Summary
An efficient semiclassical optimal control theory for controlling wavepacket dynamics on a single adiabatic potential energy surface applicable to systems with many degrees of freedom is discussed in detail. The approach combines the advantages of various formulations of the optimal control theory: quantum and classical on the one hand and global and local on the other. The efficiency and reliability of the method are demonstrated, using systems with two and four dimensions as examples.
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Kondorskiy, A., Mil’nikov, G., Nakamura, H. (2007). Laser Control of Chemical Dynamics. II. Control of Wavepacket Motion. In: Progress in Ultrafast Intense Laser Science II. Springer Series in Chemical Physics, vol 85. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-540-38156-3_6
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DOI: https://doi.org/10.1007/978-3-540-38156-3_6
Publisher Name: Springer, Berlin, Heidelberg
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