Abstract
We demonstrate quantum entanglement between a single hole spin confined to a positively charged semiconductor quantum dot (QD) and a photon spontaneously emitted from the matter’s excited state. The QD system is in the Voigt geometry with two ground hole spin states and two excited trion states. We consider the light-matter coupling initially prepared in one of the ground hole spin states. For very weak Rabi frequencies, the spin-flip process transfers most of the population to another hole spin state, leading to the disentanglement between the single photon and single QD hole spin. A maximum entanglement is achieved by increasing the intensity of Rabi frequencies. In this case, the population almost equally distributes among all the bare quantum states. Our results may pave the way toward creating a scalable QD quantum computing architecture relying on the photon as flying qubits to mediate entanglement between distant nodes of a QD network.
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Data Availability Statement
This manuscript has associated data in a data repository. [Authors’ comment: The datasets generated during and/or analyzed during the current study are available from the corresponding author on reasonable request.]
References
C.H. Bennett, G. Brassard, C. Crépeau, R. Jozsa, A. Peres, W.K. Wootters, Teleporting an unknown quantum state via dual classical and Einstein–Podolsky–Rosen channels. Phys. Rev. Lett. 70, 1895 (1993)
A.K. Ekert, Quantum cryptography based on Bell’s theorem. Phys. Rev. Lett. 67, 661 (1991)
J. Yin, Y.-H. Li, S.-K. Liao, M. Yang, Y. Cao, L. Zhang, J.-G. Ren, W.-Q. Cai, W.-Y. Liu, S.-L. Li, R. Shu, Y.-M. Huang, L. Deng, L. Li, Q. Zhang, N.-L. Liu, Y.-A. Chen, C.-Y. Lu, X.-B. Wang, F. Xu, J.-Y. Wang, C.-Z. Peng, A.K. Ekert, J.-W. Pan, Entanglement-based secure quantum cryptography over 1,120 kilometres. Nature 582, 501 (2020)
J.P. Dowling, K.P. Seshadreesan, Quantum optical technologies for metrology, sensing, and imaging. J. Lightwave Technol. 33, 2359 (2015)
R. Jozsa, N. Linden, On the role of entanglement in quantum-computational speed-up. Proc. R. Soc. Lond. Ser. A Math. Phys. Eng. Sci. 459, 211 (2003)
T.D. Ladd, F. Jelezko, R. Laflamme, Y. Nakamura, C. Monroe, J.L. O’Brien, Quantum computers. Nature 464, 45 (2010)
C. Kloeffel, D. Loss, Prospects for spin-based quantum computing in quantum dots. Annu. Rev. Condens. Matter Phys. 4, 51 (2013)
R. Blatt, D. Wineland, Entangled states of trapped atomic ions. Nature 453, 1008 (2008)
J.J. García-Ripoll, P. Zoller, J.I. Cirac, Quantum information processing with cold atoms and trapped ions. J. Phys. B At. Mol. Opt. Phys. 38, S567 (2005)
R. Barends, J. Kelly, A. Megrant, A. Veitia, D. Sank, E. Jeffrey, T.C. White, J. Mutus, A.G. Fowler, B. Campbell, Y. Chen, Z. Chen, B. Chiaro, A. Dunsworth, C. Neill, P. O’Malley, P. Roushan, A. Vainsencher, J. Wenner, A.N. Korotkov, A.N. Cleland, J.M. Martinis, Superconducting quantum circuits at the surface code threshold for fault tolerance. Nature 508, 500 (2014)
N. Roch, M.E. Schwartz, F. Motzoi, C. Macklin, R. Vijay, A.W. Eddins, A.N. Korotkov, K.B. Whaley, M. Sarovar, I. Siddiqi, Observation of measurement-induced entanglement and quantum trajectories of remote superconducting qubits. Phys. Rev. Lett. 112, 170501 (2014)
K.C. Lee, M.R. Sprague, B.J. Sussman, J. Nunn, N.K. Langford, X.-M. Jin, T. Champion, P. Michelberger, K.F. Reim, D. England, D. Jaksch, I.A. Walmsley, Entangling macroscopic diamonds at room temperature. Science (80-) 334, 1253 (2011)
W.B. Gao, A. Imamoglu, H. Bernien, R. Hanson, Coherent manipulation, measurement and entanglement of individual solid-state spins using optical fields. Nat. Photonics 9, 363 (2015)
A. Imamog, D. Awschalom, G. Burkard, D.P. DiVincenzo, D. Loss, M. Sherwin, A. Small, Quantum information processing using quantum dot spins and cavity QED. Phys. Rev. Lett. 83, 4204 (1999)
W. Yao, R.B. Liu, L.J. Sham, Theory of control of the spin-photon interface for quantum networks. Phys. Rev. Lett. 95, 1 (2005)
E. Togan, Y. Chu, A.S. Trifonov, L. Jiang, J. Maze, L. Childress, M.V.G. Dutt, A.S. Sørensen, P.R. Hemmer, A.S. Zibrov, M.D. Lukin, Quantum entanglement between an optical photon and a solid-state spin qubit. Nature 466, 730 (2010)
J.R. Schaibley, A.P. Burgers, G.A. McCracken, L.M. Duan, P.R. Berman, D.G. Steel, A.S. Bracker, D. Gammon, L.J. Sham, Demonstration of quantum entanglement between a single electron spin confined to an InAs quantum dot and a photon. Phys. Rev. Lett. 110, 1 (2013)
K. De Greve, L. Yu, P.L. McMahon, J.S. Pelc, C.M. Natarajan, N.Y. Kim, E. Abe, S. Maier, C. Schneider, M. Kamp, S. Höfling, R.H. Hadfield, A. Forchel, M.M. Fejer, Y. Yamamoto, Quantum-dot spin-photon entanglement via frequency downconversion to telecom wavelength. Nature 491, 421 (2012)
S. Sun, E. Waks, Deterministic generation of entanglement between a quantum-dot spin and a photon. Phys. Rev. A 90, 42322 (2014)
D. Loss, D.P. Divincenzo, Quantum computation with quantum dots. Phys. Rev. A 57, 120 (1998)
M. Atatüre, J. Dreiser, A. Badolato, A. Högele, K. Karrai, A. Imamoglu, Quantum-dot spin-state preparation with near-unity fidelity. Science (80-) 312, 551 (2006)
W.A. Coish, D. Loss, Hyperfine interaction in a quantum dot: non-markovian electron spin dynamics. Phys. Rev. B 70, 195340 (2004)
W. Yao, R.-B. Liu, L.J. Sham, Theory of electron spin decoherence by interacting nuclear spins in a quantum dot. Phys. Rev. B 74, 195301 (2006)
R.J. Warburton, Single spins in self-assembled quantum dots. Nat. Mater. 12, 483 (2013)
A. Tartakovskii, Holes avoid decoherence. Nat. Photonics 5, 647 (2011)
D. Brunner, B.D. Gerardot, P.A. Dalgarno, G. Wüst, K. Karrai, N.G. Stoltz, P.M. Petroff, R.J. Warburton, A coherent single-hole spin in a semiconductor. Science (80-.) 325, 70 (2009)
J. Fischer, W.A. Coish, D.V. Bulaev, D. Loss, Spin decoherence of a heavy hole coupled to nuclear spins in a quantum dot. Phys. Rev. B Condens. Matter Mater. Phys. 78, 1 (2008)
C. Testelin, F. Bernardot, B. Eble, M. Chamarro, Hole-spin dephasing time associated with hyperfine interaction in quantum dots. Phys. Rev. B Condens. Matter Mater. Phys. 79, 1 (2009)
J.H. Prechtel, A.V. Kuhlmann, J. Houel, A. Ludwig, S.R. Valentin, A.D. Wieck, R.J. Warburton, Decoupling a hole spin qubit from the nuclear spins. Nat. Mater. 15, 981 (2016)
M. Borhani, V.N. Golovach, D. Loss, Spin decay in a quantum dot coupled to a quantum point contact. Phys. Rev. B 73, 155311 (2006)
D. Press, K. De Greve, P.L. McMahon, T.D. Ladd, B. Friess, C. Schneider, M. Kamp, S. Höfling, A. Forchel, Y. Yamamoto, Ultrafast optical spin echo in a single quantum dot. Nat. Photonics 4, 367 (2010)
A. Greilich, D.R. Yakovlev, A. Shabaev, A.L. Efros, I.A. Yugova, R. Oulton, V. Stavarache, D. Reuter, A. Wieck, M. Bayer, Mode locking of electron spin coherences in singly charged quantum dots. Science (80-.) 313, 341 (2006)
L. Huthmacher, R. Stockill, E. Clarke, M. Hugues, C. Le Gall, M. Atatüre, Coherence of a dynamically decoupled quantum-dot hole spin. Phys. Rev. B 97, 1 (2018)
X. Xu, B. Sun, P.R. Berman, D.G. Steel, A.S. Bracker, D. Gammon, L.J. Sham, Coherent population trapping of an electron spin in a single negatively charged quantum dot. Nat. Phys. 4, 692 (2008)
J. Houel, J.H. Prechtel, A.V. Kuhlmann, D. Brunner, C.E. Kuklewicz, B.D. Gerardot, N.G. Stoltz, P.M. Petroff, R.J. Warburton, High resolution coherent population trapping on a single hole spin in a semiconductor quantum dot. Phys. Rev. Lett. 112, 107401 (2014)
B. Sangshekan, N. Einali Saghavaz, A. Hamrah Gharamaleki, M. Sahrai, Maximal atom-photon entanglement by the incoherent pumping fields. Eur. Phys. J. Plus 134, 274 (2019)
M. Ghaderi Goran Abad, M. Mahmoudi, Atom–photon entanglement near a plasmonic nanostructure. Eur. Phys. J. Plus 135, 352 (2020)
Z. Amini Sabegh, R. Amiri, M. Mahmoudi, Spatially dependent atom-photon entanglement. Sci. Rep. 8, 13840 (2018)
J.R. Schaibley, Spin-photon Entanglement and quantum optics with single quantum dots, Ph.D. thesis, University of Michigan, Michigan (2013)
H. Araki, E.H. Lieb, Entropy inequalities. Commun. Math. Phys. 18, 160 (1970)
K.L. Truex, Optical coherent control of a single charged indium arsenied quantum dot. Ph.D. thesis. University of Michigan, Michigan (2013)
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Appendix
Appendix
As an example, we calculate the term \( H_{14}\) in Eq. (9). From Eqs. (2), (6) and (7), one can evaluate the Hamiltonian term
where \(\Omega_{x} \equiv \frac{{\wp E_{x} }}{\hbar \surd 2}\) and \(\Omega_{y} \equiv \frac{{i\wp E_{y} }}{\hbar \surd 2}\) are the Rabi frequencies along the x- and y-axis.
Thus,
According to the RWA, we can neglect terms that oscillate at 2ω, as they will average out to zero, while the other terms remain unchanged. Therefore,\( H_{14} = \frac{\hbar }{2} \Omega_{x}^{*} \left( t \right)\). Similarly, the other terms of Eq. (9) can be obtained.
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Memarzadeh, M., Sahrai, M. & Hamedi, H.R. Quantum entanglement between a hole spin confined to a semiconductor quantum dot and a photon. Eur. Phys. J. Plus 138, 75 (2023). https://doi.org/10.1140/epjp/s13360-023-03652-8
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DOI: https://doi.org/10.1140/epjp/s13360-023-03652-8