Abstract
The combined effects of electron-hole correlation, hydrostatic pressure, and temperature on the third harmonic generation in disk-shaped parabolic GaAs quantum dots are studied under the density matrix formalism and the effective mass approximation. Two well-defined regimes are discussed: (1) the strong-confinement regime, where the Coulomb interaction between the electron and hole is neglected and (2) the weak-confinement regime where the parabolic confinement term is neglected and the system reaches the limit of a hydrogenic problem. The results show that the third harmonic-generation coefficient is strongly dependent on the localization of the electron-hole pair. Also, that by using external perturbations like hydrostatic pressure or by considering the temperature effects it is possible to induce a blue-shift and/or red-shift on the resonant peaks of the third harmonic generation coefficient.
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Acknowledgments
CAD and MEMR wish to thank Mexican CONACYT and Colombian COLCIENCIAS for support under 2008 bilateral Grant "Estudio de propiedades ópticas y electrónicas en nanoestructuras y sistemas semiconductores de baja dimensión". This research was partially supported by Colombian Agencies: CODI-Universidad de Antioquia (Estrategia de Sostenibilidad Grupo de Materia Condensada-UdeA, 2009-2010, 2010-2011), Facultad de Ciencias Exactas y Naturales-Universidad de Antioquia (CAD-exclusive dedication project 2010-2011), and the Excellence Center for Novel Materials/COLCIENCIAS (Contract no. 043-2005). This study was developed with the help of CENAPAD-SP, Brazil.
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Duque, C.M., Mora-Ramos, M.E. & Duque, C.A. Simultaneous effects of electron-hole correlation, hydrostatic pressure, and temperature on the third harmonic generation in parabolic GaAs quantum dots. J Nanopart Res 13, 6103–6112 (2011). https://doi.org/10.1007/s11051-011-0348-5
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DOI: https://doi.org/10.1007/s11051-011-0348-5