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Correlation between dynamical heterogeneities, structure and potential-energy distribution in a 2D amorphous solid

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Abstract.

We investigate the collective properties of particles in a 2D experimental system which consists of a bi-disperse mixture of colloidal particles confined at an air/water interface. We find a direct correlation between structure and dynamical heterogeneities in this system: particles belonging to locally ordered structures have lower potential energy and are slower than other particles. In a more general way we show that particles with high potential energy are dominating the dynamics especially in the α-relaxation regime.

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References

  1. W. Kob, C. Donati, S.J. Plimpton, P.H. Poole, S.C. Glotzer, Phys. Rev. Lett. 79, 2827 (1997)

    Article  ADS  Google Scholar 

  2. C. Donati, J.F. Douglas, W. Kob, S.J. Plimpton, P.H. Poole, S.C. Glotzer, Phys. Rev. Lett. 80, 2338 (1998)

    Article  ADS  Google Scholar 

  3. L. Berthier, G. Biroli, J.P. Bouchaud, L. Cipelletti, D. El Masri, D. L'Hôte, F. Ladieu, M. Pierno, Science 310, 1797 (2005)

    Article  ADS  Google Scholar 

  4. L. Berthier, D. Chandler, J.P. Garrahan, Europhys. Lett. 69, 320 (2005)

    Article  ADS  Google Scholar 

  5. H. König, R. Hund, K. Zahn, G. Maret, Eur. Phys. J. E 18, 287 (2005)

    Article  Google Scholar 

  6. G.A. Appignanesi, J.A. Rodríguez Fris, R.A. Montani, W. Kob, Phys. Rev. Lett. 96, 057801 (2006)

    Article  ADS  Google Scholar 

  7. E.R. Weeks, J.C. Crocker, A.C. Levitt, A. Schofield, D.A. Weitz, Science 287, 627 (2000)

    Article  ADS  Google Scholar 

  8. W.K. Kegel, A. van Blaaderen, Science 287, 290 (2000)

    Article  ADS  Google Scholar 

  9. V. Trappe, E. Pitard, L. Ramos, A. Robert, H. Bissig, L. Cipelletti, Phys. Rev. E 76, 051404 (2007)

    Article  ADS  Google Scholar 

  10. P. Yunker, Z. Zhang, K.B. Aptowicz, A.G. Yodh, Phys. Rev. Lett. 103, 115701 (2009)

    Article  ADS  Google Scholar 

  11. M. Dzugutov, S.I. Simdyankin, F.H. Zetterling, Phys. Rev. Lett. 89, 195701 (2002)

    Article  ADS  Google Scholar 

  12. K. Vollmayr-Lee, W. Kob, K. Binder, A. Zippelius, J. Chem. Phys. 116, 5158 (2002)

    Article  ADS  Google Scholar 

  13. K. Yoshimoto, T.S. Jain, K. Van Workum, P.F. Nealey, J.J. de Pablo, Phys. Rev. Lett. 93, 175501 (2004)

    Article  ADS  Google Scholar 

  14. L. Berthier, R.L. Jack, Phys. Rev. E 76, 041509 (2007)

    Article  ADS  Google Scholar 

  15. D. Coslovich, G. Pastore, J. Chem. Phys. 127, 124504 (2007)

    Article  ADS  Google Scholar 

  16. C.P. Royall, S.R. Williams, T. Ohtsuka, H. Tanaka, Nat. Mater. 7, 556 (2008)

    Article  ADS  Google Scholar 

  17. H. Shiba, A. Onuki, T. Araki, EPL 86, 66004 (2009)

    Article  ADS  Google Scholar 

  18. H. Shintani, H. Tanaka, Nat. Phys. 2, 200 (2006)

    Article  Google Scholar 

  19. T. Kawasaki, T. Araki, H. Tanaka, Phys. Rev. Lett. 99, 215701 (2007)

    Article  ADS  Google Scholar 

  20. G.S. Matharoo, M.S. Gulam Razul, P.H. Poole, Phys. Rev. E 74, 050502 (2006)

    Article  ADS  Google Scholar 

  21. A. Widmer-Cooper, P. Harrowell, H. Fynewever, Phys. Rev. Lett. 93, 135701 (2004)

    Article  ADS  Google Scholar 

  22. A. Widmer-Cooper, P. Harrowell, Phys. Rev. Lett. 96, 185701 (2006)

    Article  ADS  Google Scholar 

  23. B. Cui, B. Lin, S.A. Rice, J. Chem. Phys. 114, 9142 (2001)

    Article  ADS  Google Scholar 

  24. F. Ebert, P. Dillmann, G. Maret, P. Keim, Rev. Sci. Instrum. 80, 083902 (2009)

    Article  ADS  Google Scholar 

  25. F. Ebert, P. Keim, G. Maret, Eur. Phys. J. E 26, 161 (2008)

    Article  Google Scholar 

  26. L. Assoud, F. Ebert, P. Keim, R. Messina, G. Maret, H. Löwen, J. Phys.: Condens. Matter 21, 464114 (2009)

    Article  ADS  Google Scholar 

  27. L. Assoud, F. Ebert, P. Keim, R. Messina, G. Maret, H. Löwen, Phys. Rev. Lett. 102, 238301 (2009)

    Article  ADS  Google Scholar 

  28. F. Ebert, G. Maret, P. Keim, Eur. Phys. J. E 29, 301 (2009)

    Article  Google Scholar 

  29. L. Assoud, R. Messina, H. Löwen, EPL 80, 48001 (2007)

    Article  ADS  Google Scholar 

  30. J. Fornleitner, F. Lo Verso, G. Kahl, C. N. Likos, Soft Matter 4, 480 (2008)

    Article  ADS  Google Scholar 

  31. S. Mazoyer, F. Ebert, G. Maret, P. Keim, EPL 88, 66004 (2009)

    Article  ADS  Google Scholar 

  32. X.H. Zheng et al., Europhys. Lett. 41, 635 (1998)

    Article  ADS  Google Scholar 

  33. K. Zahn et al., Phys. Rev. Lett. 85, 3656 (2000)

    Article  ADS  Google Scholar 

  34. C. Klix, F. Ebert, G. Maret, P. Keim, arXiv:1108.2636v1

  35. C. Mayer, E. Zaccarelli, E. Stiakakis, C.N. Likos, F. Sciortino, A. Munam, M. Gauthier, N. Hadjichristidis, H. Iatrou, P. Tartaglia, H. Löwen, D. Vlassopoulos, Nat. Mater. 7, 780 (2008)

    Article  ADS  Google Scholar 

  36. R. Juárez-Maldonado, M. Medina-Noyola, Phys. Rev. Lett. 101, 267801 (2008)

    Article  ADS  Google Scholar 

  37. N. Hoffmann, F. Ebert, C.N. Likos, H. Löwen, G. Maret, Phys. Rev. Lett. 97, 078301 (2006)

    Article  ADS  Google Scholar 

  38. N.D. Mermin, Phys. Rev. 176, 250 (1968)

    Article  ADS  Google Scholar 

  39. E. Flenner, G. Szamel, Phys. Rev. Lett. 105, 217801 (2010)

    Article  ADS  Google Scholar 

  40. H. Tanaka, T. Kawasaki, H. Shintani, K. Watanabe, Nat. Mater. 9, 324 (2010)

    Article  ADS  Google Scholar 

  41. U. Schneider, P. Lunkenheimer, A. Pimenov, R. Brand, A. Loidl, Ferroelectics 249, 89 (2001)

    Article  Google Scholar 

  42. We omit the index $_{\rm CR}$ since we always refer to cage-relative quantities in the following

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Correspondence to P. Keim.

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Mazoyer, S., Ebert, F., Maret, G. et al. Correlation between dynamical heterogeneities, structure and potential-energy distribution in a 2D amorphous solid. Eur. Phys. J. E 34, 101 (2011). https://doi.org/10.1140/epje/i2011-11101-1

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  • DOI: https://doi.org/10.1140/epje/i2011-11101-1

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