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Adsorption of 4He N and 4He N 3He Clusters on Cesium

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Abstract

The ground-state properties of helium clusters 4He N and 4He N 3He, for N≤ 40, adsorbed on the surface of cesium are studied using variational and diffusion Monte Carlo calculations. Binding properties are determined using two different Cs–He interaction potentials. For the smallest clusters, self-binding on a Cs surface is stronger than in two or three dimensions. For N > 10 self-binding in three dimensions is stronger than on Cs for both types of Cs–He interaction potential considered. The obtained binding energies and structure are compared to results of recent density functional calculations. The emergence of edge states of 3He atom, localized along the contact line of 4He cluster with a cesium surface, is studied. First indication that 3He atom prefers to be close to the contact line appears already for the 4He3 3He cluster.

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References

  1. M. Barranco, R. Guardiola, S. Hernandez, R. Mayol, J. Navarro, M. Pi, J. Low Temp. Phys. 142, 1 (2006)

    Article  ADS  Google Scholar 

  2. E. Cheng, M.W. Cole, J. Dupont-Roc, W.F. Saam, J. Treiner, Rev. Mod. Phys. 65, 557 (1993)

    Article  ADS  Google Scholar 

  3. W.F. Saam, J. Low Temp. Phys. 157, 77 (2009)

    Article  Google Scholar 

  4. P. Taborek, J. Low Temp. Phys. 157, 101 (2009)

    Article  Google Scholar 

  5. S.M. Gatica, M.W. Cole, J. Low Temp. Phys. 157, 111 (2009)

    Article  Google Scholar 

  6. D. Ross, J.E. Rutledge, P. Taborek, Science 278, 664 (1997)

    Article  ADS  Google Scholar 

  7. L. Pricaupenko, J. Treiner, Phys. Rev. Lett. 72, 2215 (1994)

    Article  ADS  Google Scholar 

  8. D. Ross, J.A. Phillips, J.E. Rutledge, P. Taborek, J. Low Temp. Phys. 106, 81 (1997)

    Article  ADS  Google Scholar 

  9. R.B. Hallock, J. Low Temp. Phys. 121, 441 (2000)

    Article  Google Scholar 

  10. P.-C. Ho, R.B. Hallock, J. Low Temp. Phys. 121, 501 (2000) and references therein

    Article  Google Scholar 

  11. R. Mayol, M. Barranco, E.S. Hernandez, M. Pi, M. Guilleumas, Phys. Rev. Lett. 90, 185301 (2003)

    Article  ADS  Google Scholar 

  12. M. Barranco, M. Guilleumas, E.S. Hernandez, R. Mayol, M. Pi, L. Szybisz, J. Low Temp. Phys. 136, 139 (2004)

    Article  ADS  Google Scholar 

  13. S. Kilić, L. Vranješ, Physica B 329–333, 270 (2003)

    Article  Google Scholar 

  14. R.A. Aziz, F.R.W. McCourt, C.C.K. Wong, Mol. Phys. 61, 1487 (1987)

    Article  ADS  Google Scholar 

  15. L.W. Bruch, M.W. Cole, E. Zaremba, Physical Adsorption: Forces and Phenomena (Oxford University Press, New York, 1997)

    Google Scholar 

  16. F. Ancilotto, A.M. Sartori, F. Toigo, Phys. Rev. B 58, 5085 (1998)

    Article  ADS  Google Scholar 

  17. A. Chizmeshya, M.W. Cole, E. Zaremba, J. Low Temp. Phys. 110, 677 (1998)

    Article  Google Scholar 

  18. J.D. White, J. Cui, M. Strauss, R.D. Diehl, F. Ancilotto, F. Toigo, Surf. Sci. 307, 1134 (1994)

    Article  ADS  Google Scholar 

  19. J. Boronat, J. Casulleras, Phys. Rev. B 49, 8920 (1994)

    Article  ADS  Google Scholar 

  20. S. Kilić, E. Krotscheck, L. Vranješ, J. Low Temp. Phys. 119, 715 (2000)

    Article  Google Scholar 

  21. L. Vranješ, S. Kilić, Phys. Rev. A 65, 042506 (2002)

    Article  ADS  Google Scholar 

  22. T. Korona, H.L. Williams, R. Bukowski, B. Jeziorski, K. Szalewicz, J. Chem. Phys. 106, 5109 (1997)

    Article  ADS  Google Scholar 

  23. A. Sarsa, J. Mur-Petit, A. Polls, J. Navarro, Phys. Rev. B 68, 224514 (2003)

    Article  ADS  Google Scholar 

  24. S. Fantoni, R. Guardiola, J. Navarro, Phys. Rev. A 70, 023206 (2004)

    Article  ADS  Google Scholar 

  25. S.A. Chin, E. Krotscheck, Phys. Rev. B 45, 852 (1992)

    Article  ADS  Google Scholar 

  26. S. Kilić, L. Vranješ, J. Low Temp. Phys. 134, 713 (2004)

    Article  ADS  Google Scholar 

  27. K.B. Whaley, Int. Rev. Phys. Chem. 13, 41 (1994)

    Article  Google Scholar 

  28. J. Casulleras, J. Boronat, Phys. Rev. B 52, 3654 (1995)

    Article  ADS  Google Scholar 

  29. J. Mur-Petit, A. Sarsa, J. Navarro, A. Polls, Phys. Rev. B 72, 104513 (2005)

    Article  ADS  Google Scholar 

  30. F. Dalfovo, A. Lastri, L. Prichaupenko, S. Stringari, J. Treiner, Phys. Rev. B 52, 1193 (1995)

    Article  ADS  Google Scholar 

  31. R. Mayol, M. Pi, M. Barranco, F. Dalfovo, Phys. Rev. Lett. 87, 145301 (2001)

    Article  ADS  Google Scholar 

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Correspondence to L. Vranješ Markić.

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Stipanović, P., Vranješ Markić, L., Bešlić, I. et al. Adsorption of 4He N and 4He N 3He Clusters on Cesium. J Low Temp Phys 166, 68–79 (2012). https://doi.org/10.1007/s10909-011-0406-5

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  • DOI: https://doi.org/10.1007/s10909-011-0406-5

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