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Photochromism in single nitrogen-vacancy defect in diamond

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Abstract

Photochromism in single nitrogen-vacancy optical centers in diamond is demonstrated. Time-resolved optical spectroscopy shows that intense irradiation at 514 nm switches the nitrogen-vacancy defects to the negative form. This defect state relaxes back to the neutral form under dark conditions. Temporal anticorrelation of photons emitted by the different charge states of the optical center unambiguously indicates that the nitrogen-vacancy defect accounts for both 575 nm and 638 nm emission bands. Possible mechanism of photochromism involving nitrogen donors is discussed.

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References

  1. Gruber A, Drabenstedt A, Tietz C, Fleury L, Wrachtrup J, von Borczyskowski C (1997) Science 276:2012

    Article  Google Scholar 

  2. Jelezko F, Gaebel T, Popa I, Gruber A, Wrachtrup J (2004) Phys. Rev. Lett. 92:076401

    Article  PubMed  ADS  Google Scholar 

  3. Jelezko F, Popa I, Gruber A, Tietz C, Wrachtrup J, Nizovtsev A, Kilin S (2002) Appl. Phys. Lett. 81:2160

    Article  ADS  Google Scholar 

  4. Jelezko F, Gaebel T, Popa I, Domhan M, Gruber A, Wrachtrup J (2004) Phys. Rev. Lett. 93:130501

    Article  PubMed  ADS  Google Scholar 

  5. Popa I, Gaebel T, Domhan M, Wittmann C, Jelezko F, Wrachtrup J (2004) Phys. Rev. B 70:201203

    Article  ADS  Google Scholar 

  6. Davies G (1977) Nature 269:498

    Article  ADS  Google Scholar 

  7. J. Meijer, B. Burchard, M. Domhan, C. Wittmann, T. Gaebel, I. Popa, F. Jelezko, J. Wrachtrup, cond-mat/0505063 (2005) APL, in print

  8. J.R. Rabeau, G. Tamanyan, P. Reichart, D.N. Jamieson, S. Prawer F. Jelezko, T. Gaebel, I. Popa, M. Domhan, J. Wrachtrup, In preparation

  9. Davies G, Hamer MF (1976) Proc. R. Soc. Lon. Ser.-A 348:285

    Article  ADS  Google Scholar 

  10. Zaitsev AM (2001) Optical Properties of Diamond. Springer, Berlin, Heidelberg, NY

    Google Scholar 

  11. Mita Y (1996) Phys. Rev. B 53:11360

    Article  ADS  Google Scholar 

  12. Iakoubovskii K, Adriaenssens GJ, Nesladek M (2000) J. Phys.-Condens. Mat. 12:189

    Article  ADS  Google Scholar 

  13. Kupriyanov IN, Gusev AV, Pal’yanov YN, Borzdov YM (2000) J. Phys.-Condens. Mat. 12:7843

    Article  ADS  Google Scholar 

  14. Manson NB, Harrison JP (2005) Diam. Relat. Mater. 14:1705

    Article  Google Scholar 

  15. Steeds JW, Charles SJ, Davies J, Griffin I (2000) Diam. Relat. Mater. 9:397

    Article  Google Scholar 

  16. Wang WY, Moses T, Linares RC, Shigley JE, Hall M, Butler JE (2003) Gems & Gemology 39:268

    Google Scholar 

  17. Beveratos A, Brouri R, Gacoin T, Poizat JP, Grangier P (2001) Phys. Rev. A 64:061802

    Article  ADS  Google Scholar 

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Correspondence to T. Gaebel.

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61.72.-y;61.72.Ji;03.67.-a

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Gaebel, T., Domhan, M., Wittmann, C. et al. Photochromism in single nitrogen-vacancy defect in diamond. Appl. Phys. B 82, 243–246 (2006). https://doi.org/10.1007/s00340-005-2056-2

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  • DOI: https://doi.org/10.1007/s00340-005-2056-2

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