Chapter

Ultrafast Phenomena XV

Volume 88 of the series Springer Series in Chemical Physics pp 371-373

Coherently Controlled Multidimensional Optical Spectroscopy

  • Katherine W. StoneAffiliated withMassachusetts Institute of Technology
  • , Thomas HornungAffiliated withMassachusetts Institute of Technology
  • , Joshua C. VaughanAffiliated withMassachusetts Institute of Technology
  • , Keith A. NelsonAffiliated withMassachusetts Institute of Technology

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Abstract

Multidimensional optical spectroscopy of potassium dimer is demonstrated using a 2D femtosecond pulse shaper with excellent phase stability. Coherent control of intramolecular dynamics is achieved by introducing specific pulse sequences and chirps.