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Surface Phonons and their Role in Ultrafast Phenomena

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Book cover Ultrafast Dynamics of Quantum Systems

Part of the book series: NATO Science Series: B: ((NSSB,volume 372))

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Abstract

Many ultrafast optical phenomena studied with pump-and-probe techniques occur on or below the time scale of microscopic vibrations and can therefore involve or even generate high-frequency phonons. Since most semiconductor structures currently studied with ultrafast optical methods are obtained with planar technologies and retain a quasi-2D character, surface phonons are actually to be considered. In the first two lectures the basic theory and fundamental aspects of surface phonons are introduced, with a summary description of the surface phonon dispersion curves for some relevant semiconductor crystal surfaces. In the third lecture some recent pump-and-probe investigations of ultrafast phenomena involving surface phonons on semiconductor as well as metal surfaces are briefly discussed.

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References

  1. Lord Rayleigh, Proc. London Math. Soc., 17 (1887) 4.

    Article  Google Scholar 

  2. G.W. Farnell, in: Physical Acoustics, Vol. 6, Eds. W.P. Mason and R.N. Thurston (Academic Press, New York, 1970) p. 109.

    Google Scholar 

  3. A.A. Maradudin, in: Nonequilibrium Phonon Dynamics, Ed. by W.E. Bron (Plenum New York 1985) p. 395.

    Google Scholar 

  4. M. Born and Th. von Kármán, Phys. Zeit. 13 (1912) 297.

    Google Scholar 

  5. M. Born and K. Huang, “Dynamical Theory of Crystal Lattices” (Oxford University Press, London, New York 1954).

    MATH  Google Scholar 

  6. F.W. de Wette and W. Kress (eds.), Surface Phonons, Springer Ser. Surf. Sci., Vol. 21 (Springer, Berlin, Heidelberg 1991).

    Google Scholar 

  7. V. Bortolani, A. Franchini and G. Santoro in: Electronic Structure, Dynamics and Quantum Structural Properties of Condensed Matter, Eds. J.T. Devreese and P. van Camp (Plenum Press, New York 1984) p. 401.

    Google Scholar 

  8. For an updated account see the review article: J.P. Toennies and G. Benedek, Surf. Sci. Rep. (1988, in press).

    Google Scholar 

  9. For a compilation of bulk phonon data see H.R. Schober and P.H. Dedrich in Landolt-Börnstein, Neue Serie Bd. 13a (Springer V., Berlin 1981).

    Google Scholar 

  10. I.M. Lifshitz and L.M. Rozenzweig, Zh. Eksp. Teor. Fiz. 18 (1948) 1012.

    Google Scholar 

  11. I.M. Lifshitz Nuovo Cimento Suppl. 3 (1956) 732.

    Google Scholar 

  12. I.M. Lifshitz and A.M. Kosevich, Rep. Progr. Phys. 29(I) (1966) 217.

    Article  ADS  Google Scholar 

  13. A. A. Maradudin, E.W. Montroll, G.H. Weiss and I.P. Ipatova, Theory of Lattice Dynamics in the Harmonic Approximation, Solid State Physics, Suppl. 3 Academic Press, New York 1971).

    Google Scholar 

  14. A.A. Maradudin and J. Melngailis, Phys. Rev. 133 (1964) A1188.

    Article  ADS  Google Scholar 

  15. S.W. Musser and K.H. Rieder, Phys. Rev. B 2 (1970) 3034.

    Article  ADS  Google Scholar 

  16. T.P. Martin, Phys. Rev. B1 (1970) 3480.

    ADS  Google Scholar 

  17. G. Benedek, Phys. Status Sol. B58 (1973) 661.

    Article  ADS  Google Scholar 

  18. G. Benedek, Surface Sci. 61 (1976) 603.

    Article  ADS  Google Scholar 

  19. G. Benedek, M. Miura, W. Kress and H. Bilz, Phys. Rev. Lett. 52 (1984) 1907.

    Article  ADS  Google Scholar 

  20. G. Benedek and L. Miglio, in: Surface Phonons, Eds. F.W. deWette and W. Kress, Springer Ser. Surf. Sci., Vol. 27 (Springer, Berlin, Heidelberg 1991)

    Google Scholar 

  21. A.A. Maradudin, R.F. Wallis and L. Dobrzynski, Handbook of Surfaces and Interfaces, Vol. 3 (Garland, New York 1980).

    Google Scholar 

  22. F. Garcia-Moliner, Ann. Phys. (Paris) 2 (1977) 179.

    Google Scholar 

  23. G. Armand, Phys. Rev. B14 (1976) 2218.

    ADS  Google Scholar 

  24. T.E. Feuchtwang, Phys. Rev. 155 (1967) 731.

    Article  ADS  Google Scholar 

  25. V. Bortolani, F. Nizzoli and G. Santoro, in: Lattice Dynamics, Ed. M. Balkanski (Flammarion, Paris 1978) p..

    Google Scholar 

  26. J. Szeftel and A. Khater, J. Phys. C20 (1987) 4725; J. Szeftel, A. Khater, F. Mila, S. d’Addato, N. Auby, J. Phys. C21 (1988) 2133; A. Khater, N. Auby and R.F. Wallis, Physica B167 (1991) 273; A. Khater, H. Grimeck, J. Lapujoulade and F. Fabre, Surf. Sci. 251/252(1991)291.

    ADS  Google Scholar 

  27. S. Trullinger, J. Math. Phys. 17 (1976) 1884.

    Article  ADS  Google Scholar 

  28. J.E. Black, in Dynamical Properties of Solids, Eds. G.K. Horton and A.A. Maradudin (Elsevier, Amsterdam 1990) Chap. 5.

    Google Scholar 

  29. F.W. de Wette, in: Surface Phonons, Eds. F.W. de Wette and W. Kress, Springer Series on Surf. Sci. Vol. 27 (Springer, Berlin, Heidelberg 1991) p. 67.

    Google Scholar 

  30. R.E. Allen and F.W. de Wette, Phys. Rev. 179 (1969) 873.

    Article  ADS  Google Scholar 

  31. R.E. Allen, F.W. de Wette and A. Rahman, Phys. Rev. 179 (1969) 887.

    Article  ADS  Google Scholar 

  32. G.P. Alldredge, R.E. Allen and F.W. de Wette, J. Acoust. Soc. Am. 49 (1971) 1453.

    Article  ADS  Google Scholar 

  33. R.E. Allen, G.P. Alldredge and F.W. de Wette, Phys. Rev. Lett. 23 (1969) 1285.

    Article  ADS  Google Scholar 

  34. R.E. Allen, G.P. Alldredge and F.W. de Wette, Phys. Rev. B4 (1971) 1648 and 1661.

    ADS  Google Scholar 

  35. T.S. Chen, G.P. Alldredge, F.W. de Wette and R.E. Allen, Phys. Rev. Letters 26 (1971) 1543.

    Article  ADS  Google Scholar 

  36. T.S. Chen, G.P. Alldredge and F.W. de Wette, Solid State Commun. 10 (1972) 941.

    Article  ADS  Google Scholar 

  37. T.S. Chen, G.P. Alldredge and F.W. de Wette, Phys. Lett. 40A (1972) 401.

    ADS  Google Scholar 

  38. T.S. Chen, F.W. de Wette and G.P. Alldredge, Phys. Rev. B15 (1977) 1167.

    ADS  Google Scholar 

  39. G.P. Alldredge, Phys. Lett. 41A (1972) 291.

    ADS  Google Scholar 

  40. V.L. Zoth, G.P. Alldredge and F.W. de Wette, Phys. Lett. 47A (1974) 247.

    ADS  Google Scholar 

  41. F.W. de Wette, in: Dynamical Properties of Solids, Eds. G.K. Horton and A.A. Maradudin (Elsevier, Amsterdam 1990) Chap. 5.

    Google Scholar 

  42. A. Lock, J.P. Toennies and G. Witte, J. Electr. Spectr. Rel. Phenom. 54/55 (1990) 309.

    Article  Google Scholar 

  43. Ch. Wöll, Thesis (University of Gottingen, 1987); Max-Planck-Institut für Strömungs-forschung, Report 18/1987. The calculation of a one layer two dimensional lattice is described in O. Madelung, Festkörpertheorie II (Springer, Berlin 1972).

    Google Scholar 

  44. R. Berndt, Diplom thesis ( University of Göttingen, 1987).

    Google Scholar 

  45. G. Benedek, J. Ellis, A. Reichmuth, P. Ruggerone, H. Schief and J.P. Toennies, Phys. Rev. Lett. 69 (1992) 2951.

    Article  ADS  Google Scholar 

  46. G. Benedek, G.P. Brivio, L. Miglio and V.R. Velasco, Phys. Rev. B26 (1982) 497.

    ADS  Google Scholar 

  47. G. Benedek and L. Miglio, in: Ab-Initio Calculation of Phonon Spectra, Eds. J.T. Devreese, V.E. van Doren and P.E. Van Camp (Plenum, New York 1983).

    Google Scholar 

  48. G. Brusdeylins, R.B. Doak, and J.P. Toennies, Phys. Rev. B 27 (1983) 3662.

    Article  ADS  Google Scholar 

  49. G. Brusdeylins, R. Rechsteiner, J.G. Skofronick, J.P. Toennies, G. Benedek and L. Miglio, Phys. Rev. Lett., 54 (1985) 466.

    Article  ADS  Google Scholar 

  50. A.A. Lucas, J. Chem. Phys. 48 (1968) 3156.

    Article  ADS  Google Scholar 

  51. L. Miglio and G. Benedek, in: Structure and Dynamics of Surfaces II, Eds. W. Duke and P. von Blanckenhagen (Springer, Heidelberg 1987) p. 35.

    Google Scholar 

  52. W.J.L. Buyers, Phys. Rev. 153 (1967) 923

    Article  ADS  Google Scholar 

  53. P. Santini, L. Miglio, G. Benedek, U. Harten, P. Ruggerone and J.P. Toennies, Phys. Rev. B42 (1990) 11942.

    ADS  Google Scholar 

  54. Y.R. Wang and C.B. Duke, Surf. Sci. 205 (1988) L755.

    Article  ADS  Google Scholar 

  55. J.L.T. Waugh and G. Dolling, Phys. Rev. 132 (1963) 2410.

    Article  ADS  Google Scholar 

  56. L. Miglio, P. Santini, P. Ruggerone and G. Benedek, Phys. Rev.Lett. 62 (1989) 3070.

    Article  ADS  Google Scholar 

  57. M.W. Finnis and V. Heine, J. Phys. F (Metal Phys). 4 (1974) L37.

    Article  ADS  Google Scholar 

  58. S. Lehwald, F. Wolf, H. Ibach, B.M. Hall and D.L. Mills, Surf. Sci. 192 (1987) 131.

    Article  Google Scholar 

  59. R.B. Doak, U. Harten, and J.P. Toennies, Phys. Rev.Lett. 51 (1983) 578.

    Article  ADS  Google Scholar 

  60. W. Drexel, Z. Phys. 255 (1977) 281.

    ADS  Google Scholar 

  61. W. Kohn, Phys. Rev. Lett. 2 (1959) 393.

    Article  ADS  Google Scholar 

  62. H.-J. Ernst, E. Hulpke and J.P. Toennies, Europhys. Lett. 10 (1989) 747.

    Article  ADS  Google Scholar 

  63. A. Larose and B.N. Brockhouse, Can. J. Phys. 54 (1976) 1819.

    ADS  Google Scholar 

  64. E. Hulpke and J. Lüdecke, Phys. Rev. Lett. 68 (1992) 2846.

    Article  ADS  Google Scholar 

  65. E. Hulpke and J. Lüdecke, Surface Sci. 287/288 (1993) 837.

    Article  ADS  Google Scholar 

  66. J.C. Phillips, Phys. Rev. 166 (1968) 832

    Article  ADS  Google Scholar 

  67. S.K. Sinha, Crit. Rev. Solid State Sci. 3 (1973) 273.

    Article  Google Scholar 

  68. C. Falter, Physics Reports 164 (1988) 1.

    Article  ADS  Google Scholar 

  69. R.M. Martin, Chem. Phys. Lett. 2 (1968) 268; Phys. Rev. 186 (1969) 871.

    Article  ADS  Google Scholar 

  70. F.A. Johnson, Proc. R. Soc. (London) Ser. A 339 (1974) 73.

    Article  ADS  Google Scholar 

  71. W. Weber, Phys. Rev. Lett. 33 (1974) 371; Phys. Rev. B15 (1977) 4789.

    Article  ADS  Google Scholar 

  72. K.C. Rustagi and W. Weber, Solid State Comm. 18 (1976) 1027.

    Google Scholar 

  73. D. Hanneman, Rep. Prog. Phys. 50 (1987) 1045.

    Article  ADS  Google Scholar 

  74. H. Ibach, Phys. Rev. Lett. 27 (1971) 253.

    Article  ADS  Google Scholar 

  75. U. Harten, J.P. Toennies, and Ch. Wöll, Phys. Rev. Lett. 57 (1986) 2947.

    Article  ADS  Google Scholar 

  76. K.C. Pandey, Phys. Rev. Lett. 47 (1981) 1913; 49 (1982) 223.

    Article  ADS  Google Scholar 

  77. E. Northrup and M.L. Cohen, Phys. Rev. Lett. 49 (1982) 1349; J. Vac. Sci. Technol. 21 (1982) 333.

    Article  ADS  Google Scholar 

  78. F.J. Himpsel, P.M. Marcus, R. Tromp, I.P. Batra, M.R. Cook, F. Jona, H. Liu, Phys. Rev. B30 (1984) 2257.

    ADS  Google Scholar 

  79. T. Takayanagi, Y. Tanshiro, M. Takahashi and S. Takahashi, J. Vac. Sci. Technol. A3 (1985) 1502; Surf. Sci. 164 (1985) 367.

    ADS  Google Scholar 

  80. G. Lange, P. Ruggerone, G. Benedek and J. P. Toennies, Europhys. Lett. (1998, to appear)

    Google Scholar 

  81. U. Harten, J. P. Toennies, Ch. Wöll, L. Miglio, P. Ruggerone, L. Colombo and G. Benedek, Phys. Rev. B 38 (1988) 3305.

    Article  ADS  Google Scholar 

  82. J. Kim, M. Yeh, F.S. Khan, and J.W. Wilkins, Phys. Rev. B52 (1995) 14709

    ADS  Google Scholar 

  83. I. Štich, J. Kohanoff, and K. Terakura, Phys. Rev. B 54, 2642 (1996).

    Article  ADS  Google Scholar 

  84. W. Mönch, Semiconductor Surfaces and Interfaces, Springer, Berlin 1993, p. 96

    Google Scholar 

  85. H. Lüth and R. Matz, Phys. Rev. Lett. 46 (1981) 1652

    Article  ADS  Google Scholar 

  86. L.H. Dubois and G.P. Schwartz, Phys. Rev. B26 (1982) 794

    ADS  Google Scholar 

  87. T.J. Godin, J.P. La Femina and C.B. Duke, J. Vac. Sci. Technol. B 9 (1991) 2282.

    Article  Google Scholar 

  88. J. Fritsch, P. Pavone and U. Schröder, Phys. Rev. Lett. 71 (1993) 4194.

    Article  ADS  Google Scholar 

  89. R. de Felice, A. I. Shkrebtii, F. Finocchi, C.M. Bertoni and G. Onida, J. El. Spectr. Rel. Phenom., 64/65 (1995) 697.

    Article  Google Scholar 

  90. W.G. Schmidt, F. Bechstedt and G.P. Srivastava, Phys. Rev. B 52 (1995) 2001.

    Article  ADS  Google Scholar 

  91. U. Harten and J.P. Toennies, Europhys. Lett. 4 (1987) 833.

    Article  ADS  Google Scholar 

  92. R.B. Doak and D.B. Nguyen, J. El. Spectr. Rel. Phenom., 44 (1987) 205.

    Article  Google Scholar 

  93. L.H. Dubois and G.P. Schwartz, Phys. Rev. B 26 (1982) 794.

    Article  ADS  Google Scholar 

  94. M.G. Betti, U. del Pennino and C. Mariani, Phys. Rev. B 39 (1989) 5887.

    Article  ADS  Google Scholar 

  95. H. Niehaus and W. Mönch, Phys. Rev. B 50 (1994) 11750.

    Article  ADS  Google Scholar 

  96. For an introduction to early P&P experiments see, e.g., S. L. Shapiro, ed., Topics in Applied Physics (Springer-Verlag, Heidelberg 1977), Vol. 18.

    Google Scholar 

  97. R. Merlin, in Highlights In Condensed Matter Physics and Materials Science, edited by M. Cardona and A. Pinczuk as a special issue of Sol. St. Comm. 102 (1997) 207.

    Google Scholar 

  98. D. von der Linde, J. Kuhl and H. Klingenberg, Phys. Rev. Lett. 44 (1980) 1505.

    Article  ADS  Google Scholar 

  99. J. A. Kash, J. C. Tsang and J. M. Hvam, Phys. Rev. Lett. 54 (1985) 2151.

    Article  ADS  Google Scholar 

  100. W. Kütt, in Festkörperprobleme, Advances in Solid State Physics, Vol. 32, U. Rössler ed. (Vieweg, Braunschweig, 1992); T. Dekorsy, W. Kütt, T. Pfeifer and H. Kurz, Europhys. Lett. 23 (1993) 223.

    Google Scholar 

  101. T. K. Cheng, L. H. Acioli, J. Vidal, H. J. Zeiger, G. Dresselhaus, M. S. Dresselhaus and E. P. Ippen, Appl. Phys. Lett. 62 (1993) 1901.

    Article  ADS  Google Scholar 

  102. O. B. Wright and K. Kawashima, Phys. Rev. Lett. 69 (1992) 1668.

    Article  ADS  Google Scholar 

  103. M. Nisoli, S. Stagira, S. de Silvestri, A. Stella, P. Tognini, P. Cheyssac and R. Kofman, Phys. Rev. Lett. 78 (1997) 3575

    Article  ADS  Google Scholar 

  104. J. Ding, D. M. Photiadis and Z. Barber, Bull. Am. Phys. Soc. 42 (1997) 82.

    Google Scholar 

  105. C. Rocke, S. Zimmermann, A. Wixworth, J. P. Kotthaus, G. Bohm and G. Weinman, Phys. Rev. Letters 78, 4009 (1997).

    Article  ADS  Google Scholar 

  106. V. I. Talyanskii, J. M. Shilton, M. Pepper, C. G. Smith, C.J.B. Ford, E.H. Linfield, D.A. Ritchie and G.A.C. Jones, Phys. Rev. B 56, 15180 (1997).

    Article  ADS  Google Scholar 

  107. H. Totland, Ø.L. Bø and Y.M. Galperin, Phys. Rev. B 56, 15299 (1997).

    Article  ADS  Google Scholar 

  108. N.-H. Ge, C.M. Wong, R.L.Lingle, Jr., J.D. McNeill, K.J. Gaffney and C.B. Harris, Science, 279, 202 (1998). Se also the report by U. Höfer in Science, 279, 190 (1998).

    Article  ADS  Google Scholar 

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Benedek, G. (2002). Surface Phonons and their Role in Ultrafast Phenomena. In: Di Bartolo, B., Gambarota, G. (eds) Ultrafast Dynamics of Quantum Systems. NATO Science Series: B:, vol 372. Springer, Boston, MA. https://doi.org/10.1007/0-306-47080-2_8

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  • DOI: https://doi.org/10.1007/0-306-47080-2_8

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