Abstract
Coherent control method steers a quantum system to a desirable final quantum state among a number of final states otherwise possible in a given light-matter interaction, by using a specially shaped light form programmed in its spectral and/or temporal domain. In this chapter, we briefly review a number of light-form shaping methods previously considered for coherent control of ultra-fast laser interaction with atoms, and provide their application examples along with their experimental demonstrations.
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Notes
- 1.
We notice that Fourier domain and frequency domain have the same physical meaning in this chapter.
- 2.
(field) means that the description is about electric field. Readers should care whether (field) or (intensity) arise at the end of a description.
- 3.
Four-photon sequential path is \(3\text {S}{-}4\text {S}-7\text {P}\) \(2+1\) photon process in addition to \(7\text {P}{-}4\text {S}\) one-photon de-excitation. In this experiment, several order of magnitude is smaller than two-photon direct path.
- 4.
The linear spectral chirp \(\varPhi ''\) in (4.3) and \(a_2\) here is identical parameter.
- 5.
For more detailed description, we would recommend readers to read [13].
- 6.
Three ultra-fast pulses are incident on the target, with separately controllable pico-second scale time delays \(\tau _1\) and \(\tau _2\) between each consecutive pulse. The excited states induced by each pulse are interfered and the final fluorescence signal \(I(\tau _1, \tau _2)\) is recorded. Two-dimensional Fourier transform of \(I(\tau _1, \tau _2)\) acquires both amplitude and phase information. Detailed theoretical description on this experiment can be found from [22].
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Kim, H., Lee, H., Lim, J., Ahn, J. (2015). Optimal Pulse Shaping for Ultrafast Laser Interaction with Quantum Systems. In: Yamanouchi, K., Nam, C., Martin, P. (eds) Progress in Ultrafast Intense Laser Science XI. Springer Series in Chemical Physics(), vol 109. Springer, Cham. https://doi.org/10.1007/978-3-319-06731-5_4
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