. Appl. Phys. 33, 5463 (1994)
R.I. Scott, M. Thomas, C. Hampson, J. Eur. Ceram. Soc. 23, 2467 (2003)
D. Liu, X.M. Chen, X. Hu, Mater. Lett. 61, 1166 (2007).
A. Manan, Y. Iqbal, Bull. Mater. Sci. 37, 1215 (2014).
A. Manan, I. Ullah, A.S. Ahmad, A. Ullah, J. Mater. Sci. 27, 6128 (2016)
G. Subodh, M.T. Sebastian, J. Am. Ceram. Soc. 90, 2266 (2007)
C.F. Shih, W.M. Li, M.M. Lin, C.Y. Hsiao, K.T. Hung, J. Alloys Compd. 485, 408 (2009)
I.S. Cho, S.K. Kang, D.W. Kim, K.S. Hong, J. Eur. Ceram. Soc. 26, 2007 (2006)
S.H. Yoon, G.K. Choi, D.W. Kim, S.Y. Cho, K.S. Hong, J. Eur. Ceram. Soc. 27, 3087 (2007)
K. Fukuda, R. Kitoh, I. Awai, Jpn. J. Appl. Phys. 32, 4584 (1993)
J.J. Bian, K. Yan, H.B. Gao, Mater. Chem. Phys. 96, 349 (2006)
C.L. Huang, J.T. Tsai, Y.B. Chen, Mater. Res. Bull. 36, 547 (2001)
Acknowledgements
The authors acknowledge the financial support extended by the Higher Education Commission Islamabad Pakistan under “Pakistan Program for Collaborative Research (PPCR)”. The authors also acknowledge the laboratory support extended by the School of Materials Science and Engineering Wuhan University of Technology, China.
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Manan, A., Liu, H., Khan, J. et al. The effects of TiO2 addition on the phase formation and microwave dielectric properties of CaLa4Ti5O17 ceramic. J Mater Sci: Mater Electron 28, 15552–15555 (2017). https://doi.org/10.1007/s10854-017-7443-z
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DOI: https://doi.org/10.1007/s10854-017-7443-z