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Experimental Observations of Gas-sorption-Induced Strain Gradients and their Implications on Permeability Evolution of Shale

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Abstract

Gas adsorption/desorption can result in swelling/shrinking of the matrix in fractured shale. The significant contrast in permeability between fractures and matrix results in an extended duration for the equilibration of the gas injection or depletion-created pressure difference. This spatially non-uniform pressure dissipation induces non-uniform deformations inside the matrix. We follow this response with carefully constrained laboratory measurements integrated with numerical modelling to explore the relation between the strain gradients that develop in the matrix adjacent to fractures and the evolution of permeability each under conditions of constant confining pressure. The microstructures of the sample were characterized by X-ray computed tomography, field-emission scanning electron microscopy and mercury injection capillary pressure porosimetry. A distributed array of strain gauges was attached to the matrix to directly measure the evolving strain. Then a 3D multiphysics numerical model was built to model the evolution of strain gradients from initial to ultimate equilibrium. The influence of these strain gradients on the evolution of fracture permeability is evaluated by a non-uniform strain-based permeability model. The results indicate that the swelling of the matrix near fractures can also compress the matrix away from the fracture under constant confining pressure conditions. Under the influence of the matrix–fracture interaction, a transient and complex distribution of strain gradients develops within the matrix.

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Abbreviations

b 0 :

Initial fracture aperture (m)

Δb :

Fracture aperture change (m)

f i :

The component of body force in the i –direction (N)

E :

Young's modulus (MPa)

G :

Shear modulus (MPa)

K :

Bulk modulus (MPa)

k m :

The permeability of matrix system (m2)

k m0 :

The initial permeability of matrix system (m2)

k f :

The permeability of fracture system (m2)

k f0 :

The initial permeability of fracture system (m2)

M:

The molecular mass of gas (kg/mol)

p m :

The gas pressure in the matrix systems (MPa)

p f :

The gas pressure in the fracture systems (MPa)

p L :

Langmuir pressure (MPa)

p :

Pore pressure (MPa)

R :

The universal gas constant (J/(mol K))

T :

The absolute gas temperature (K)

u i :

The component of displacement in the i-direction (m)

V L :

Langmuir volume constant (m3/kg)

Φ m :

The porosity of matrix system

Φ f :

The porosity of fracture system

\(\bar{\sigma}\) :

Mean compressive stress (MPa)

\(\varepsilon_e\) :

Total effective volumetric strain

\(\varepsilon_m\) :

Volumetric strain in the shale matrix

\(\varepsilon_{mp}\) :

Effective-stress-induced volumetric strain

\(\varepsilon_{ms}\) :

Sorption-induced volumetric strain

\(\varepsilon_{f}\) :

Fracture strain

\(\varepsilon_{f}^{t}\) :

Uniform strain component

\(\varepsilon\prime_{f}\) :

Non-uniform strain component

\(\varepsilon_{L}\) :

Langmuir volumetric strain constant

ν :

Poisson ratio

α :

Biot coefficient

ρ s :

Shale density (kg/m3)

ρ a :

Gas density at atmospheric pressure (kg/m3)

ρ g :

Gas density (kg/m3)

μ :

Dynamic viscosity of the gas (mPa s)

References

  • Aljamaan H, Alnoaimi K, Kovscek A (2013) In-depth experimental investigation of shale physical and transport properties. In: Paper presented at the In: Unconventional Resources Technology Conference, Denver, Colorado, USA,

  • Alnoaimi K, Kovscek A (2013) Experimental and numerical analysis of gas transport in shale including the role of sorption. In: Paper presented at the In: SPE Annual Technical Conference and Exhibition, New Orleans, Louisiana, USA, 30 September-2 October

  • Alnoaimi KR, Duchateau C, Kovscek (2014) A Characterization and measurement of multi-scale gas transport in shale core samples. In: Unconventional Resources Technology Conference, Denver, Colorado, USA, 25–27 August 2014. pp 1–19. https://doi.org/10.15530/urtec-2014-1920820

  • Chen T, Feng X-T, Cui G, Tan Y, Pan Z (2019) Experimental study of permeability change of organic-rich gas shales under high effective stress. J Nat Gas Sci Eng 64:1–14

    Google Scholar 

  • Chen Y, Jiang C, Yin G, Wojtanowicz AK, Zhang D (2020) Permeability and effective stress in dipping gas shale formation with bedding—experimental study. J Energy Resour Technol 142

  • Cui XA, Bustin RM, Brezovski R, Nassichuk B, Glover K, Pathi V (2010) A new method to simultaneously measure in-situ permeability and porosity under reservoir conditions: implications for characterization of unconventional gas reservoirs. In: Canadian Unconventional Resources and International Petroleum Conference, Calgary, Alberta, Canada, 2010. pp 1–8. https://doi.org/10.2118/138148-MS

  • Cui G, Liu J, Wei M, Feng X, Elsworth D (2018a) Evolution of permeability during the process of shale gas extraction. J Nat Gas Sci Eng 49:94–109

    Google Scholar 

  • Cui G, Liu J, Wei M, Shi R, Elsworth D (2018b) Why shale permeability changes under variable effective stresses: new insights. Fuel 213:55–71. https://doi.org/10.1016/j.fuel.2017.10.068

    Article  Google Scholar 

  • Fan C, Elsworth D, Li S, Zhou L, Yang Z, Song Y (2019) Thermo-hydro-mechanical-chemical couplings controlling CH4 production and CO2 sequestration in enhanced coalbed methane recovery. Energy 173:1054–1077

    Google Scholar 

  • Fink R, Krooss BM, Gensterblum Y, Amann-Hildenbrand A (2017) Apparent permeability of gas shales–superposition of fluid-dynamic and poro-elastic effects. Fuel 199:532–550

    Google Scholar 

  • Firouzi M, Alnoaimi K, Kovscek A, Wilcox J (2014) Klinkenberg effect on predicting and measuring helium permeability in gas shales. Int J Coal Geol 123:62–68. https://doi.org/10.1016/j.coal.2013.09.006

    Article  Google Scholar 

  • Florence FA, Rushing J, Newsham KE, Blasingame TA (2007) Improved permeability prediction relations for low permeability sands. In: Rocky Mountain Oil and Gas Technology Symposium, Denver, Colorado, USA, 16–18 April 2007. pp 1–18. https://doi.org/10.2118/107954-MS

  • Gallé C (2001) Effect of drying on cement-based materials pore structure as identified by mercury intrusion porosimetry: a comparative study between oven-, vacuum-, and freeze-drying. Cem Concr Res 31:1467–1477

    Google Scholar 

  • Gan H, Nandi S, Walker P Jr (1972) Nature of the porosity in American coals. Fuel 51:272–277

    Google Scholar 

  • Gao J, Yu Q (2018) Effect of Water Saturation on Pressure-Dependent Permeability of Carboniferous Shale of the Qaidam Basin, China. Transp Porous Media 123:147–172. https://doi.org/10.1007/s11242-018-1029-y

    Article  Google Scholar 

  • Ghanizadeh A, Amann-Hildenbrand A, Gasparik M, Gensterblum Y, Krooss BM, Littke R (2014) Experimental study of fluid transport processes in the matrix system of the European organic-rich shales: II. Posidonia Shale (Lower Toarcian, northern Germany). Int J Coal Geol 123:20–33

    Google Scholar 

  • Guo F (2014) Experimental Investigation of Shale Permeability. The University of Western Australia

  • He B, Xie L, Zhao P, Ren L, Zhang Y (2020) Highly efficient and simplified method for measuring the permeability of ultra-low permeability rocks based on the pulse-decay technique. Rock Mech Rock Eng 53:291–303

    Google Scholar 

  • Heller R, Vermylen J, Zoback M (2014) Experimental investigation of matrix permeability of gas shales. AAPG Bull 98:975–995. https://doi.org/10.1306/09231313023

    Article  Google Scholar 

  • Hu Q, Ewing RP, Rowe HD (2015) Low nanopore connectivity limits gas production in Barnett formation. J Geophys Res 120:8073–8087

    Google Scholar 

  • Jin G, Pérez HG, Agrawal G, Khodja MR, Ali AZ, Hussaini SR, Jangda ZZ (2015) The impact of gas adsorption and composition on unconventional shale permeability measurement. In: SPE Middle east oil and gas show and conference, Manama, Bahrain, 8–11 March 2015. pp 1–13. https://doi.org/10.2118/172744-MS

  • Kang Y, Chen M, Li X, You L, Yang B (2015) Laboratory measurement and interpretation of nonlinear gas flow in shale. Int J Mod Phys C 26:1550063. https://doi.org/10.1142/S0129183115500631

    Article  Google Scholar 

  • Karacan CÖ (2007) Swelling-induced volumetric strains internal to a stressed coal associated with CO2 sorption. Int J Coal Geol 72:209–220

    Google Scholar 

  • Karacan CÖ, Ruiz FA, Cotè M, Phipps S (2011) Coal mine methane: a review of capture and utilization practices with benefits to mining safety and to greenhouse gas reduction. Int J Coal Geol 86:121–156

    Google Scholar 

  • Katz A, Thompson A (1986) Quantitative prediction of permeability in porous rock. Phys Rev B 34:8179

    Google Scholar 

  • Kiyama T, Nishimoto S, Fujioka M, Xue Z, Ishijima Y, Pan Z, Connell LD (2011) Coal swelling strain and permeability change with injecting liquid/supercritical CO2 and N2 at stress-constrained conditions. Int J Coal Geol 85:56–64

    Google Scholar 

  • Klinkenberg L (1974) The permeability of porous media to liquids and gases. In: Drilling and production practice, New York, USA, pp 200–213.

  • Kumar H, Elsworth D, Mathews J, Marone C (2016) Permeability evolution in sorbing media: analogies between organic-rich shale and coal. Geofluids 16:43–55. https://doi.org/10.1111/gfl.12135

    Article  Google Scholar 

  • Letham EA (2011) Matrix permeability measurements of gas shales: gas slippage and adsorption as sources of systematic. Error. https://doi.org/10.14288/1.0053604

    Article  Google Scholar 

  • Li X, Feng Z, Han G, Elsworth D, Marone C, Saffer D, Cheon D-S (2017) Permeability evolution of propped artificial fractures in green river shale. Rock Mech Rock Eng 50:1473–1485. https://doi.org/10.1007/s00603-017-1186-2

    Article  Google Scholar 

  • Li W, Liu J, Zeng J, Leong Y-K, Elsworth D, Tian J, Li L (2020) A fully coupled multidomain and multiphysics model for evaluation of shale gas extraction. Fuel 278:118214

    Google Scholar 

  • Liu S, Harpalani S (2013) A new theoretical approach to model sorption-induced coal shrinkage or swelling. AAPG Bull 97:1033–1049

    Google Scholar 

  • Liu S, Harpalani S (2014) Determination of the effective stress law for deformation in coalbed methane reservoirs. Rock Mech Rock Eng 47:1809–1820

    Google Scholar 

  • Liu J, Chen Z, Elsworth D, Miao X, Mao X (2010) Evaluation of stress-controlled coal swelling processes. Int J Coal Geol 83:446–455

    Google Scholar 

  • Liu J, Chen Z, Elsworth D, Qu H, Chen D (2011) Interactions of multiple processes during CBM extraction: a critical review. Int J Coal Geol 87:175–189. https://doi.org/10.1016/j.coal.2011.06.004

    Article  Google Scholar 

  • Liu S, Wang Y, Harpalani S (2016) Anisotropy characteristics of coal shrinkage/swelling and its impact on coal permeability evolution with CO2 injection. Greenhouse Gases Sci Technol 6:615–632

    Google Scholar 

  • Liu X, Sheng J, Liu J, Hu Y (2018) Evolution of coal permeability during gas injection—from initial to ultimate equilibrium. Energies 11(10):2800

    Google Scholar 

  • Liu T, Lin B, Fu X, Gao Y, Kong J, Zhao Y, Song H (2020) Experimental study on gas diffusion dynamics in fractured coal: a better understanding of gas migration in in-situ coal seam. Energy 195:117005

    Google Scholar 

  • Lomize G (1951) Flow in fractured rocks. Gosenergoizdat Moscow 127:635

    Google Scholar 

  • Ma Y, Pan Z, Zhong N, Connell LD, Down DI, Lin W, Zhang Y (2016) Experimental study of anisotropic gas permeability and its relationship with fracture structure of Longmaxi Shales, Sichuan Basin, China. Fuel 180:106–115

    Google Scholar 

  • McKernan R, Rutter E, Mecklenburgh J, Taylor K, Covey-Crump S (2014) Influence of effective pressure on mudstone matrix permeability: implications for shale gas production. In: SPE/EAGE European Unconventional Resources Conference and Exhibition, 2014. vol 1. European Association of Geoscientists and Engineers, pp 1–13

  • Moghadam AA, Chalaturnyk R (2015) Laboratory investigation of shale permeability. In: SPE/CSUR Unconventional Resources Conference, Calgary, Alberta, Canada,. pp 1–27. https://doi.org/10.2118/175919-MS

  • Moghadam AA, Chalaturnyk R (2016) Analytical and experimental investigations of gas-flow regimes in shales considering the influence of mean effective stress. SPE J 21:557–572. https://doi.org/10.2118/178429-PA

    Article  Google Scholar 

  • Moghaddam RN, Jamiolahmady M (2016) Fluid transport in shale gas reservoirs: Simultaneous effects of stress and slippage on matrix permeability. Int J Coal Geol 163:87–99. https://doi.org/10.1016/j.coal.2016.06.018

    Article  Google Scholar 

  • Pan Z, Connell LD (2007) A theoretical model for gas adsorption-induced coal swelling. Int J Coal Geol 69:243–252

    Google Scholar 

  • Pan Z, Ma Y, Danesh NN, Connell LD, Sander R, Down DI, Camilleri M (2015a) Measurement of shale anisotropic permeability and its impact on shale gas production. In: SPE Asia Pacific Unconventional Resources Conference and Exhibition, Society of Petroleum Engineers,

  • Pan Z, Ma Y, Danesh NN, Connell LD, Sander R, Down DI, Camilleri M (2015b) Measurement of shale anisotropic permeability and its impact on shale gas production. In: SPE Asia Pacific Unconventional Resources Conference and Exhibition, Brisbane, Australia, pp 1–15. https://doi.org/10.2118/176955-MS

  • Peng S, Loucks B (2016) Permeability measurements in mudrocks using gas-expansion methods on plug and crushed-rock samples. Mar Pet Geol 73:299–310

    Google Scholar 

  • Ren Y, Guo X, Xie C, Wu H (2016) Experimental study on gas slippage of Marine Shale in Southern China. Petroleum 2:171–176. https://doi.org/10.1016/j.petlm.2016.03.003

    Article  Google Scholar 

  • Sander R, Pan Z, Connell LD (2017) Laboratory measurement of low permeability unconventional gas reservoir rocks: a review of experimental methods. J Nat Gas Sci Eng 37:248–279. https://doi.org/10.1016/j.jngse.2016.11.041

    Article  Google Scholar 

  • Sang G, Elsworth D, Miao X, Mao X, Wang J (2016) Numerical study of a stress dependent triple porosity model for shale gas reservoirs accommodating gas diffusion in kerogen. J Nat Gas Sci Eng 32:423–438

    Google Scholar 

  • Sang G, Elsworth D, Liu S, Harpalani S (2017) Characterization of swelling modulus and effective stress coefficient accommodating sorption-induced swelling in coal. Energy Fuels 31:8843–8851

    Google Scholar 

  • Shen Y, Pang Y, Shen Z, Tian Y, Ge H (2018) Multiparameter analysis of gas transport phenomena in shale gas reservoirs: apparent permeability characterization. Sci Rep 8:2601. https://doi.org/10.1038/s41598-018-20949-2

    Article  Google Scholar 

  • Shi R, et al. (2020) Experimental observations of heterogeneous strains inside a dual porosity sample under the influence of gas-sorption: a case study of fractured coal. Int J Coal Geol:103450

  • Shi R, Liu J, Wei M, Elsworth D, Wang X (2018) Mechanistic analysis of coal permeability evolution data under stress-controlled conditions. Int J Rock Mech Min Sci 110:36–47. https://doi.org/10.1016/j.ijrmms.2018.07.003

    Article  Google Scholar 

  • Tan Y, Pan Z, Liu J, Wu Y, Haque A, Connell LD (2017) Experimental study of permeability and its anisotropy for shale fracture supported with proppant. J Nat Gas Sci Eng 44:250–264

    Google Scholar 

  • Tan Y, Pan Z, Liu J, Feng X-T, Connell LD (2018) Laboratory study of proppant on shale fracture permeability and compressibility. Fuel 222:83–97

    Google Scholar 

  • Tan Y, Pan Z, Feng X-T, Zhang D, Connell LD, Li S (2019) Laboratory characterisation of fracture compressibility for coal and shale gas reservoir rocks: a review. Int J Coal Geol 204:1–17

    Google Scholar 

  • van Noort R, Yarushina V (2019) Water, CO2 and argon permeabilities of intact and fractured shale cores under stress. Rock Mech Rock Eng 52:299–319

    Google Scholar 

  • Wang Q, Chen X, Jha AN, Rogers H (2014) Natural gas from shale formation–the evolution, evidences and challenges of shale gas revolution in United States. Renew Sustain Energy Rev 30:1–28

    Google Scholar 

  • Wang C, Liu J, Feng J, Wei M, Wang C, Jiang Y (2016) Effects of gas diffusion from fractures to coal matrix on the evolution of coal strains: Experimental observations. Int J Coal Geol 162:74–84

    Google Scholar 

  • Wang X, Zhu Y, Fu C (2019) Experimental investigation of the stress-dependent permeability in the Longmaxi Formation shale. J Pet Sci Eng 175:932–947

    Google Scholar 

  • Washburn EW (1921) The dynamics of capillary flow. Phys Rev 17:273

    Google Scholar 

  • Wei M, Liu J, Feng X, Wang C, Zhou F (2016) Evolution of shale apparent permeability from stress-controlled to displacement-controlled conditions. J Nat Gas Sci Eng 34:1453–1460. https://doi.org/10.1016/j.jngse.2016.07.012

    Article  Google Scholar 

  • Wei M, Liu Y, Liu J, Elsworth D, Zhou F (2019) Micro-scale investigation on coupling of gas diffusion and mechanical deformation of shale. J Pet Sci Eng 175:961–970

    Google Scholar 

  • Wei M, Liu J, Elsworth D, Li S, Zhou F (2019) Influence of gas adsorption induced non-uniform deformation on the evolution of coal permeability. Int J Rock Mech Min Sci 114:71–78

    Google Scholar 

  • Wei M, Liu J, Elsworth D, Liu Y, Zeng J, He Z (2021) Impact of equilibration time lag between matrix and fractures on the evolution of coal permeability. Fuel 290:120029

    Google Scholar 

  • Werner AK, Vink S, Watt K, Jagals P (2015) Environmental health impacts of unconventional natural gas development: a review of the current strength of evidence. Sci Total Environ 505:1127–1141

    Google Scholar 

  • Wildenschild D, Sheppard AP (2013) X-ray imaging and analysis techniques for quantifying pore-scale structure and processes in subsurface porous medium systems. Adv Water Resour 51:217–246

    Google Scholar 

  • Wu Y, Liu J, Elsworth D, Chen Z, Connell L, Pan Z (2010) Dual poroelastic response of a coal seam to CO2 injection. Int J Greenh Gas Control 4:668–678

    Google Scholar 

  • Wu Y, Liu J, Chen Z, Elsworth D, Pone D (2011) A dual poroelastic model for CO2-enhanced coalbed methane recovery. Int J Coal Geol 86:177–189

    Google Scholar 

  • Yang Y, Liu S (2019) Estimation and modeling of pressure-dependent gas diffusion coefficient for coal: a fractal theory-based approach. Fuel 253:588–606

    Google Scholar 

  • Zamirian M, Aminian KK, Ameri S, Fathi E (2014a) New steady-state technique for measuring shale core plug permeability. In: SPE/CSUR Unconventional Resources Conference–Canada, Calgary, Alberta, Canada, pp 1–11. https://doi.org/10.2118/171613-MS

  • Zamirian M, Aminian KK, Ameri S, Fathi E (2014b) New steady-state technique for measuring shale core plug permeability. In: SPE/CSUR unconventional resources conference–canada, Society of Petroleum Engineers

  • Zeng J, Liu J, Li W, Leong Y-K, Elsworth D, Guo J (2020) Evolution of shale permeability under the influence of gas diffusion from the fracture wall into the matrix. Energy Fuels 34:4393–4406

    Google Scholar 

  • Zhang H, Liu J, Elsworth D (2008) How sorption-induced matrix deformation affects gas flow in coal seams: a new FE model. Int J Rock Mech Min Sci 45:1226–1236

    Google Scholar 

  • Zhao Y, Wang C, Zhang Y, Liu Q (2019) Experimental study of adsorption effects on shale permeability. Nat Resour Res 28:1575–1586

    Google Scholar 

  • Zhou J, Liu G, Jiang Y, Xian X, Liu Q, Zhang D, Tan J (2016) Supercritical carbon dioxide fracturing in shale and the coupled effects on the permeability of fractured shale: an experimental study. J Nat Gas Sci Eng 36:369–377. https://doi.org/10.1016/j.jngse.2016.10.005

    Article  Google Scholar 

  • Zhou J, Zhang L, Li X, Pan Z (2019) Experimental and modeling study of the stress-dependent permeability of a single fracture in shale under high effective stress. Fuel 257:116078

    Google Scholar 

  • Zhou J et al (2020) Experimental investigation on the influence of sub-and super-critical CO2 saturation time on the permeability of fractured shale. Energy 191:116574

    Google Scholar 

  • Zhu W, Tian W, Gao Y, Deng J, Zhang X, Qi Q, Ma Q (2016) Study on experiment conditions of marine shale gas seepage law. J Nat Gas Geosci 1:157–163. https://doi.org/10.1016/j.jnggs.2016.05.006

    Article  Google Scholar 

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Acknowledgements

This work was funded by the Natural Science Foundation of China (41972184), the Fund of Outstanding Talents in Discipline of China University of Geosciences (Wuhan) (102-162301192664), the Natural Science Foundation of Hebei Province (E2020209074), and the Fundamental Research Funds for National Universities, China University of Geosciences (Wuhan). These supports are gratefully acknowledged.

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Correspondence to Xiaoming Wang.

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Research Highlights

A dense array of strain gauges is used to constrain the complex evolution of strain in shales containing a fracture. Complex transient and non-uniform strains develop as a result of even uniform confining stress. These strain gradients suggest a heterogeneous evolution of fracture permeability that can be rationalized from the mechanics of deformation.

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Shi, R., Liu, J., Wang, X. et al. Experimental Observations of Gas-sorption-Induced Strain Gradients and their Implications on Permeability Evolution of Shale. Rock Mech Rock Eng 54, 3927–3943 (2021). https://doi.org/10.1007/s00603-021-02473-4

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