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A high-resolution time-of-flight mass spectrometer for the detection of ultracold molecules

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Abstract

We have realized a high-resolution time-of-flight mass spectrometer combined with a magneto-optical trap. The spectrometer enables excellent optical access to the trapped atomic cloud using specifically devised acceleration and deflection electrodes. The ions are extracted along a laser beam axis and deflected onto an off-axis detector. The setup is applied to detect atoms and molecules photoassociated from ultracold atoms. The detection is based on resonance-enhanced multi-photon ionization. Mass resolution up to m/Δmrms=1000 at the mass of 133Cs is achieved. The performance of this spectrometer is demonstrated in the detection of photoassociated ultracold 7Li133Cs molecules near a large signal of 133Cs ions.

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References

  1. J. Ullrich, V.P. Shevelko, editors, Many-Particle Quantum Dynamics in Atomic and Molecular Fragmentation, (Springer, Berlin, 2003)

  2. G. Petty, C. Tai, F.W. Dalby, Phys. Rev. Lett. 34, 1207 (1975)

    Article  ADS  Google Scholar 

  3. A. Fioretti, D. Comparat, A. Crubellier, O. Dulieu, F. Masnou-Seeuws, P. Pillet, Phys. Rev. Lett. 80, 4402 (1998)

    Article  ADS  Google Scholar 

  4. C. Gabbanini, A. Fioretti, A. Lucchesini, S. Gozzini, M. Mazzoni, Phys. Rev. Lett. 84, 2814 (2000)

    Article  ADS  Google Scholar 

  5. A.N. Nikolov, E.E. Eyler, X.T. Wang, J. Li, H. Wang, W.C. Stwalley, P.L. Gould, Phys. Rev. Lett. 82, 703 (1999)

    Article  ADS  Google Scholar 

  6. A. Kerman, J.M. Sage, S. Sainis, T. Bergeman, D. DeMille, Phys. Rev. Lett. 92, 153001 (2004)

    Article  ADS  Google Scholar 

  7. M.W. Mancini, G.D. Telles, A.R.L. Caires, V.S. Bagnato, L.G. Marcassa, Phys. Rev. Lett. 92, 133203 (2004)

    Article  ADS  Google Scholar 

  8. D. Wang, J. Qi, M.F. Stone, O. Nikolayeva, H. Wang, B. Hattaway, S.D. Gensemer, P.L. Gould, E.E. Eyler, W.C. Stwalley, Phys. Rev. Lett. 93, 243005 (2004)

    Article  ADS  Google Scholar 

  9. C. Haimberger, J. Kleinert, M. Bhattacharya, N.P. Bigelow, Phys. Rev. A 70, 021402 (2004)

    Article  ADS  Google Scholar 

  10. W.C. Wiley, I.H. McLaren, Rev. Sci. Instrum. 26, 1150 (1955)

    Article  ADS  Google Scholar 

  11. C. Weickhardt, F. Moritz, J. Grotemeyer, Mass Spectrom. Rev. 15, 139 (1996)

    Google Scholar 

  12. W. Paul, H.P. Reinhard, U. von Zahn, Z. Phys. 152, 143 (1958)

    Article  ADS  Google Scholar 

  13. J.L. Wiza, Nucl. Instrum. Methods 162, 587 (1979)

    Article  Google Scholar 

  14. SimIon 3D Version 7.0, Idaho National Engineering and Environmental Laboratory

  15. U. Boesl, H.J. Neusser, R. Weinkauf, E.W. Schlag, J. Phys. Chem. 86, 4857 (1982)

    Article  Google Scholar 

  16. R. Frey, G. Weiss, H. Kaminski, E.W. Schlag, Z. Naturforsch. 40a, 1349 (1985)

    Google Scholar 

  17. R.P. Schmid, C. Weickhardt, Int. J. Mass Spectrom. 206, 181 (2001)

    Google Scholar 

  18. S.D. Kraft, P. Staanum, J. Lange, L. Vogel, R. Wester, M. Weidemüller, J. Phys. B 39, S993 (2006)

    Article  ADS  Google Scholar 

  19. P. Staanum, A. Pashov, H. Knöckel, E. Tiemann, Phys. Rev. A 75, 042513 (2007)

    Article  ADS  Google Scholar 

  20. U. Schlöder, H. Engler, U. Schünemann, R. Grimm, M. Weidemüller, Eur. Phys. J. D 73, 802 (1999)

    Google Scholar 

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Correspondence to S.D. Kraft.

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07.75.+h; 32.80.Rm; 37.10.Gh

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Kraft, S., Mikosch, J., Staanum, P. et al. A high-resolution time-of-flight mass spectrometer for the detection of ultracold molecules. Appl. Phys. B 89, 453–457 (2007). https://doi.org/10.1007/s00340-007-2855-8

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  • DOI: https://doi.org/10.1007/s00340-007-2855-8

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