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Magnetic Ti3C2Tx/Fe3O4/Aramid nanofibers composite paper with tunable electromagnetic interference shielding performance

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Abstract

Increasingly popularity of electronic devices and wireless apparatus requires advanced materials to cope with severe electromagnetic wave pollution. Herein, magnetic EM wave shielding material, Ti3C2Tx/Fe3O4/aramid nanofibers composite paper, composed of low-dimensional Ti3C2Tx flakes and carboxylation Fe3O4 nanoparticles, was developed via vacuum-assisted filtration. At the meanwhile, uniform dispersion of components was achieved to overcome magnetic through ingenious electrostatic force regulation originated from negative functional groups. The Ti3C2Tx/Fe3O4/aramid nanofibers composite paper exhibited suitable magnetic performance, outstanding electrical conductivity, and excellent electromagnetic interference shielding performance. Moreover, the Ti3C2Tx/Fe3O4/aramid nanofibers composite paper demonstrated favorable mechanical properties, whose tensile strength and Young’s modulus reached 132.2 ± 2.1 MPa and 5.23 ± 0.14 GPa, respectively. The combination of electromagnetic shielding capacity (derived from Ti3C2Tx flakes, carboxylation Fe3O4 nanoparticles) and mechanical properties (derived from aramid nanofibers) provided feasible strategy in fabricating advanced EMI shielding composite with astonishing comprehensive performance.

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Acknowledgements

The authors acknowledge 302 colleagues for their assistance during the research. The authors appreciate for the financial support from National Natural Science Foundation of China (Grant No. 51803110), National Key Research and Development Plan (2017YFB0308300, 2017YFB0308302), Zhejiang Province key research and development project (2019C04008). Shaanxi Natural Science Basic Research Program (2020JQ-724) and the Opening Foundation of Key Laboratory of Auxiliary Chemistry and Technology for Chemical Industry (KFKT2020-07) sincerely. Finally, FJ thanks the inimitable support of QW in the toughest times.

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Authors and Affiliations

  1. Shaanxi Provincial Key Laboratory of Papermaking Technology and Specialty Paper Development, Key Laboratory of Paper Based Functional Materials of China National Light Industry, National Demonstration Center for Experimental Light Chemistry Engineering Education, College of Bioresources Chemical and Materials Engineering, Shaanxi University of Science and Technology, No. 6, Xuefu Road, Xi’an, 710021, People’s Republic of China

    Fengfeng Jia, Fan Xie, Shanshan Chen, Danni Wang, Zhanfan Jin, Longhai Zhuo & Zhaoqing Lu

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  1. Fengfeng Jia
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Contributions

FJ contributed to conceptualization, methodology, software, formal analysis, and writing-original draft. FX was involved in validation, formal analysis, data curation, and funding acquisition. SC contributed to investigation, validation. DW was involved in investigation. ZJ contributed to software. LZ was involved in supervision and funding acquisition, and ZL contributed to validation, supervision and funding acquisition.

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Correspondence to Zhaoqing Lu.

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Jia, F., Xie, F., Chen, S. et al. Magnetic Ti3C2Tx/Fe3O4/Aramid nanofibers composite paper with tunable electromagnetic interference shielding performance. Appl. Phys. A 127, 175 (2021). https://doi.org/10.1007/s00339-021-04295-1

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