Abstract
The results of a comparison between monthly mean ozone column variations calculated from the chemical transport model Oslo CTM2 and those derived from solar backscatter ultraviolet (SBUV) satellite observations are presented for the period 1998–2009. Monthly mean total ozone derived from improved model simulations were used to compute monthly zonal means over 10° latitude zones over the northern and southern hemispheres. Ozone column variations from Oslo CTM2 are highly correlated with SBUV retrievals at all latitude zones. Equatorial zonal winds at 30 hPa were used as index to study the impact of quasi-biennial oscillation (QBO) on ozone. Correlations between modeled ozone and the QBO were found to be the order of +0.8 in the tropics. The impact of QBO was most pronounced at equatorial latitudes with amplitudes of +4 to −4 %. Seasonal variations in surface ozone and tropospheric ozone column calculated by the model are also presented.
Similar content being viewed by others
References
Andersen, S. B., Weatherhead, E. C., Stevermer, A., Austin, J., Brühl, C., Fleming, E. L., de Grandpré, J., Grewe, V., Isaksen, I., Pitari, G., Portmann, R. W., Rognerud, B., Rosenfield, J. E., Smyshlyaev, S., Nagashima, T., Velders, G. J. M., Weisenstein, D. K., & Xia, J. (2006). Comparison of recent modelled and observed trends in total column ozone. Journal of Geophysical Research, 111, D02303. doi:10.1029/2005JD006091.
Balis, D., Isaksen, I. S. A., Zerefos, C., Zyrichidou, I., Eleftheratos, K., Tourpali, K., Bojkov, R., Rognerud, B., Stordal, F., Søvde, O. A., & Orsolini, Y. (2011). Observed and modelled record ozone decline over the Arctic during winter/spring 2011. Geophysical Research Letters, 38, L23801. doi:10.1029/2011GL049259.
Bhartia, P. K., Wellemeyer, C. G., Taylor, S. L., Nath, N., Gopolan, A. (2004). Solar backscatter ultraviolet (SBUV) version 8 profile algorithm. In: C.S. Zerefos (ed) Ozone, vol. I, 1–8 June 2004, Proceedings of the XX Quadrennial Ozone Symposium, pp. 295–296, Kos, Greece
Chipperfield, M. P., Fioletov, V. E. (Lead Authors), Bregman, B., Burrows, J., Connor, B. J., Haigh, J. D., Harris, N. R. P., Hauchecorne, A., Hood, L. L., Kawa, S. R., Krzyscin, J. W., Logan, J. A., Muthama, N. J., Polvani, L., Randel, W. J., Sasaki, T., Staehelin, J., Stolarski, R. S., Thomason, L. W., Zawodny, J. M. (2007) Global ozone: past and present, chapter 4. In: Scientific assessment of ozone depletion: 2006. Global ozone research and monitoring project, report no. 50. World Meteorological Organization, Geneva, pp 1–572.
Eleftheratos, K., Zerefos, C. S., Gerasopoulos, E., Isaksen, I. S. A., Rognerud, B., Dalsoren, S., & Varotsos, C. (2011). A note on the comparison between total ozone from Oslo CTM2 ans SBUV satellite data. International Journal of Remote Sensing, 32, 2535–2545. doi:10.1080/01431161003698401.
Eyring, V., Butchart, N., Waugh, D. W., Akiyoshi, H., Austin, J., et al. (2006). Assessment of temperature, trace species, and ozone in chemistry climate model simulations of the recent past. Journal of Geophysical Research, 111, D22308. doi:10.1029/2006JD007327.
Fioletov, V. E., Tarasick, D. W., & Petropavlovskikh, I. (2006). Estimating ozone variability and instrument uncertainties from SBUV(/2), ozonesonde, Umkehr, and SAGE II measurements: short-term variations. Journal of Geophysical Research, 111, D02305. doi:10.1029/2005JD006340.
Gauss, M., Isaksen, I. S. A., Wong, S., Wang, W.-C. (2003). Impact of H2O emissions from cryoplanes and kerosene aircraft on the atmosphere. Journal of Geophysical Research, 108, doi:10.1029/2002JD002623.
Harris, N. R. P., Ancellet, G., Bishop, L., Hofmann, D. J., Kerr, J. B., McPeters, R. D., Prendez, M., Randel, W. J., Staehelin, J., Subbaraya, B. H., Volz-Thomas, A., Zawodny, J., & Zerefos, C. S. (1997). Trends in stratospheric and free tropospheric ozone. Journal of Geophysical Research, 102, 1571–1590.
Isaksen, I. S. A., Rognerud, B., Stordal, F., Coffey, M. T., & Mankin, W. G. (1990). Studies of Arctic stratospheric ozone in a 2-d model including some effects of zonal asymmetries. Geophysical Research Letters, 17, 557–560.
Isaksen, I. S. A., Zerefos, C., Kourtidis, K., Meleti, C., Dalsøren, S. B., Sundet, J. K., Grini, A., Zanis, P., & Balis, D. (2005). Tropospheric ozone changes at unpolluted and semipolluted regions induced by stratospheric ozone changes. Journal of Geophysical Research, 110, D02302. doi:10.1029/2004JD004618.
Isaksen, I. S. A., Zerefos, C. S., Wang, W.-C., Balis, D., Eleftheratos, K., Rognerud, B., Stordal, F., Berntsen, T., LaCasce, J. H., Sovde, O. A., Olivie, D., Orsolini, Y. J., Zyrichidou, E., Prather, M. J., & Tuinder, O. (2012). Attribution of the Arctic ozone column deficit in March 2011. Geophysical Research Letters, 39, L24810. doi:10.1029/2012GL053876.
McPeters, R., Stolarski, R., Frith, S. (2011). A long-term merged global ozone data set Proceedings of the 34th International Symposium on Remote Sensing of Environment. The GEOSS Era: Towards Operational Environmental Monitoring, Sydney, Australia, 10–15 April 2011.
Nazaryan, H., & McCormick, M. P. (2005). Comparisons of stratospheric aerosol and gas experiment (SAGE II) and solar backscatter ultraviolet instrument (SBUV/2) ozone profiles and trend estimates. Journal of Geophysical Research, 110, D17302. doi:10.1029/2004JD005483.
Petropavlovskikh, I., Ahn, C., Bhartia, P. K., & Flynn, L. E. (2005). Comparison and covalidation of ozone anomalies and variability observed in SBUV(/2) and Umkehr northern midlatitude ozone profile estimates. Geophysical Research Letters, 32, L06805. doi:10.1029/2004GL022002.
Søvde, O. A., Gauss, M., Smyshlyaev, S. P., & Isaksen, I. S. A. (2008). Evaluation of the chemical transport model Oslo CTM2 with focus on arctic winter ozone depletion. Journal of Geophysical Research, 113, D09304. doi:10.1029/2007JD009240.
Stolarski, R. S., Douglass, A. R., Steenrod, S., & Pawson, S. (2006). Trends in stratospheric ozone: Lessons learned from a 3D chemical transport model. Journal of the Atmospheric Sciences, 63, 1028–1041.
Terao, Y., & Logan, J. A. (2007). Consistency of time series and trends of stratospheric ozone as seen by ozonesonde, SAGE II, HALOE, and SBUV(/2). Journal of Geophysical Research, 112, D06310. doi:10.1029/2006JD007667.
Varotsos, C. (1989). Comment on connections between the 11-year solar cycle, the Q.B.O. and total ozone. Journal of Atmospheric and Terrestrial Physics, 51, 367–370.
Varotsos, C. A., Cracknell, A. P., & Tzanis, C. (2012). The exceptional ozone depletion over the Arctic in January–March 2011. Remote Sensing Letters, 3, 343–352.
WMO (2012) World Data Centre for Greenhouse Gases (WDCGG) Data Summary, WDCGG no. 36, 106 pages
Zerefos, C. S. (1983). On the quasi-biennial oscillation in stratospheric temperatures and total ozone. Advances in Space Research, 2, 177–181.
Acknowledgments
The COMECAP 2012 Conference, Athens, Greece. The Mariolopoulos-Kanaginis Foundation for the Environmental Sciences
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Eleftheratos, K., Isaksen, I., Zerefos, C. et al. Ozone Variations Derived by a Chemical Transport Model. Water Air Soil Pollut 224, 1585 (2013). https://doi.org/10.1007/s11270-013-1585-2
Received:
Accepted:
Published:
DOI: https://doi.org/10.1007/s11270-013-1585-2