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Photoactive Molecules within MOFs

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Dyes and Photoactive Molecules in Microporous Systems

Part of the book series: Structure and Bonding ((STRUCTURE,volume 183))

Abstract

Photochromic molecules have been considered to be applied in responsive functional materials. Recently, the combination of a porous host matrix and these photoactive species has become an emerging field of research. Especially the use of crystalline nanoporous metal-organic frameworks (MOFs) as host materials has proven to be very promising. The combination of crystallinity and the ability to be systematically functionalized is one of the main advantages of these porous host materials. The resulting switch@MOF hybrid systems exhibit fascinating and even surprising properties ranging from the “simple” possibility of solid-state switching to remote control gas uptake and conductance photoswitching. After a short introduction to photochromism, solvatochromism, and MOFs, this chapter discusses the formation and the developments of these switch@MOF materials and the recent advances in exploitation of the light-induced structural changes.

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Abbreviations

AZB:

Azobenzene

BET:

Brunauer-Emmett-Teller

BSP:

1-(2-hydroxy-ethyl)-3,3-dimethyl-indolino-6′-nitrobenzospiropyran

c :

Closed

COF:

Covalent-organic framework

CT:

Charge-transfer

d:

Day(s)

DAE:

Diarylethenes

DC:

Direct current

DFT:

Density functional theory

DMF:

N,N′-dimethylformamide

DSC:

Difference scanning calorimetry

DTE:

Dithienylethenes

EDS/EDX:

Energy dispersive X-ray spectroscopy

EDTM:

Electric dipole transition moment

EtOH:

Ethanol

ext:

Extinction

h:

Hour(s)

HKUST:

Hong Kong University of Science and Technology

IR:

Infrared

IR-MOF:

Isoreticular MOF

IRRA:

Infrared reflection-absorption

irrad:

Irradiated

JUC:

Jilin University China

LED:

Light-emitting diode

LPE:

Liquid phase epitaxial growth

max:

Maximum

MC:

Merocyanine

MeOH:

Methanol

MIL:

Matériaux de l’Institut Lavoisier

min:

Minute or minimal

MOF:

Metal-organic framework

nm:

Nanometer

NMR:

Nuclear magnetic resonance

o :

Open

oF :

4H, 4H’-octafluoro

PAP:

2-phenylazopyridine

PCN:

Porous coordination network

PCP:

Porous coordination polymer

PDF:

Pair distribution function

PEG:

Poly(ethylene glycol)

pF :

Perfluoro

PIZOF:

Porous interpenetrated zirconium-organic frameworks

PM:

Porous material

PSS:

Photostationary state

QCM:

Quartz crystal microbalance

SBU:

Secondary building unit

SEM:

Scanning electron microscopy

SP:

Spiropyran

SP-Nitro:

1,3,3-trimethyl-indolino-6′-nitrobenzo-pyrylospiran

SP-O:

1,3,3-trimethyl-indolino-naphtho-spirooxazine

SURMOF:

Surface-mounted MOF

tF :

Ortho-tetrafluoro

TGA:

Thermogravimetric analysis

ToF-SIMS:

Time-of-flight secondary ion mass spectrometry

UHPLC:

Ultra-high-performance liquid chromatography

UiO:

Universitetet i Oslo

UV:

Ultra-violet

vis:

Visible (light)

XPS:

X-ray photoelectron spectroscopy

XR(P)D:

X-ray (powder) diffraction

ε0:

Elution power

λ:

Wavelength

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Author information

Authors and Affiliations

  1. Institute of General, Inorganic and Theoretical Chemistry, University of Innsbruck, Innsbruck, Austria

    Heidi Annemarie Schwartz

  2. Department of Chemistry, University of Cologne, Cologne, Germany

    Uwe Ruschewitz

Authors
  1. Heidi Annemarie Schwartz
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  2. Uwe Ruschewitz
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Correspondence to Uwe Ruschewitz .

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Editors and Affiliations

  1. Department of Physical Chemistry, University of the Basque Country UPV/EHU, Bilbao, Vizcaya, Spain

    Virginia Martínez-Martínez

  2. Department of Physical Chemistry, University of the Basque Country UPV/EHU, Bilbao, Vizcaya, Spain

    Fernando López Arbeloa

Appendix

Appendix

This book chapter was completed in October 2019 and covers almost all the literature available at that time. As MOFs as hosts for photoactive molecules are a very fast developing field of research, it was not possible to include the many interesting papers published after this deadline.

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Schwartz, H.A., Ruschewitz, U. (2020). Photoactive Molecules within MOFs. In: Martínez-Martínez, V., López Arbeloa, F. (eds) Dyes and Photoactive Molecules in Microporous Systems. Structure and Bonding, vol 183. Springer, Cham. https://doi.org/10.1007/430_2020_56

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