Abstract
The activity of natural radionuclides in soil has become an environmental concern for local public and national authorities because of the harmful effects of radiation exposure on human health. In this context, modelling and mapping the activity of natural radionuclides in soil is an important research topic. The study was aimed to model, in a spatial sense, the soil radioactivity in an urban and peri-urban soils area in southern Italy to analyse the seasonal influence on soil radioactivity. Measures of gamma radiation naturally emitted through the decay of radioactive isotopes (potassium, uranium and thorium) were analysed using a geostatistical approach to map the spatial distribution of soil radioactivity. The activity of three radionuclides was measured at 181 locations using a high-resolution ?-ray spectrometry. To take into account the influence of season, the measurements were carried out in summer and in winter. Activity data were analysed by using a geostatistical approach and zones of relatively high or low radioactivity were delineated. Among the main processes which influence natural radioactivity such as geology, geochemical, pedological, and ecological processes, results of this study showed a prominent control of radio-emission measurements by seasonal changes. Low natural radioactivity levels were measured in December associated with winter weather and moist soil conditions (due to high rainfall and low temperature), and higher activity values in July, when the soil was dry and no precipitations occurred.
Similar content being viewed by others
References
Agbalagba E O and Onoja R A 2011 Evaluation of natural radioactivity in soil, sediment and water samples of Niger Delta (Biseni) flood plain lakes, Nigeria; J. Environ. Radioact. 102 667–671.
Ajayi O S and Ibikunle S B 2013 Radioactivity of surface soils from Oyo state, Southwestern Nigeria; Int. J. Radiat. Res. 11 271–278.
Argyraki A and Kelepertzis E 2014 Urban soil geochemistry in Athens, Greece: The importance of local geology in controlling the distribution of potentially harmful trace elements; Sci. Total Environ. 482–483 366–377.
Askouri N A, Hussain M O and Al-Ojaily A -R S S 2011 Natural radioactivity survey in Al-Jabal Al-Gharbi Mountain Region Libya; Iraq J. Phys. 9 96–101.
Baciu A C 2006 Outdoor absorbed dose rate in air in relation to airborne natural radioactivity and meteorological conditions at Bucharest (Romania); J. Radioanal. Nucl. Ch. 268 3–14.
Beamish D 2013 Gamma ray attenuation in the soils of Northern Ireland, with special reference to peat; J. Environ. Radioact. 115 13–27.
Beamish D 2015 Relationships between gamma-ray attenuation and soils in SW England; Geoderma 259–260 174–186.
Bleines C, Deraisme J, Geoffrey F, Jeannée N, Perseval S, Rambert F, Renard D, Torres O and Touffait Y 2008 Isatis Software Manual, 5th edn, Géovariances & Ecole des Mines de Paris, Avon.
Bruno C, Buttafuoco G, Falcone G, Greco R, Guagliardi I, Iovine G and Tallarico A 2012 Soil gas radon concentrations in three study areas of Calabria (southern Italy); Rend. Online Soc. Geol. It. 21 381–383.
Buccianti A, Apollaro C, Bloise A, De Rosa R, Falcone G, Scarciglia F, Tallarico A and Vecchio G 2009 Natural radioactivity levels (K, Th, U and Rn) in the Cecita Lake area (Sila Massif, Calabria, southern Italy): An attempt to discover correlations with soil features on a statistical base; Geoderma 152 145–156.
Buttafuoco G, Tallarico A, Falcone G and Guagliardi I 2010 A geostatistical approach for mapping and uncertainty assessment of geogenic radon gas in soil in an area of southern Italy; Environ. Earth Sci. 61 491–505.
Buttafuoco G, Caloiero T and Coscarelli R 2011 Spatial and temporal patterns of the mean annual precipitation at decadal time scale in southern Italy (Calabria region); Theor. Appl. Climatol. 105 431–444.
Chandrasekaran A, Ravisankar R, Rajalakshmi A, Eswaran P, Vijayagopal P and Venkatraman B 2015 Assessment of natural radioactivity and function of minerals in soils of Yelagiri hills, Tamilnadu, India by gamma ray spectroscopic and Fourier transform infrared (FTIR) techniques with statistical approach; Spectrochim. Acta A 136 1734–1744.
Chilès J P and Delfiner P 2012 Geostatistics: Modelling spatial uncertainty, 2nd edn; Wiley, New York.
de Groot A V, van der Graaf E R, de Meijer R J and Maucec M 2009 Sensitivity of in-situ ?-ray spectra to soil density and water content; Nucl. Instrum. Meth. A 600 519–523.
Dent D L, MacMillan R A, Mayr T L, Chapman W K and Berch S M 2013 Use of airborne gamma radiometrics to infer soil properties for a forested area in British Columbia, Canada; J. Ecosyst. Manag. 14 1–12.
Dragovic S, Gajic B, Dragovic R, Jankovic-Mandic L, Slavkovic-Beškoski L, Mihailovic N, Momcilovic M and Cujic M 2012 Edaphic factors affecting the vertical distribution of radionuclides in the different soil types of Belgrade, Serbia; J. Environ. Monit. 14 127–137.
Fabbricatore D, Robustelli G and Muto F 2014 Facies analysis and depositional architecture of shelf-type deltas in the Crati Basin (Calabrian Arc, south Italy); It. J. Geosci. 133 131–148.
GF Instruments 2001 Geophysical gamma-ray spectrometer GRM-260; Operating manual version 2.0, Brno, Czech Republic.
Goovaerts P 1997 Geostatistics for natural resources evaluation; Oxford University Press, New York.
Guagliardi I, Cicchella D and De Rosa R 2012 A geostatistical approach to assess concentration and spatial distribution of heavy metals in urban soils; Water Air Soil Pollut. 223 5983–5998.
Guagliardi I, Apollaro C, Scarciglia F and De Rosa R 2013a Influence of particle-size on geochemical distribution of stream sediments in the Lese river catchment, southern Italy; Biotechnol. Agron. Soc. Environ. 17 43–55.
Guagliardi I, Buttafuoco G, Apollaro C, Bloise A, De Rosa R and Cicchella D 2013b Using gamma-ray spectrometry and geostatistics for assessing geochemical behaviour of radioactive elements in the Lese catchment (southern Italy); Int. J. Environ. Res. 7 645–658.
Guagliardi I, Buttafuoco G, Cicchella D and De Rosa R 2013c A multivariate approach for anomaly separation of potentially toxic trace elements in urban and peri-urban soils: An application in a southern Italy area ; J. Soil Sediment. 13 117–128.
Guagliardi I, Buttafuoco G, Ricca N, Cipriani M G, Civitelli D, Froio R, Gabriele A L and De Rosa R 2013d Modelling seasonal variations of natural radionuclides in agricultural soils; E3S Web of Conferences, doi:10.1051/e3sconf/20130108009.
Guagliardi I, Cicchella D, De Rosa R and Buttafuoco G 2015 Assessment of lead pollution in topsoils of a southern Italy area: Analysis of urban and peri-urban environment ; J. Environ. Sci. 33 179–187.
Guagliardi I, Rovella N, Apollaro C, Bloise A, De Rosa R, Scarciglia F and Buttafuoco G 2016 Effects of source rocks, soil features and climate on natural gamma radioactivity in the Crati valley (Calabria, southern Italy); Chemosphere 150 97–108.
Johnson S S 1979 Radioactivity surveys; Virginia Minerals 25 9–16.
Journel A G and Huijbregts C J 1978 Mining geostatistics; Academic, San Diego.
Korobova E M, Dogadkin N N, Shiryaev A A, Kolotov V P, Kononkova N N and Turkov V A 2014 A study of Cs-137 spatial distribution in soil thin sections by digital autoradiography and microscopy; J. Geochem. Explor. 142 94–100.
Le Pera E, Arribas J, Critelli S and Tortosa A 2001 The effects of source rocks and chemical weathering on the petrogenesis of siliciclastic sand from the Neto River (Calabria, Italy); Sedimentology 48 357–378.
Lebedyte M, Butkus D and Morkunas G 2003 Variations of the ambient dose equivalent rate in the ground level air; J. Environ. Radioact. 64 45–57.
Lesch S M and Corwin D L 2008 Prediction of spatial soil property information from ancillary sensor data using ordinary linear regression: model derivations, residual assumptions and model validation tests; Geoderma 148 130–140.
Maharana M, Krishnan N and Sengupta D 2010 Spatial distribution of gamma radiation levels in surface soils from Jaduguda uranium mineralization zone, Jharkhand, India, using ?-ray spectrometry, and determination of outdoor dose to the population; J. Med. Phys. 35 235–241.
Matheron G 1971 The theory of regionalised variables and its applications, Les Cahiers du Centre de Morphologie Mathématique de Fontainebleau 5.
McBratney A B, Odeh I O A, Bishop T F A, Dunbar M S and Shatar T M 2000 An overview of pedometric techniques for use in soil survey; Geoderma 97 293–327.
Milenkovic B, Stajic J M, Gulan L J, Zeremski T and Nikezic D 2015 Radioactivity levels and heavy metals in the urban soil of central Serbia; Environ. Sci. Pollut. R. Int. 22 16,732–16,741.
Munazza F, Mujahid S A and Matiullah 2008 Assessment of radiological hazards due to the natural radioactivity in soil and building material samples collected from six districts of the Punjab province-Pakistan; Radiat. Meas. 43 1443–1447.
Prasad B S N, Nagaraja T K, Chandrashekara M S, Paramesh L and Madhava M S 2005 Diurnal and seasonal variations of radioactivity and electrical conductivity near the surface for a continental location, Mysore, India; Atmos. Res. 76 65–77.
Priori S, Bianconi N and Costantini E A C 2014 Can ?-radiometrics predict soil textural data and stoniness in different parent materials? A comparison of two machine-learning methods; Geoderma 266–267 354–364.
Ramasamy V, Sundarrajan M, Paramasivam K and Suresh G 2015 Spatial and depth wise characterization of radionuclides and minerals in various beach sediments from high background radiation area, Kerala, India; Appl. Radiat. Isotopes 95 159–168.
Ricca N and Guagliardi I 2015 Multi-temporal dynamics of land use patterns in a site of community importance in southern Italy; Appl. Ecol. Environ. Res. 13 677–691.
Scarciglia F, Barca D, De Rosa R and Pulice I 2009 Application of laser ablation ICP–MS and traditional micromorphological techniques to the study of an Alfisol (Sardinia, Italy) in thin sections: Insights into trace element distribution; Geoderma 152 113–126.
Scarciglia F, Tuccimei P, Vacca A, Barca D, Pulice I, Salzano R and Soligo M 2011 Soil genesis, morphodynamic processes and chronological implications in two soil transects of SE Sardinia, Italy: Traditional pedological study coupled with laser ablation ICP-MS and radionuclide analyses; Geoderma 162 39–64.
Singh J, Singh H, Singh S, Bajwa B S and Sonkawade R G 2009 Comparative study of natural radioactivity levels in soil samples from the Upper Siwaliks and Punjab, India using gamma-ray spectrometry; J. Environ. Radioact. 100 94–98.
Wackernagel H 2003 Multivariate geostatistics: An introduction with applications; Springer-Verlag, Berlin.
Webster R and Oliver M A 2007 Geostatistics for environmental scientists, 2nd edn; Wiley, Chichester.
Wilding L P and Drees L R 1983 Spatial variability and pedology; In: Pedogenesis and soil taxonomy: I. Concepts and interactions (eds) Wilding L P, Smeck N E and Hall G F, Elsevier, Amsterdam, pp. 83–116.
Yamazaki K, Tonouchi S and Hashimoto T 2002 Factors associated with the variations in environmental gamma-ray spectra in Kashiwazaki Kariwa area; J. Radioanal. Nucl. Ch. 252 359–366.
Author information
Authors and Affiliations
Corresponding author
Additional information
Corresponding editor: Pulak Sengupta
Rights and permissions
About this article
Cite this article
Guagliardi, I., Rovella, N., Apollaro, C. et al. Modelling seasonal variations of natural radioactivity in soils: A case study in southern Italy. J Earth Syst Sci 125, 1569–1578 (2016). https://doi.org/10.1007/s12040-016-0758-y
Received:
Revised:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s12040-016-0758-y