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Vapor Phase Synthesis of Annelated Pyridines over Metal Modified Zeolite Beta

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Abstract

Vapor phase synthesis of annelated pyridines from cyclic ketones, aldehydes and ammonia was carried out over various zeolite molecular sieves like Hβ, HZSM-5 (240), HZSM-5 (40), HY, HX, HMCM-41 and Mordenite. The preliminary screening of catalyst clearly shows that Hβ catalyst was found to be more active for the vapor phase synthesis of annelated pyridines. Hβ was further modified with transition metals like Fe, Cu, Pb, Mo, Zn, Ni, Co, Ce, W and Sn to get higher yields.

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Acknowledgments

We thank the CSIR Network project CSC-0123 for financial support. M.A.K., M.M.R. and M.N., thank the CSIR and. P.S. and K.S. the UGC, India for a fellowship.

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Authors and Affiliations

  1. I&PC Division, CSIR-IICT, Hyderabad, 500 007, India

    Arun Kumar Macharla, Mahender Reddy Marri, Swamy Peraka, Naresh Mameda, Srujana Kodumuri, V. V. Krishna Mohan Kandepi & Narender Nama

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  1. Arun Kumar Macharla
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  2. Mahender Reddy Marri
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  3. Swamy Peraka
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  6. V. V. Krishna Mohan Kandepi
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  7. Narender Nama
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Correspondence to V. V. Krishna Mohan Kandepi or Narender Nama.

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Macharla, A.K., Marri, M.R., Peraka, S. et al. Vapor Phase Synthesis of Annelated Pyridines over Metal Modified Zeolite Beta. Catal Lett 145, 1922–1930 (2015). https://doi.org/10.1007/s10562-015-1598-0

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