Applied Physics B

, Volume 75, Issue 8, pp 803–815

Study of UV laser interaction with gold nanoparticles embedded in silica

  • F. Bonneau
  • P. Combis
  • J.L. Rullier
  • J. Vierne
  • M. Pellin
  • M. Savina
  • M. Broyer
  • E. Cottancin
  • J. Tuaillon
  • M. Pellarin
  • L. Gallais
  • J.Y. Natoli
  • M. Perra
  • H. Bercegol
  • L. Lamaignère
  • M. Loiseau
  • J.T. Donohue

DOI: 10.1007/s00340-002-1049-7

Cite this article as:
Bonneau, F., Combis, P., Rullier, J. et al. Appl Phys B (2002) 75: 803. doi:10.1007/s00340-002-1049-7

Abstract.

In order to resolve problems concerning the understanding and the control of laser-induced damage of silica optical elements, a collaboration between the CEA and different university laboratories has been undertaken. Ultra-pure silica model samples, seeded with gold nanoparticles whose diameter did not exceed 5 nm, were prepared. The aim in using these samples was to observe the mechanism of damage initiation that could be attributed to inclusions of nanometric size. This paper presents the different steps encountered during this study: preparation of the samples, the laser-induced damage tests, the Nomarski and atomic-force microscope observations of this damage and a series of experiments using a time-of-flight mass spectrometer at Argonne National Laboratory. The experimental data are then interpreted, and, in particular, compared to numerical simulations. A very encouraging result is the existence of a pre-damage phase at very low fluences that is not detectable by classical optical devices. The experimental means developed for such model samples should be transposable to the analysis of industrial glasses.

PACS: 61.80.Ba; 42.70.-a; 52.38.Mf

Copyright information

© Springer-Verlag 2002

Authors and Affiliations

  • F. Bonneau
    • 1
  • P. Combis
    • 1
  • J.L. Rullier
    • 1
  • J. Vierne
    • 1
  • M. Pellin
    • 2
  • M. Savina
    • 2
  • M. Broyer
    • 3
  • E. Cottancin
    • 3
  • J. Tuaillon
    • 3
  • M. Pellarin
    • 3
  • L. Gallais
    • 4
  • J.Y. Natoli
    • 4
  • M. Perra
    • 4
  • H. Bercegol
    • 5
  • L. Lamaignère
    • 5
  • M. Loiseau
    • 5
  • J.T. Donohue
    • 6
  1. 1.Département de Physique Théorique et Appliquée, CEA/DAM Ile de France, BP 12, 91680 Bruyères le Châtel, FranceFR
  2. 2.Materials Science Division, Argonne National Laboratory, Argonne, IL 60439, USAUS
  3. 3.Centre Agrégat LASIM and DPM, Université Claude Bernard Lyon 1 and CNRS, 69622 Villeurbanne, FranceFR
  4. 4.Institut Fresnel, Domaine Universitaire de St. Jérôme, 13397 Marseille, FranceFR
  5. 5.Département des Lasers de Puissance, CEA/Centre d’Etudes Scientifiques et Techniques d’Aquitaine, BP 2, 33114 Le Barp, FranceFR
  6. 6.Centre d’Etudes Nucléaires de Bordeaux-Gradignan, BP 120, 33175 Gradignan, FranceFR