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Deformation of the Raman scattering spectrum of Ih ice under local laser heating near 0°C

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Abstract

The Raman band of Nd:YAG laser second-harmonic scattering from the O-H stretching vibrations of hexagonal ice was observed to broaden asymmetrically by 90 cm−1 near 0°C with the pulse repetition frequency increasing from 1 to 8 Hz. The center of this band was found to undergo simultaneously a Stokes shift by 25 cm−1. The observed spectral features can be accounted for by the ice being heated by pulsed laser radiation through the electrocaloric effect, because the one-photon absorption mechanism produces a negligible contribution.

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Authors and Affiliations

  1. Wave Research Center, General Physics Institute, Russian Academy of Sciences, Moscow, 117942, Russia

    N. P. Andreeva, A. F. Bunkin & S. M. Pershin

Authors
  1. N. P. Andreeva
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  2. A. F. Bunkin
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  3. S. M. Pershin
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__________

Translated from Optika i Spektroskopiya, Vol. 93, No. 2, 2002, pp. 269–273.

Original Russian Text Copyright © 2002 by Andreeva, Bunkin, Pershin.

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Andreeva, N.P., Bunkin, A.F. & Pershin, S.M. Deformation of the Raman scattering spectrum of Ih ice under local laser heating near 0°C. Opt. Spectrosc. 93, 252–256 (2002). https://doi.org/10.1134/1.1503755

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  • DOI: https://doi.org/10.1134/1.1503755

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