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Electron-β-Nuclear Spectroscopy of Atoms and Molecules and Chemical Bond Effect on the β-Decay Parameters

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Book cover Advances in the Theory of Atomic and Molecular Systems

Part of the book series: Progress in Theoretical Chemistry and Physics ((PTCP,volume 20))

Abstract

We discuss the cooperative electron β-nuclear processes in atoms and molecules, including the excitation, ionization, electronic rearrangement, induced by the nuclear reactions and β-decay. The relativistic many-body perturbation theory (PT) with the optimized Dirac–Kohn–Sham (DKS) zeroth approximation is used to calculate the β-decay parameters for a number of allowed (superallowed) transitions (33P–33S, 241Pu–241Am, etc.) and study a chemical bond effect on β-decay parameters. A few factors are taken into account: changing the integration limits in the Fermi function integral, energy corrections for different chemical substances and the possibility of the bound β-decay or other decay channels. We studied the electronic rearrangement induced by nuclear transmutation in the β-decay \({}_{\rm{2}}^{\rm{6}} {\rm{He}}_{\rm{4}} \to ({}_3^6 {\rm{Li}}_{\rm{3}}^{\rm{ + }} )^* + e^ - + \bar \nu _e \). The half-life period T 1 / 2 for β-decay of tritium atom (ion) has been estimated while taking into account the bound β-decay channel and some other accompanying effects. The estimated values of T 1 / 2 for the tritium β-decay and free triton decay are (T 1 / 2)a=12.26 years (correction due to the electron-atomic effects (Δ T 1 / 2/T 1 / 2) a =0.82%) for the tritium atom and (T 1 / 2) t =12.36 years for the triton decay. These data are in physically reasonable agreement with experimental data. We first present the value T 1 / 2 in a case of the β-decay in the halogen-containing molecular tritium (3HCl): (T 1 / 2) m =12.28 years (3HCl) and the correction due to the chemical bond effect is (Δ T 1 / 2) am =0.024 (i.e. 0.20%).

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Authors and Affiliations

  1. Odessa University, 65009, Odessa-9, Ukraine

    Alexander V. Glushkov & Olga Yu. Khetselius

  2. Russian Academy of Sciences, 142090, Troitsk, Russia

    Alexander V. Glushkov & Olga Yu. Khetselius

  3. UK National Academy of Sciences and Bookdata Co, SW1Y 5AG, London, UK

    Ludmila Lovett

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  1. Alexander V. Glushkov
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  2. Olga Yu. Khetselius
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  3. Ludmila Lovett
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Editors and Affiliations

  1. Department of Chemistry, Michigan State University, 48824, East Lansing, MI, USA

    Piotr Piecuch

  2. Laboratoire de Chimie Physique, CNRS and UPMC, 11 rue Pierre et Marie Curie, 75005, Paris, France

    Jean Maruani

  3. Instituto de Física Fundamental CSIC, Serrano, 123, E-28006, Madrid, Spain

    Gerardo Delgado-Barrio

  4. Physical & Theoretical Chemistry Laboratory, University of Oxford, South Parks Rd, OX1 3QZ, Oxford, United Kingdom

    Stephen Wilson

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Glushkov, A.V., Khetselius, O.Y., Lovett, L. (2009). Electron-β-Nuclear Spectroscopy of Atoms and Molecules and Chemical Bond Effect on the β-Decay Parameters. In: Piecuch, P., Maruani, J., Delgado-Barrio, G., Wilson, S. (eds) Advances in the Theory of Atomic and Molecular Systems. Progress in Theoretical Chemistry and Physics, vol 20. Springer, Dordrecht. https://doi.org/10.1007/978-90-481-2985-0_7

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