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Abstract:

The femtosecond photodissociation of CsI in the CsI-CH3CN complex has been studied. Recurrences are observed in the detection of the Cs+-CH3CN ion complex. They are assigned to the first vibrations of the Cs-NCCH3 bond formed after the CsI dissociation. This result is in good agreement with calculations on the similar NaI-CH3CN system which predict a linear structure for the ground state complex.

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Received 27 October 1999

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Grégoire, G., Mons, M., Dimicoli, I. et al. Observation of the first vibrations of the newly born Cs-CH CN complex. Eur. Phys. J. D 11, 227–231 (2000). https://doi.org/10.1007/s100530070087

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  • DOI: https://doi.org/10.1007/s100530070087

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