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Investigation into the microstructure and soft magnetic property of co-sputtering FeNi–MgO nanogranular films

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Abstract

A series of FeNi–MgO nanogranular soft magnetic films with different sputtering powers of MgO were deposited by co-sputtering at room temperature on naturally oxidized silicon substrates. By adjusting the sputtering power of MgO, the average grain size of FeNi–MgO granular film reduces from 6.5 to 4 nm. The easy-axis coercivity Hce decreases from 8 to 0.3 Oe and saturation field Hs decreases from 14 to 1 Oe. When the sputtering power of MgO is above 60 W, Hce and Hs keep nearly unchanged. The results of permeability spectra indicate that the resonant frequency fr can be modulated in a small range from 0.61 to 0.71 GHz. Meanwhile, Gilbert damping α first decreases and then increases with increasing the sputtering power of MgO. The initial permeability is higher than 500 when the frequency is below 0.5 GHz, indicating that the FeNi–MgO nanogranular films are the excellent candidate for a high-frequency application.

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References

  1. Greaves SJ, Kanai Y (2019) Effect of spin-torque oscillator tilt angle in microwave-assisted magnetic recording. IEEE Trans Magn 55:300404

    Article  Google Scholar 

  2. Lekas MS, Davies R, Sturcken N (2019) Magnetic thin-film inductors with induced radial anisotropy for improved inductance density. IEEE Magn Lett 10(7):100604

    Google Scholar 

  3. Wu H, Khdour M, Apsangi P, Yu H (2017) High-frequency magnetic thin-film inductor integrated on flexible organic substrates. IEEE Trans Magn 53:2004507

    Google Scholar 

  4. Röbisch V, Yarar E, Urs NO, Teliban I, Knöchel R, McCord J, Quandt E, Meyners D (2015) Exchange biased magnetoelectric composites for magnetic field sensor application by frequency conversion. J Appl Phys 117:17B513

    Article  Google Scholar 

  5. Kong S, Okamoto T, Nakagawa S (2003) Improvement of soft magnetic properties of Fe–Co–B underlayer with large saturation magnetization by Ni–Fe–O seedlayers. J Appl Phys 93:6778

    Article  Google Scholar 

  6. Liu X, Zangari G, Shamsuzzoha M (2003) Structural and magnetic characterization of electrodeposited, high moment FeCoNi films. J Electrochem Soc 150:C159–C168

    Article  Google Scholar 

  7. Ge S, Yang X, Kim Y, Xi K, Kou L, Yao X, Li D, Wang B, Wang X (2005) Study on mechanism of soft magnetic properties for high-frequency application in Ni75Fe25–SiO2 granular films. Phys Stat Sol A. 202:2021–2027

    Article  Google Scholar 

  8. Cao Y, Zhang Y, Ohnuma S, Kobayashi N, Masumoto H (2015) Structure and isotropic high-frequency response of Co-HfN nanogranular films. IEEE Trans Magn 51:2801404

    Google Scholar 

  9. Ge S, Yao D, Yamaguchi M, Yang X, Zuo H, Ishii T, Zhou D, Li F (2007) Microstructure and magnetism of FeCo–SiO2 nano-granular films for high frequency application. J Phys D Appl Phys 40:3660–3664

    Article  Google Scholar 

  10. Seki TO, Takahashi YK, Hono K (2008) Microstructure and magnetic properties of FePt–SiO2 granular films with Ag addition. J Appl Phys 103:023910

    Article  Google Scholar 

  11. Geng H, Wei JQ, Wang ZW, Nie SJ, Guo HZ, Wang LS, Chen Y, Yue GH, Peng DL (2013) Soft magnetic property and high-frequency permeability of [Fe80Ni20–O/TiO2] n multilayer thin films. J. Alloys Compd. 576:13–17

    Article  Google Scholar 

  12. Kenane S, Voiron J, Benbrahim N, Chaînet E, Robaut F (2006) Magnetic properties and giant magnetoresistance in electrodeposited Co–Ag granular films. J Magn Magn Mater 297:99–106

    Article  Google Scholar 

  13. Yildiz F, Kazan S, Aktas B, Tarapov SI, Tagirov L, Granovsky B (2006) Ferromagnetic resonance studies on (Co40Fe40B20)x(SiO2)1−x granular magnetic films. J Magn Magn Mater 305:24–27

    Article  Google Scholar 

  14. Bai G, Wu C, Jin J, Yan M (2016) Structural, electron transportation and magnetic behavior transition of metastable FeAlO granular films. Sci Rep 6:24410

    Article  Google Scholar 

  15. Wang C, Xiao X, Hu H, Rong Y, Hsu TY (2007) Nanoparticle morphology in FeNi–Cu granular films with giant magnetoresistance. Phys B 392:72–78

    Article  Google Scholar 

  16. Liang HF, Liu CL, Liang ZH, Meng LG (2008) Electron emission characteristics of Al–AlN granular films. Appl Surf Sci 254:6922–6927

    Article  Google Scholar 

  17. Bai G, Jin J, Wu C, Yan M (2018) Microstructure and electromagnetic performance of the FeCoAlON films tuned by N2 pressure during reactive pulsed laser deposition. J. Alloys Compd. 739:866–872

    Article  Google Scholar 

  18. Bai G, Jin J, Wu C, Yan M (2019) Ultrafine FeCo nanoparticles isolated by ultrathin dielectric shells for microwave application. ACS Appl Nano Mater 2(6):3570–3576

    Article  Google Scholar 

  19. Wang Y, Zhang H, Wang L, Bai F (2014) Compositional dependence of magnetic and high frequency properties of nanogranular FeCo–TiO2 films. J Appl Phys 115:17A306

    Article  Google Scholar 

  20. Peng D, Wang J, Wang L, Liu X, Wang Z, Chen Y (2013) Electron transport properties of magnetic granular films. Sci China Phys Mech Astron 56:15–27

    Article  Google Scholar 

  21. Kravets VG, Poperenko LV, Yurgelevych IV, Pogorily AM, Kravets AF (2005) Optical and magneto-optical properties and magnetorefractive effect in metal-insulator CoFe–Al2O3 granular films. J Appl Phys 98:043705

    Article  Google Scholar 

  22. Van Cuong G, Anh Tuan N, Tuan Anh N, Van Tuong D, Anh Tue N, Tuyet Nga N, Phuong Lien D (2015) Structural characteristics and magnetic properties of Al2O3 matrix-based Co-cermet nanogranular films. J Mater 10:834267

    Google Scholar 

  23. Kondo K, Chiba T, Ono H, Yoshida S, Shimada Y, Matsushita N, Abe M (2006) Conducted noise suppression up to GHz range by spin-sprayed Ni0.2ZnxFe2.8−xO4 (x = 0:3, 0.6) films having different natural resonance frequencies. J Magn Magn Mater 301:107–111

    Article  Google Scholar 

  24. Hao G, Zhang D, Jin L, Zhang H, Jia N, Tang X (2015) Compositional dependence of magnetic and high frequency properties of nanogranular CoFe–Yttrium-doped Zirconia films. J Alloy Compd 648:270–275

    Article  Google Scholar 

  25. Shimada Y, Ma J, Ito T, Yanagi K, Endo Y, Muroga S, Yamaguchi M (2014) Performance of crossed anisotropy multilayered CoZrNb films as IC chip level electromagnetic noise suppressor. IEEE Trans Magn 50:2801704

    Article  Google Scholar 

  26. Lu G, Huang X, Piao H, Pan L (2016) The dependence of electromagnetic noise suppress characteristics on magnetic and high-frequency properties of FeCoSiO thin films. J Alloy Compd 668:107–112

    Article  Google Scholar 

  27. Schoen MA, Thonig D, Schneider ML, Silva TJ, Nembach HT, Eriksson O, Karis O, Shaw JM (2016) Ultra-low magnetic damping of a metallic ferromagnet. Nat Phys 12:839

    Article  Google Scholar 

  28. Zhu Z, Feng H, Xie H, Liu Q, Wang J (2018) Enhancement of damping in FeNiN film due to two-magnon scattering effect. Appl Phys Lett 113:232402

    Article  Google Scholar 

  29. Lindner J, Barsukov I, Raeder C, Hassel C, Posth O, Meckenstock R, Landeros P, Mills DL (2009) Two-magnon damping in thin films in case of canted magnetization: theory versus experiment. Phys Rev B 80:224421

    Article  Google Scholar 

  30. Wei J, Wang J, Liu Q, Li X, Cao D, Sun X (2014) An induction method to calculate the complex permeability of soft magnetic films without a reference sample. Rev Sci Instrum 85:054705

    Article  Google Scholar 

  31. Lv Y, Ji L, Liu X, Li H, Zhou H, Chen J (2012) Influence of substrate bias voltage on structure and properties of the CrAlN films deposited by unbalanced magnetron sputtering. Appl Surf Sci 258:3864–3870

    Article  Google Scholar 

  32. Chen LC, Chen CC, Sung YT, Hsu YY (2009) Oblique-angle sputtering effects on characteristics of nanocolumnar structure anisotropic indium tin oxide films. J Electrochem Soc 156:H471–H474

    Article  Google Scholar 

  33. Liu XL, Wang LS, Xu R, Luo Q, Xu L, Yuan BB, Zou CY, Wang JB, Peng DL (2015) Influence of total film thickness on high-frequency magnetic properties of the [FeCoSiN/SiNx]n multilayer thin films. J Magn Magn Mater 374:85–91

    Article  Google Scholar 

  34. Wei Q, Li Z, Zhou X, Tian Y, Feng L, Yao D (2012) Dependence of soft magnetic properties and high frequency characteristics on film thickness for Ni75Fe25–ZnO nano-granular films. J Alloy Compd 513:23–26

    Article  Google Scholar 

  35. Phuoc NN, Ong CK (2012) Diluted antiferromagnet effect on magnetic and microwave characteristics of exchange-biased multilayered thin films. J Appl Phys 111:093919

    Article  Google Scholar 

  36. Liu Y, Zhang J, Yu L, Jia G, Jing C, Cao S (2005) Magnetic and frequency properties for nanocrystalline Fe–Ni alloys prepared by high-energy milling method. J Magn Magn Mater 285:138–144

    Article  Google Scholar 

  37. Ingvarsson S, Ritchie L, Liu XY, Xiao G, Slonczewski JC, Trouilloud PL, Koch RH (2002) Role of electron scattering in the magnetization relaxation of thin Ni81Fe19 films. Phys Rev B 66:214416

    Article  Google Scholar 

  38. Wu K, Tang M, Li D, Guo X, Cui B, Yun T, Zuo Y, Xi Y, Zhang ZZ (2017) Modulation of magnetic damping constant of Fe2Co films by heavy doping of rare-earth Yb. J Phys D Appl Phys 50:135001

    Article  Google Scholar 

  39. Wei J, Zhu Z, Feng H, Du J, Liu Q, Wang J (2015) Top-down control of dynamic anisotropy in permalloy thin films with stripe domains. J Phys D Appl Phys 48:465001

    Article  Google Scholar 

Download references

Acknowledgements

The authors gratefully acknowledge the National Natural Scientific Fund of China (51771086 and 11574121) for the financial support.

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Correspondence to Jianbo Wang.

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Feng, H., Zhu, Z., Liu, W. et al. Investigation into the microstructure and soft magnetic property of co-sputtering FeNi–MgO nanogranular films. J Mater Sci 54, 14189–14196 (2019). https://doi.org/10.1007/s10853-019-03862-5

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