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Hybrid-Organic Photonic Structures for Light Emission Modification

  • Chapter
Organic and Hybrid Photonic Crystals

Abstract

We report the modification of the photoluminescence (PL) and decay rates of two different green-emitting conjugated polymers incorporated into photonic crystals with the stop-bands spectrally tuned on their emission. We observe both suppression (in the stop-band) and enhancement (at the high-energy band-edge) of the photoluminescence. Time-resolved measurements also reveal a concomitant modification of the emission lifetime that is enhanced at the band-edge and suppressed within the stop-band, thus confirming a variation of the radiative decay rate of the excitations in such photonic nanostructures. We propose two examples of fluorescent photonic composite systems. The first consists of a hybrid Si-organic system, obtained by infiltration of the polymer inside a rugate filter (a 1D photonic crystal). The second example is a fully organic system obtained by self-assembling of solvent-compatible microspheres-polymer system for obtaining a synthetic opal (a 3D photonic crystal) with a uniform distribution of the emitting material across the photonic structure.

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Authors and Affiliations

  1. Department of Physics and Astronomy and London Centre for Nanotechnology, University College London, Gower Street, WC1E 6BT, London, UK

    Valentina Robbiano & Franco Cacialli

  2. Nanochemistry Department, Istituto Italiano di Tecnologia, Via Morego 30, 16163, Genoa, Italy

    Francesco Di Stasio

  3. Dipartimento di Ingegneria dell’Informazione, Università di Pisa, Via Diotisalvi 2, 56122, Pisa, Italy

    Salvatore Surdo & Giuseppe Barillaro

  4. Department of Physics, McDaniel College, Westminster, MD, 21157, USA

    Shabbir Mian

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  1. Valentina Robbiano
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  2. Francesco Di Stasio
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Correspondence to Franco Cacialli .

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  1. Department of Chemistry and Industrial Chemistry, University of Genova, Genova, Italy

    Davide Comoretto

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Robbiano, V., Di Stasio, F., Surdo, S., Mian, S., Barillaro, G., Cacialli, F. (2015). Hybrid-Organic Photonic Structures for Light Emission Modification. In: Comoretto, D. (eds) Organic and Hybrid Photonic Crystals. Springer, Cham. https://doi.org/10.1007/978-3-319-16580-6_15

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