Skip to main content
Log in

A cluster source for photoelectron spectroscopy in VUV and X-ray ranges

  • Regular Article - Molecular Physics and Chemical Physics
  • Published:
The European Physical Journal D Aims and scope Submit manuscript

Abstract

A detailed description of a custom-made gas aggregation cluster source is given as well as of its coupling to permanent molecular beam end-stations of the beamlines DESIRS and PLEIADES at the French national facility synchrotron SOLEIL. Using (hydrated) hypoxanthine clusters as a case study, the production of clusters with different source parameters is discussed based on Vacuum Ultra-Violet (VUV) mass spectrometry. The ability of the cluster source to perform photoelectron spectroscopy is illustrated by photoelectron spectra obtained for valence and core shells.

Graphic abstract

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7

Similar content being viewed by others

Data Availability Statement

This manuscript has no associated data, or the data will not be deposited. [Authors comment: The datasets generated during and/or analysed during the current study are available from the corresponding author on reasonable request.]

References

  1. A. Abo-Riziq, L. Grace, E. Nir, M. Kabelac, P. Hobza, M.S. De Vries, Proc. Natl. Acad. Sci. U.S.A. 102, 20 (2005)

    Article  ADS  Google Scholar 

  2. T. Schlathölter, F. Alvarado, S. Bari, A. Lecointre, R. Hoekstra, V. Bernigaud, B. Manil, J. Rangama, B. Huber, ChemPhysChem 7, 2339 (2006)

    Article  Google Scholar 

  3. S. Maclot, M. Capron, R. Maisonny, A. Lawicki, A. Méry, J. Rangama, J.Y. Chesnel, S. Bari, R. Hoekstra, T. Schlathölter, B. Manil, L. Adoui, P. Rousseau, B.A. Huber, ChemPhysChem 12, 930 (2011)

    Article  Google Scholar 

  4. S.K. Kim, W. Lee, D.R. Herschbach, J. Phys. Chem. 100, 7933 (1996)

    Article  Google Scholar 

  5. A. Domaracka, M. Capron, S. Maclot, J.Y. Chesnel, A. Méry, J.C. Poully, J. Rangama, L. Adoui, P. Rousseau, B.A. Huber ,Phys. Conf. Ser. 373, 012005 (2012)

  6. B. Barc, M. Ryszka, J. Spurrell, M. Dampc, P. Limão-Vieira, R. Parajuli, N.J. Mason, S. Eden, J. Chem. Phys. 139, 244311 (2013)

  7. M. Neustetter, J. Aysina, F.F. Da Silva, S. Denifl, Angew. Chemie—Int. Ed. 54, 9124 (2015)

    Article  Google Scholar 

  8. E. Wang, X. Ren, W.Y. Baek, H. Rabus, T. Pfeifer, A. Dorn, Nat. Commun. 11, 2194 (2020)

    Article  ADS  Google Scholar 

  9. S. Lee, S.J. Valentine, J.P. Reilly, D.E. Clemmer, J. Am. Chem. Soc. 133, 15834 (2011)

    Article  Google Scholar 

  10. M. Nihamkin, A. Isaak, A. Albeck, Y. Mastai, Y. Toker, J. Phys. Chem. Lett. 10, 10100 (2020)

  11. P. Rousseau, D.G. Piekarski, M. Capron, A. Domaracka, L. Adoui, F. Martín, M. Alcamí, S. Díaz-Tendero, B.A. Huber, Nat. Commun. 11, 3818 (2020)

    Article  ADS  Google Scholar 

  12. S. Hüfner, Photoelectron Spectroscopy—-Principles and Applications (Springer, Berlin, 2003)

    Book  Google Scholar 

  13. J. Stöhr, R. Gomer, NEXAFS Spectroscsopy (Springer, Berlin, 1992)

    Book  Google Scholar 

  14. Martin Schwell, M. Hochlaf, Top. Curr. Chem. 355, 155 (2014)

    Article  Google Scholar 

  15. K.C. Prince, P. Bolognesi, V. Feyer, O. Plekan, L. Avaldi, J. Electron Spectros. Relat. Phenomena 204, 335 (2015)

    Article  Google Scholar 

  16. P. Bolognesi, L. Avaldi, in Photoprocesses with Biomolecules in the Gas Phase in Nanoscale Insights into Ion-Beam Cancer Therapy, ed. by A.V. Solov’yov (Springer International Publishing, Berlin, 2017), p. 209

  17. F. Gaie-Levrel, G. A. Garcia, M. Schwell, L. Nahon

  18. M. Tia, B. Cunha De Miranda, S. Daly, F. Gaie-Levrel, G.A. Garcia, L. Nahon, I. Powis, J. Phys. Chem. A 118, 2765 (2014)

    Article  Google Scholar 

  19. A. Giuliani, A.R. Milosavljevic, F. Canon, L. Nahon, Mass Spectrom. Rev. 33, 424 (2014)

    Article  ADS  Google Scholar 

  20. A.R. Milosavljevic, A. Giuliani, C. Nicolas, Gas-Phase Near-Edge X-Ray Absorption Fine Structure (NEXAFS) Spectroscopy of Nanoparticles, Biopolymers, and Ionic Species in X-ray and Neutron Techniques for Nanomaterials Characterization, ed. by C.S.S.R. Kumar (Springer, Berlin, 2016), p. 451

  21. S. Bari, D. Egorov, T.L.C. Jansen, R. Boll, R. Hoekstra, S. Techert, V. Zamudio-Bayer, C. Bülow, R. Lindblad, G. Leistner, A. Lawicki, K. Hirsch, P.S. Miedema, B. von Issendorff, J.T. Lau, T. Schlathölter, Chem. —A Eur. J. 24, 7631 (2018)

    Article  Google Scholar 

  22. O. Björneholm, G. Öhrwall, M. Tchaplyguine, Nucl. Instr. Methods Phys. Res. Sect. A Accel. Spectrometers, Detect. Assoc. Equip. 601, 161 (2009)

    Article  ADS  Google Scholar 

  23. M. Ahmed, O. Kostko, Phys. Chem. Chem. Phys. 22, 2713 (2020)

    Article  Google Scholar 

  24. A. Karshikoff, Non-Covalent Interactions in Proteins (Imperial College Press, London, 2006)

  25. G. Mattioli, L. Avaldi, P. Bolognesi, J.D. Bozek, M.C. Castrovilli, J. Chiarinelli, A. Domaracka, S. Indrajith, S. Maclot, A.R. Milosavljevic, C. Nicolafrancesco, C. Nicolas, P. Rousseau, Sci. Rep. 10, 13081 (2020)

    Article  ADS  Google Scholar 

  26. L. Nahon, N. De Oliveira, G.A. Garcia, J.F. Gil, B. Pilette, O. Marcouillé, B. Lagarde, F. Polack, J. Synchrotron Radiat. 19, 508 (2012)

    Article  Google Scholar 

  27. Synchrotron SOLEIL, PLEIADES beamline (2021). https://www.synchrotronsoleil.fr/en/beamlines/pleiades. Accessed 31 Mar 2021

  28. U. Zimmermann, N. Malinowski, U. Näher, S. Frank, T.P. Martin, Z. Phys. D 31,85(1994)

  29. K. Hansen, R. Muller, H. Hohmann, E.E.B. Campbell, Z. Phys. D 40, 361 (1997)

  30. B. Manil, L. Maunoury, B.A. Huber, J. Jensen, H.T. Schmidt, H. Zettergren, H. Cederquist, S. Tomita, P. Hvelplund, Phys. Rev. Lett. 91, 215504 (2003)

    Article  ADS  Google Scholar 

  31. M. Schmidt, A. Masson, C. Bréchignac, Int. J. Mass Spectrom. 252, 173 (2006)

    Article  Google Scholar 

  32. P. Rousseau, A. Lawicki, A.I.S. Holm, M. Capron, R. Maisonny, S. MacLot, E. Lattouf, H.A.B. Johansson, F. Seitz, A. Méry, J. Rangama, H. Zettergren, S. Rosén, H.T. Schmidt, J.Y. Chesnel, A. Domaracka, B. Manil, L. Adoui, H. Cederquist, B.A. Huber, Nucl. Instr. Methods Phys. Res. Sect. B Beam Interact. with Mater. Atoms 279, 140 (2012)

    Article  ADS  Google Scholar 

  33. S. Zamith, P. Labastie, J.M. Lhermite, J. Chem. Phys. 136, 214301 (2012)

  34. R. Maisonny, M. Capron, S. Maclot, J.C. Poully, A. Domaracka, A. Méry, L. Adoui, P. Rousseau, B.A. Huber In: J. Phys. Conf. Ser. 438, 012007 (2013)

  35. P. Markush, P. Bolognesi, A. Cartoni, P. Rousseau, S. Maclot, R. Delaunay, A. Domaracka, J. Kocisek, M.C. Castrovilli, B.A. Huber, L. Avaldi, Phys. Chem. Chem. Phys. 18, 16721 (2016)

    Article  Google Scholar 

  36. I. Braud, S. Zamith, J. Cuny, L. Zheng, J.M. L’Hermite, J. Chem. Phys. 150, 014303 (2019)

  37. H. Haberland, Clusters of Atoms and Molecules (Springer, Berlin, 1994)

    Book  Google Scholar 

  38. S. Hartweg, B.L. Yoder, G.A. Garcia, L. Nahon, R. Signorell, Phys. Rev. Lett. 118, 103402 (2017)

    Article  ADS  Google Scholar 

  39. T.E. Gartmann, S. Hartweg, L. Ban, E. Chasovskikh, B.L. Yoder, R. Signorell, Phys. Chem. Chem. Phys. 20, 16364 (2018)

    Article  Google Scholar 

  40. C. Joblin, L. Dontot, G.A. Garcia, F. Spiegelman, M. Rapacioli, L. Nahon, P. Parneix, T. Pino, P. Bréchignac, J. Phys. Chem. Lett. 8, 3697 (2017)

    Article  Google Scholar 

  41. A. Mauracher, O. Echt, A.M. Ellis, S. Yang, D.K. Bohme, J. Postler, A. Kaiser, S. Denifl, P. Scheier, Phys. Rep. 751, 1 (2018)

    Article  ADS  Google Scholar 

  42. M. Fárník, J. Fedor, J. Kocišek, J. Lengyel, E. Pluharová, V. Poterya, A. Pysanenko, Phys. Chem. Chem. Phys. 23, 3195 (2021)

    Article  Google Scholar 

  43. K. Kitajima, T. Majima, T. Nishio, Y. Oonishi, S. Mizutani, J.ya Kohno, M. Saito, H. Tsuchida, Nucl. Instr. Methods Phys. Res. Sect. B Beam Interact. with Mater. Atoms 424, 10 (2018)

    Article  ADS  Google Scholar 

  44. J. Zahardis, S. Geddes, G.A. Petrucci, Anal. Chem. 83, 2409 (2011)

    Article  Google Scholar 

  45. T. Bergen, X. Biquard, A. Brenac, F. Chandezon, B.A. Huber, D. Jalabert, H. Lebius, M. Maurel, E. Monnand, J. Opitz, A. Pesnelle, B. Pras, C. Ristori, J.C. Rocco, Rev. Sci. Instrum. 70, 3244 (1999)

    Article  ADS  Google Scholar 

  46. C. Bréchignac, P. Cahuzac, F. Carlier, M. de Frutos, A. Masson, J. Roux, Z. Phys. D19, 195 (1991)

  47. J. Kocišek, A. Pysanenko, M. Fárník, J. Fedor, J. Phys. Chem. Lett. 7, 3401 (2016)

    Article  Google Scholar 

  48. X. Tang, G.A. Garcia, J.F. Gil, L. Nahon, Rev. Sci. Instrum. 86, 123108 (2015)

    Article  ADS  Google Scholar 

  49. G.A. Garcia, B.K. Cunha De Miranda, M. Tia, S. Daly, L. Nahon, Rev. Sci. Instrum. 84, 053112 (2013)

  50. G.W. Fraser, Int. J. Mass Spectrom. 215, 13 (2002)

    Article  Google Scholar 

  51. M. Tia, Ph.D. thesis, Université Paris-Sud (2014)

  52. A. Lindblad, J. Söderström, C. Nicolas, E. Robert, C. Miron, Rev. Sci. Instrum. 84, 113105 (2013)

  53. R.T. Jongma, Y. Huang, S. Shi, A.M. Wodtke, J. Phys. Chem. A 102, 8847 (1998)

    Article  Google Scholar 

  54. V. Feyer, O. Plekan, R. Richter, M. Coreno, K.C. Prince, Chem. Phys. 358, 33 (2009)

    Article  Google Scholar 

  55. O. Plekan, V. Feyer, R. Richter, A. Moise, M. Coreno, K.C. Prince, I.L. Zaytseva, T.E. Moskovskaya, D.Y. Soshnikov, A.B. Trofimov, J. Phys. Chem. A 116, 5653 (2012)

    Article  Google Scholar 

  56. V. Myrseth, J.D. Bozek, E. Kukk, L.J. Sathre, T.D. Thomas, J. Electron Spectros. Relat. Phenomena 122, 57 (2002)

    Article  Google Scholar 

Download references

Acknowledgements

CN is co-funded by Région Normandie and Synchrotron SOLEIL. We thank the technical staff of SOLEIL for running smoothly the facility under projects 20191563 and 20191936.

Author information

Authors and Affiliations

Authors

Contributions

PR and ARM designed the experiments. JFG, ER, and JMR designed the mechanical parts. CN, SH, LN, SI, ChrN, JB, PR, and ARM performed the experiments. CN and SH analysed the data. CN, SH, LN, PR, and ARM prepared the draft manuscript. All authors commented the draft manuscript and approved the final manuscript.

Corresponding author

Correspondence to Aleksandar R. Milosavljević.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Nicolafrancesco, C., Hartweg, S., Gil, JF. et al. A cluster source for photoelectron spectroscopy in VUV and X-ray ranges. Eur. Phys. J. D 75, 117 (2021). https://doi.org/10.1140/epjd/s10053-021-00124-5

Download citation

  • Received:

  • Accepted:

  • Published:

  • DOI: https://doi.org/10.1140/epjd/s10053-021-00124-5

Navigation