A calculation of the removal of radionuclides by groundwaters from a subsurface repository of solid low-level waste was performed. A two-dimensional model of the groundwater flow and advective-dispersive transport of radionuclides in a vertical section of a subsurface aquifer, along which radionuclide-contaminated groundwater moves from the repository to an open body of water, was studied. Data from many years of experimentation on the leaching of cemented low-level waste were used in the calculations. It was shown that the rocks of the aquifer effectively retain medium half-life radionuclides (60Co, 137Cs, 90Sr). An engineered barrier – a 0.7 m thick layer of consolidated bentonite clay – can secure the safety of a repository for long-lived transuranium radionuclides (235U, 239Pu) for 20000 years.
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References
B. T. Kochkin, V. I. Malkovskii, and S. V. Yudintsev, Scientific Basis for Safety Assessment of Geological Isolation of Long-Lived Radioactive Waste (Yenisei project), IGEM RAS, Moscow (2017).
G. deMarsily, Quantitative Hydrogeology, Academic Press, Orlando (1986).
O. Zenkevich and K. Morgan, Finite Elements and Approximation, Mir, Moscow (1986).
V. I. Malkovskii and A. A. Pek, “Assessment of the impact of high-permeability fault on the transport of pollutants by regional groundwater flow,” Geol. Rudn. Mestorozhd., 43, No. 3, 243–251 (2001).
P. Roache, Computational Fluid Dynamics, Mir, Moscow (1980).
J. Fried, Pollution of Groundwater [Russian translation], Nedra, Moscow (1981).
S. Sheppard, J. Long, and B. Sanipelli, Solid/Liquid Partition Coefficients (K d ) for Selected Soils and Sediments at Forsmark and Laxemar-Simpevarp, Svensk Kämbränslehantering AB, Stockholm (2009).
I. A. Sobolev, S. A. Dmitriev, A. S. Barinov, et al., “39-Years performance of cemented radioactive waste in a mound type repository,” in: Mat. Res. Soc. Proc., 932, 721–726 (2006).
M. Ojovan (ed.), Handbook of Advanced Radioactive Waste Conditioning Technologies, Woodhead Publishing Ltd., Oxford (2011).
SanPin 2.1.4.1074-01, Drinking Water. Hygienic Requirements for Water Quality of Centralized Drinking Water Supply Systems. Quality Control, Federal Center for State Sanitary and Epidemiological Surveillance of the Ministry of Health of Russia, Moscow (2002).
V. Malkovsky, “Theoretical analysis of colloid-facilitated transport of radionuclides by groundwater,” in: Actinide Nanoparticle Research, S. N. Kalmykov and M. A. Denecke (eds.), Springer-Verlag, Berlin (2011).
A. Kersting, D. Efurd, D. Finnegan, et al., “Migration of plutonium in ground water at the Nevada Test Site,” Nature, 397, No. 1, 56–59 (1999).
B. Honeyman, “Colloidal culprits in contamination,” ibid., 23–24.
V. I. Malkovskii and A. A. Pek, “The effect of colloids on the transport of radionuclides by groundwater,” Geol. Rudn. Mestorozhd., 51, No. 2, 91–106 (2009).
B. Christiansen and B. Torstenfelt, “Diffusion of nickel, strontium, iodine, cesium and americium in loosely compacted bentonite at high pH,” Radiochim. Acta, 44/45, 219–223 (1988).
M. Molera and T. Eriksen, “Diffusion of 22Na+, 85Sr2+, 134Cs+ and 57Co+ in bentonite clays compacted to different densities: experiments and modeling,” Radiochim. Acta, 90, 753–760 (2002).
U. Alonso, T. Missana, M. Garcia-Gutierrez, and A. Patelli, “Diffusion coefficient measurements in consolidated clay by RBS micro-scale profiling,” Appl. Clay Sci., 43, 477–484 (2009).
K. Idemitsu, K. Ishiguro, Y. Yusa, et al, “Plutonium diffusivity in compacted bentonite,” Eng. Geology, 28, 455–462 (1990).
A. Muurinen, “Diffusion of uranium in compacted sodium bentonite,” ibid., 359–367.
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Translated from Atomnaya Énergiya, Vol. 126, No. 2, pp, 102–108, February, 2019.
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Mal’kovskii, V.I., Yudintsev, S.V. & Gupalo, V.S. Assessment of the Safe Isolation of Solid Radwaste in Subsurface Repositories. At Energy 126, 116–123 (2019). https://doi.org/10.1007/s10512-019-00524-2
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DOI: https://doi.org/10.1007/s10512-019-00524-2