Abstract
The Cahn–Hilliard equation is a common model to describe phase separation processes of a mixture of two components. We study the Cahn–Hilliard equation coupled with the homogeneous strong anchoring condition (i.e., homogeneous Dirichlet condition) on the relative concentration u of the two phases. Moreover, we adopt no-flux boundary condition to keep conservation of mass. With a specific quartic form of the double-well potential, we prove the existence and uniqueness of the weak solution to this model by interpreting the problem as a gradient flow of the Cahn–Hilliard free energy. Utilizing the minimizing movement scheme and time discretization method, we show that the approximation solutions converge to the weak solution of the Cahn–Hilliard equation. Finally, we prove that the weak solution satisfies an energy dissipation inequality.
Similar content being viewed by others
Data Availability
All data generated or analysed during this study are included in this published article.
References
Alessio, F., Wilfrid, G., Türkay, Y.: A variational method for a class of parabolic PDEs. Annali della Scuola Normale Superiore di Pisa - Classe di Scienze 5(10), 207–252 (2011)
Ambrosio, L., Gigli, N., Savaré, G.: Gradient flows in metric spaces and the Wasserstein spaces of probability measures. Lectures in Mathematics, ETH Zürich, Birkhäuser (2005)
Arendt, W., Chalendar, I., Eymard, R.: Galerkin approximation of linear problems in Banach and Hilbert spaces. IMA Journal of Numerical Analysis, Oxford University Press (OUP), (2020). arXiv:0226.4895v3f [hal]
Baňas, L., Nürnberg, R.: Adaptive finite element methods for Cahn-Hilliard equations. J. Comput. Applied Math. 218(1), 2–11 (2008)
Baňas, L., Nürnberg, R.: A posteriori estimates for the Cahn-Hilliard equation with obstacle free energy. ESAIM: Math. Modelling Numer. Anal. 43(5), 1003–1026 (2009)
Badalassi, V.E., Ceniceros, H.D., Banerjee, S.: Computation of multiphase systems with phase field models. J. Comput. Phys. 190(2), 371–397 (2003)
Bates, P., Han, J.: The Dirichlet boundary problem for a nonlocal Cahn-Hilliard equation. J. Math. Anal. Appl. 311(1), 289–312 (2005)
Beard, R.W., Saridis, G.N., Wen, J.T.: Galerkin approximations of the generalized Hamilton-Jacobi-Bellman equation. Automatica 33(12), 2159–2177 (1997)
Bertozzi, A.L., Esedoglu, S., Gillette, A.: Inpainting of binary images using the Cahn-Hilliard equation. IEEE Trans. Image Process. 16(1), 285–291 (2007)
Bronsard, L., Hilhorst, D.: On the slow dynamics for the Cahn-Hilliard equation in one space dimension. Proc. Royal Soc. A 439(1907), 669–682 (1992)
Cahn, J.W., Elliott, C.M., Novick-Cohen, A.: The Cahn-Hilliard equation with a concentration-dependent mobility: Motion by minus the Laplacian of the mean curvature. European J. Appl. Math. 7, 287–301 (1996)
Cahn, J.W., Hilliard, J.E.: Free energy of a nonuniform system. I. Interfacial free energy. J. Chem. Phys. 28, 258–267 (1958)
Cahn, J.W., Hilliard, J.E.: Free energy of a nonuniform system. II. Thermodynamic basis. J. Chem. Phys. 30, 1121–1135 (1959)
Ceniceros, H.D., Roma, A.M.: A nonstiff, adaptive mesh refinement-based method for the Cahn-Hilliard equation. J. Comput. Phys. 225(2), 1849–1862 (2007)
Choksi, R., Peletier, M.A., Williams, J.F.: On the phase diagram for microphase separation of diblock copolymers: An approach via a nonlocal Cahn-Hilliard functional. SIAM J. Applied Math. 69(6), 1712–1738 (2009)
Choksi, R., Sternberg, P.: Periodic phase separation: the periodic Cahn–Hilliard and isoperimetric problems. Interfaces Free Bound. 8(3), 371–392 (2006)
Cohen, D., Murray, J.M.: A generalized diffusion model for growth and dispersion in a population. J. Math. Biol. 12, 237–248 (1981)
Dai, S., Du, Q.: Coarsening mechanism for systems governed by the Cahn–Hilliard equation with degenerate diffusion mobility. Multiscale Model. Simul. 12(4), 1870–1889 (2014)
Dai, S., Du, Q.: Weak solutions for the Cahn–Hilliard equation with degenerate mobility. Arch. Ration. Mech. Anal. 219(3), 1161–1184 (2016)
Dai, S., Du, Q.: Weak solutions for the Cahn–Hilliard equation with phase-dependent diffusion mobility. Arch. Ration. Mech. Anal. 219(3), 1161–1184 (2016)
Dai, S., Li, B., Luong, T.: Minimizers for the Cahn–Hilliard energy under strong anchoring conditions. SIAM J. Appl. Math. 80(5), 2299–2317 (2020)
Dai, S., Liu, Q., Luong, T., Promislow, K.: On nonnegative solutions for the functionalized Cahn–Hilliard equation with degenerate mobility. Results Appl. Math. 12, 100195 (2021)
Dai, S., Liu, Q., Promislow, K.: Weak solutions for the Functionalized Cahn–Hilliard equation with degenerate mobility. Appl. Anal. (2019). https://doi.org/10.1080/00036811.2019.1585536
DeGroot, S.R., Mazur, P.: Non-Equilibrium Thermodynamics. Dover Publications Inc., Mineola, N. Y. (1984)
Dehghan, M.: Finite difference procedures for solving a problem arising in modeling and design of certain optoelectronic devices. Math. Comput. Simul. 71, 16–30 (2006)
Dehghan, M., Mohebbi, A.: Multigrid solution of high order discretisation for three-dimensional biharmonic equation with Dirichlet boundary conditions of second kind. Appl. Math. Comput. 180, 575–593 (2006)
Du, Q., Nicolaides, R.: Numerical analysis of a continuum model of phase transition. SIAM J. Numer. Anal. 28(5), 1310–1322 (1991)
Elliott, C., Garcke, H.: On the Cahn–Hilliard equation with degenerate mobility. SIAM J. Math. Anal. 27(2), 404–423 (1996)
Elliott, C., Garcke, H.: On the Cahn–Hilliard equation with degenerate mobility. SIAM J. Math. Anal. 27(2), 404–423 (1996)
Evans, L.C.: Partial Differential Equations, 2nd edn. Amer. Math. Soc., Providence (2010)
Feng, W.M., Yu, P., Hu, S.Y., Liu, Z.K., Du, Q., Chen, L.Q.: Spectral implementation of an adaptive moving mesh method for phase-field equations. J. Comput. Phys. 220(1), 498–510 (2006)
Fleißner, F.C.: A minimizing movement approach to a class of scalar reaction-diffusion equations. ESAIM Control Optim. Calc. Var. 27(18) (2021)
Garcke, H., Lam, K.F.: Analysis of a Cahn–Hilliard system with non-zero Dirichlet conditions modeling tumor growth with chemotaxis. Disc. Cont. Dyn. Syst. 37(8), 4277–4308 (2017)
Garcke, H., Nestler, B., Stoth, B.: A multiphase field concept: numerical simulations of moving phase boundaries and multiple junctions. SIAM J. Appl. Math. 60(1), 295–315 (1999)
De Giorgi, E.: New Problems on Minimizing Movements. In: Boundary Value Problems for PDEs and Applications, pp. 81–98. Masson (1993)
De Giorgi, E., Mariono, A., Tosques, M.: Problems of evolution in metric spaces and maximal decreasing curve. Atti. Accad. Naz. Lincei Rend. Cl. Sci. Mat. Natur. 68(8), 180–187 (1980)
Gómez, H., Calo, V., Bazilevs, Y., Hughes, T.: Isogeometric analysis of the Cahn–Hilliard phase-field model. Comput. Meth. Appl. Mech. Eng. 197(49–50), 4333–4352 (2008)
He, L.: Error estimation of a class of stable spectral approximation to the Cahn–Hilliard equation. J. Sci. Comput. 41(3), 461–482 (2009)
He, Y., Liu, Y., Tang, T.: On large time-stepping methods for the Cahn–Hilliard equation. Appl. Numer. Math. 57(5–7), 616–628 (2007)
Klapper, I., Dockery, J.: Role of cohesion in the material description of biofilms. Phys. Rev. E 74, 0319021–0319028 (2006)
Ladyzhenskaya, O.A.: Global solvability of a boundary value roblem for the Navier–Stokes equations in the case of two spatial variables. Doklady USSR 123, 427–429 (1958)
Lamorgese, A.G., Mauri, R.: Diffuse-interface modeling of phase segregation in liquid mixtures. Intern. J. Multiphase Flow 34(10), 987–995 (2008)
Li, M., Ober, C.K.: Block copolymer patterns and templates. Mater. Today 9(9), 30–39 (2006)
Li, Y., Jeong, D., Shin, J., Kim, J.: A conservative numerical method for the Cahn-Hilliard equation with Dirichlet boundary conditions in complex domains. Comput. Math. Appl. 65(1), 102–115 (2013)
Lions, J.L., Magenes, E.: Non-Homogeneous Boundary Value Problems and Applications, vol. I. Springer, Berlin (1972)
Lisini, S.: Nonlinear diffusion equations with variable coefficients as gradient flows in Wasserstein spaces. ESAIM Control Optim. Calc. Var. 15(3), 712–740 (2008)
Liu, Y., Liu, W.K.: Rheology of red blood cell aggregation by computer simulation. J. Comput. Phys. 220, 139–154 (2006)
Moelans, N., Blanpain, B., Wollants, P.: An introduction to phase-field modeling of microstructure evolution. Comput. Coupling Phase Diagr. Thermochem. 32, 268–294 (2008)
Oron, A., Davis, S.H., Bankoff, S.G.: Long-scale evolution of thin liquid films. Rev. Mod. Phys. 69, 931–980 (1997)
Pego, R.L.: Front migration in the nonlinear Cahn–Hilliard equation. Proc. Royal Soc. Lond. A 442, 261–278 (1989)
Rossi, R., Savaré, G.: Gradient flows of non convex functionals in hilbert spaces and applications. ESAIM Control Optim. Calc. Var. 12(3), 564–614 (2006)
Tremaine, S.: On the origin of irregular structure in Saturn’s rings. Astron. J. 125, 894 (2003)
Santambrogio, F.: Euclidean, metric, and Wasserstein gradient flows: an overview. Bull. Math. Sci. 7, 87–154 (2017)
Saxena, R., Caneba, G.T.: Studies of spinodal decomposition in a ternary polymer-solvent-nonsolvent systems. Polym. Eng. Sci. 42, 1019–1031 (2002)
Simon, J.: Compact sets in the space \(L^p(0, T; B)\). Ann. Mat. 146, 65–96 (1986)
Stefanelli, U.: A new minimizing-movements scheme for curves of maximal slope. arXiv:2103.00846. March (2021)
Thiele, U., Knobloch, E.: Thin liquid films on a slightly inclined heated plate. Physica D 190, 213–248 (2004)
Wells, G.N., Kuhl, E., Garikipati, K.: A discontinuous Galerkin method for the Cahn–Hilliard equation. J. Comput. Phys. 218(2), 860–877 (2006)
Wheeler, B., Hammadi, R., Ma, X.: Self-assembled 3d nanoporous biomimetic material embedded with green synthesized gold nanoparticles for high-performance non-enzymatic glucose sensor (submitted)
Wise, S., Lowengrub, J., Frieboes, H., Cristini, V.: Three-dimensional multispecies nonlinear tumor growth-I: model and numerical method. J. Theor. Biol. 253, 524–543 (2008)
Yang, W., Huang, Z., Zhu, W.: Image segmentation using the Cahn–Hilliard equation. J. Sci. Comput. 79, 1057–1077 (2019)
Ye, X.: The Fourier collocation method for the Cahn–Hilliard equation. Comput. Math. Appl. 44(1–2), 213–229 (2002)
Zhou, B., Powell, A.: Phase field simulation of early stage structure formation during immersion precipitation of polymeric membranes in 2D and 3D. J. Membr. Sci. 268, 150–164 (2006)
Zhu, Y., Aissou, K., Andelman, D., Man, X.: Orienting cylinder-forming block copolymer thin films: The combined effect of substrate corrugation and its surface energy. Macromolecules 52(3), 1241–1248 (2019)
Zinsl, J., Matthes, D.: Discrete approximation of the minimizing movement scheme for evolution equations of Wasserstein gradient flow type with nonlinear mobility. arXiv:1609.06907, September (2016)
Funding
The work of the first author was partially supported by the U.S. National Science Foundation through Grant DMS-1815746.
Author information
Authors and Affiliations
Contributions
Both authors contribute equally to this work.
Corresponding author
Ethics declarations
Conflict of interest
The authors have no relevant financial or non-financial interests to disclose.
Additional information
Publisher's Note
Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
Appendix: Ladyzhenskaya’s inequality
Appendix: Ladyzhenskaya’s inequality
The Ladyzhenskaya’s inequality was introduced by O. A. Ladyzhenskaya [41] to prove the existence and uniqueness of long-time solutions to the Navier–Stokes equations in \({\mathbb {R}}^2\) when the initial data is sufficiently smooth. This inequality is a member of a class of inqualities known as interpolation inequalities.
Lemma 4.3
(Ladyzhenskaya’s inequality) Let \(\Omega \) be a Lipschitz domain in \({\mathbb {R}}^d\) (\(d=2\) or 3) and \(f \in H_0^1(\Omega )\). Then there exists a constant \(C > 0\) depending only on \(\Omega \) such that
Rights and permissions
Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.
About this article
Cite this article
Dai, S., Luong, T. On the Cahn–Hilliard equation with no-flux and strong anchoring conditions. Nonlinear Differ. Equ. Appl. 30, 49 (2023). https://doi.org/10.1007/s00030-023-00854-y
Received:
Accepted:
Published:
DOI: https://doi.org/10.1007/s00030-023-00854-y