Applied Physics B

, Volume 99, Issue 1, pp 285–297

Dy-doped Lu2SiO5 single crystal: spectroscopic characteristics and luminescence dynamics

  • G. Dominiak-Dzik
  • W. Ryba-Romanowski
  • R. Lisiecki
  • P. Solarz
  • M. Berkowski
Article

DOI: 10.1007/s00340-009-3852-x

Cite this article as:
Dominiak-Dzik, G., Ryba-Romanowski, W., Lisiecki, R. et al. Appl. Phys. B (2010) 99: 285. doi:10.1007/s00340-009-3852-x

Abstract

Spectroscopic and kinetics properties of Lu2SiO5:Dy3+ (LSO:Dy) single crystal with 1 and 5 at.% of activator were investigated. The polarised absorption and unpolarised emission spectra were measured at 10–300 K. Parameters characterising radiative relaxations of LSO:Dy were estimated by the Judd–Ofelt model. The crystal-field energy structure was derived from low-temperature optical spectra exhibiting the presence of two non-equivalent Dy3+ sites. It was found that dysprosium ions in site 1 and in site 2 do not form isolated subsystems; these subsystems are coupled by an effective spectral energy migration process. The LSO:Dy crystal exhibits a strong luminescence in the visible. Strong ion–ion interactions were observed for LSO:Dy (5 at.%); luminescence decays are non-exponential and the macro-parameter of donor–acceptor interaction Cda amounts to 5.3 (10−52 m6 s−1) and 7.8 (10−52 m6 s−1) at 10 and 300 K, respectively. Laser potential related to the 4F9/26H13/2 yellow luminescence in Dy:LSO was assessed based on evaluation of the emission cross section values. It was concluded that the crystal is a promising material for visible laser operation.

Copyright information

© Springer-Verlag 2009

Authors and Affiliations

  • G. Dominiak-Dzik
    • 1
  • W. Ryba-Romanowski
    • 1
  • R. Lisiecki
    • 1
  • P. Solarz
    • 1
  • M. Berkowski
    • 2
  1. 1.Institute of Low Temperature and Structure ResearchPolish Academy of SciencesWrocławPoland
  2. 2.Institute of PhysicsPolish Academy of SciencesWarsawPoland

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