, Volume 85, Issue 11, pp 539-543

Fiber-optic synthesizer of controlled sequences of ultrashort light pulses for single-beam coherent anti-Stokes Raman scattering microspectroscopy

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Abstract

A photonic-crystal fiber operated in the regime of modulation instability is shown to simultaneously enable efficient spectral transformation and pulse shaping of laser fields, synthesizing optimal field waveforms for single-beam coherent anti-Stokes Raman scattering and coherence-controlled excitation of molecular systems.