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Heterostructured graphene quantum dot/WSe2/Si photodetector with suppressed dark current and improved detectivity

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Abstract

A high-performance heterojunction photodetector is formed by combining an n-type Si substrate with p-type monolayer WSe2 obtained using physical vapor deposition. The high quality of the WSe2/Si heterojunction is demonstrated by the suppressed dark current of 1 nA and the extremely high rectification ratio of 107. Under illumination, the heterojunction exhibits a wide photoresponse range from ultraviolet to near-infrared radiation. The introduction of graphene quantum dots (GQDs) greatly elevates the photodetective capabilities of the heterojunction with strong light absorption and long carrier lifetimes. The GQDs/WSe2/Si heterojunction exhibits a high responsivity of ∼ 707 mA·W–1, short response time of 0.2 ms, and good specific detectivity of ∼ 4.51 × 109 Jones. These properties suggest that the GQDs/WSe2/Si heterojunction holds great potential for application in future high-performance photodetectors.

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Acknowledgements

This work was supported by the National Natural Science Foundation of China (NSFC) (Nos. 51672154 and 51372130), MoST(No. 2016YFA0200200), Natural Science Foundation of Jiangsu Province (No. BK20160328), and Open Research Fund Program of the State Key Laboratory of Low-Dimensional Quantum Physics (No. KF201517).

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Authors and Affiliations

  1. Institute of Microelectronics & Tsinghua National Laboratory for Information Science and Technology (TNList), Tsinghua University, Beijing, 100084, China

    Mengxing Sun, Dan Xie, Yilin Sun, Changjiu Teng, Weiwei Li & Tianling Ren

  2. Department of Materials Science and Engineering, College of Engineering, Peking University, Beijing, 100084, China

    Qiyi Fang & Yanfeng Zhang

  3. Department of Chemistry, Tsinghua University, Beijing, 100084, China

    Liu Qian

  4. Institute of Functional Nano & Soft Materials (FUNSOM), Jiangsu Key Laboratory for Carbon-Based Functional Materials & Devices, Soochow University, Suzhou, 215123, China

    Jianlong Xu & Peng Xiao

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  1. Mengxing Sun
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  4. Yilin Sun
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Correspondence to Dan Xie or Yanfeng Zhang.

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Sun, M., Fang, Q., Xie, D. et al. Heterostructured graphene quantum dot/WSe2/Si photodetector with suppressed dark current and improved detectivity. Nano Res. 11, 3233–3243 (2018). https://doi.org/10.1007/s12274-017-1855-1

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  • DOI: https://doi.org/10.1007/s12274-017-1855-1

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